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Title: Characterization of immiscible fluid displacement processes with various capillary numbers and viscosity ratios in 3D natural sandstone

Abstract

We characterize the influence of reservoir conditions upon multiphase flow, we calculated fluid displacements (drainage processes) in 3D pore spaces of Berea sandstone using two-phase lattice Boltzmann (LB) simulations. The results of simulations under various conditions were used to classify the resulting two-phase flow behavior into three typical fluid displacement patterns on the diagram of capillary number (Ca) and viscosity ratio of the two fluids (M). In addition, the saturation of the nonwetting phase was calculated and mapped on the Ca–M diagram. We then characterized dynamic pore-filling events (i.e., Haines jumps) from the pressure variation of the nonwetting phase, and linked this behavior to the occurrence of capillary fingering. The results revealed the onset of capillary fingering in 3D natural rock at a higher Ca than in 2D homogeneous granular models, with the crossover region between typical displacement patterns broader than in the homogeneous granular model. Furthermore, saturation of the nonwetting phase mapped on the Ca–M diagram significantly depends on the rock models. These important differences between two-phase flow in 3D natural rock and in 2D homogeneous models could be due to the heterogeneity of pore geometry in the natural rock and differences in pore connectivity. By quantifying two-phase fluidmore » behavior in the target reservoir rock under various conditions (e.g., saturation mapping on the Ca–M diagram), our approach could provide useful information for investigating suitable reservoir conditions for geo-fluid management (e.g., high CO2 saturation in CO2 storage).« less

Authors:
ORCiD logo [1];  [1];  [2]
  1. Kyushu Univ. (Japan)
  2. Kyushu Univ. (Japan) ; Univ. of Notre Dame, IN (United States)
Publication Date:
Research Org.:
Energy Frontier Research Centers (EFRC) (United States). Center for Geologic Storage of CO2 (GSCO2)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1388385
Alternate Identifier(s):
OSTI ID: 1344939
Grant/Contract Number:  
SC0012504; 15H01143; 24246148; SC0C12504
Resource Type:
Accepted Manuscript
Journal Name:
Advances in Water Resources
Additional Journal Information:
Journal Volume: 95; Journal Issue: C; Related Information: GSCO2 partners with University of Illinois Urbana-Champaign (lead); National Energy Technology Laboratory; Schlumberger; SINTEF; Stiftelsen Norsar; Texas Tech University; University of Notre Dame; University of Southern California; University of Texas at Austin; Wright State University; Journal ID: ISSN 0309-1708
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
58 GEOSCIENCES; defects; mechanical behavior; carbon sequestration; mesostructured materials

Citation Formats

Tsuji, Takeshi, Jiang, Fei, and Christensen, Kenneth T. Characterization of immiscible fluid displacement processes with various capillary numbers and viscosity ratios in 3D natural sandstone. United States: N. p., 2016. Web. doi:10.1016/j.advwatres.2016.03.005.
Tsuji, Takeshi, Jiang, Fei, & Christensen, Kenneth T. Characterization of immiscible fluid displacement processes with various capillary numbers and viscosity ratios in 3D natural sandstone. United States. https://doi.org/10.1016/j.advwatres.2016.03.005
Tsuji, Takeshi, Jiang, Fei, and Christensen, Kenneth T. Fri . "Characterization of immiscible fluid displacement processes with various capillary numbers and viscosity ratios in 3D natural sandstone". United States. https://doi.org/10.1016/j.advwatres.2016.03.005. https://www.osti.gov/servlets/purl/1388385.
@article{osti_1388385,
title = {Characterization of immiscible fluid displacement processes with various capillary numbers and viscosity ratios in 3D natural sandstone},
author = {Tsuji, Takeshi and Jiang, Fei and Christensen, Kenneth T.},
abstractNote = {We characterize the influence of reservoir conditions upon multiphase flow, we calculated fluid displacements (drainage processes) in 3D pore spaces of Berea sandstone using two-phase lattice Boltzmann (LB) simulations. The results of simulations under various conditions were used to classify the resulting two-phase flow behavior into three typical fluid displacement patterns on the diagram of capillary number (Ca) and viscosity ratio of the two fluids (M). In addition, the saturation of the nonwetting phase was calculated and mapped on the Ca–M diagram. We then characterized dynamic pore-filling events (i.e., Haines jumps) from the pressure variation of the nonwetting phase, and linked this behavior to the occurrence of capillary fingering. The results revealed the onset of capillary fingering in 3D natural rock at a higher Ca than in 2D homogeneous granular models, with the crossover region between typical displacement patterns broader than in the homogeneous granular model. Furthermore, saturation of the nonwetting phase mapped on the Ca–M diagram significantly depends on the rock models. These important differences between two-phase flow in 3D natural rock and in 2D homogeneous models could be due to the heterogeneity of pore geometry in the natural rock and differences in pore connectivity. By quantifying two-phase fluid behavior in the target reservoir rock under various conditions (e.g., saturation mapping on the Ca–M diagram), our approach could provide useful information for investigating suitable reservoir conditions for geo-fluid management (e.g., high CO2 saturation in CO2 storage).},
doi = {10.1016/j.advwatres.2016.03.005},
journal = {Advances in Water Resources},
number = C,
volume = 95,
place = {United States},
year = {Fri Mar 11 00:00:00 EST 2016},
month = {Fri Mar 11 00:00:00 EST 2016}
}

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Works referenced in this record:

Geological storage of CO2 in saline aquifers—A review of the experience from existing storage operations
journal, July 2010

  • Michael, K.; Golab, A.; Shulakova, V.
  • International Journal of Greenhouse Gas Control, Vol. 4, Issue 4
  • DOI: 10.1016/j.ijggc.2009.12.011

Lattice Boltzmann Simulations of Supercritical CO 2 –Water Drainage Displacement in Porous Media: CO 2 Saturation and Displacement Mechanism
journal, December 2014

  • Yamabe, Hirotatsu; Tsuji, Takeshi; Liang, Yunfeng
  • Environmental Science & Technology, Vol. 49, Issue 1
  • DOI: 10.1021/es504510y

Impact of Wettability on Pore-Scale Characteristics of Residual Nonaqueous Phase Liquids
journal, July 2009

  • Al-Raoush, Riyadh I.
  • Environmental Science & Technology, Vol. 43, Issue 13
  • DOI: 10.1021/es802566s

The effect of displacement rate on imbibition relative permeability and residual saturation
journal, June 2006

  • Nguyen, Viet Hoai; Sheppard, Adrian P.; Knackstedt, Mark A.
  • Journal of Petroleum Science and Engineering, Vol. 52, Issue 1-4
  • DOI: 10.1016/j.petrol.2006.03.020

Exploring capillary trapping efficiency as a function of interfacial tension, viscosity, and flow rate
journal, January 2011


Control of interfacial instabilities using flow geometry
journal, August 2012

  • Al-Housseiny, Talal T.; Tsai, Peichun A.; Stone, Howard A.
  • Nature Physics, Vol. 8, Issue 10
  • DOI: 10.1038/nphys2396

Real-time 3D imaging of Haines jumps in porous media flow
journal, February 2013

  • Berg, S.; Ott, H.; Klapp, S. A.
  • Proceedings of the National Academy of Sciences, Vol. 110, Issue 10
  • DOI: 10.1073/pnas.1221373110

Pore-scale imaging and modelling
journal, January 2013


Drainage in two-dimensional porous media: From capillary fingering to viscous flow
journal, October 2010


Viscous Fingering in Porous Media
journal, January 1987


A methodology for velocity field measurement in multiphase high‐pressure flow of CO 2 and water in micromodels
journal, April 2015

  • Kazemifar, Farzan; Blois, Gianluca; Kyritsis, Dimitrios C.
  • Water Resources Research, Vol. 51, Issue 4
  • DOI: 10.1002/2014WR016787

The study of heterogeneous two-phase flow around small-scale heterogeneity in porous sandstone by measured elastic wave velocities and lattice Boltzmann method simulation
journal, October 2014

  • Kitamura, Keigo; Jiang, Fei; Valocchi, Albert J.
  • Journal of Geophysical Research: Solid Earth, Vol. 119, Issue 10
  • DOI: 10.1002/2014JB011281

Impact of geometrical properties on permeability and fluid phase distribution in porous media
journal, September 2008


Mush microphysics and the reactivation of crystal‐rich magma reservoirs
journal, August 2014

  • Parmigiani, Andrea; Huber, Christian; Bachmann, Olivier
  • Journal of Geophysical Research: Solid Earth, Vol. 119, Issue 8
  • DOI: 10.1002/2014JB011124

Three-Dimensional Imaging of Pore-Scale Water Flooding Phenomena in Water-Wet and Oil-Wet Porous Media
journal, January 2014

  • Setiawan, Arief; Suekane, Tetsuya; Deguchi, Yoshihiro
  • Journal of Flow Control, Measurement & Visualization, Vol. 02, Issue 02
  • DOI: 10.4236/jfcmv.2014.22005

Dynamic Capillary Pressure in Porous Media: Origin of the Viscous-Fingering Length Scale
journal, December 1987


Numerical models and experiments on immiscible displacements in porous media
journal, April 1988


Crossover from capillary fingering to viscous fingering for immiscible unstable flow: Experiment and modeling
journal, July 2004


Two-phase flow in porous media: Crossover from capillary fingering to compact invasion for drainage
journal, February 2005


Crossover from fractal capillary fingering to compact flow: The effect of stable viscosity ratios
journal, October 2007


Growth activity during fingering in a porous Hele-Shaw cell
journal, August 2004


Influence of pore-scale disorder on viscous fingering during drainage
journal, August 2005


Two-Phase Flow: Structure, Upscaling, and Consequences for Macroscopic Transport Properties
journal, January 2012

  • Toussaint, R.; Måløy, K. J.; Méheust, Y.
  • Vadose Zone Journal, Vol. 11, Issue 3
  • DOI: 10.2136/vzj2011.0123

Experimental Study of Crossover from Capillary to Viscous Fingering for Supercritical CO 2 –Water Displacement in a Homogeneous Pore Network
journal, June 2012

  • Wang, Ying; Zhang, Changyong; Wei, Ning
  • Environmental Science & Technology, Vol. 47, Issue 1
  • DOI: 10.1021/es3014503

Lattice-Boltzmann simulations in reconstructed parametrized porous media
journal, July 2006

  • Ahrenholz, Benjamin; Tölke, Jonas; Krafczyk, Manfred
  • International Journal of Computational Fluid Dynamics, Vol. 20, Issue 6
  • DOI: 10.1080/10618560601024694

Changes in pore geometry and relative permeability caused by carbonate precipitation in porous media
journal, November 2014


Direct simulations of two-phase flow on micro-CT images of porous media and upscaling of pore-scale forces
journal, December 2014


Distribution of multiphase fluids in porous media: Comparison between lattice Boltzmann modeling and micro-x-ray tomography
journal, February 2008


Lattice Boltzmann simulations of binary fluid flow through porous media
journal, March 2002

  • Tölke, Jonas
  • Philosophical Transactions of the Royal Society of London. Series A: Mathematical, Physical and Engineering Sciences, Vol. 360, Issue 1792
  • DOI: 10.1098/rsta.2001.0944

Use of the Boltzmann Equation to Simulate Lattice-Gas Automata
journal, November 1988


Lattice-Boltzmann simulation of two-phase flow in porous media: LB SIMULATION OF TWO-PHASE FLOW
journal, January 2004

  • Pan, C.; Hilpert, M.; Miller, C. T.
  • Water Resources Research, Vol. 40, Issue 1
  • DOI: 10.1029/2003WR002120

Dynamics of slow drainage in porous media
journal, April 1992


Reconstruction of Berea sandstone and pore-scale modelling of wettability effects
journal, September 2003


Impact of interfacial tension on residual CO 2 clusters in porous sandstone
journal, March 2015


Evaluation of three lattice Boltzmann models for multiphase flows in porous media
journal, June 2011


Theory of the lattice Boltzmann method: From the Boltzmann equation to the lattice Boltzmann equation
journal, December 1997


Discrete Boltzmann equation model for nonideal gases
journal, January 1998


Kinetic theory representation of hydrodynamics: a way beyond the Navier–Stokes equation
journal, February 2006


Lattice-Boltzmann Method for Complex Flows
journal, January 2010


An adaptive scheme using hierarchical grids for lattice Boltzmann multi-phase flow simulations
journal, September 2006


A comparison study of multi-component Lattice Boltzmann models for flow in porous media applications
journal, March 2013


Lattice Boltzmann equation model for multi-component multi-phase flow with high density ratios
journal, February 2013


Numerical evaluation of two recoloring operators for an immiscible two-phase flow lattice Boltzmann model
journal, May 2012

  • Leclaire, Sébastien; Reggio, Marcelo; Trépanier, Jean-Yves
  • Applied Mathematical Modelling, Vol. 36, Issue 5
  • DOI: 10.1016/j.apm.2011.08.027

Diffusion properties of gradient-based lattice Boltzmann models of immiscible fluids
journal, May 2005


TeraFLOP computing on a desktop PC with GPUs for 3D CFD
journal, August 2008

  • Tölke, J.; Krafczyk, M.
  • International Journal of Computational Fluid Dynamics, Vol. 22, Issue 7
  • DOI: 10.1080/10618560802238275

Interfacial jumps and pressure bursts during fluid displacement in interacting irregular capillaries
journal, July 2012


Inertial effects during irreversible meniscus reconfiguration in angular pores
journal, December 2014


CO 2 wettability of seal and reservoir rocks and the implications for carbon geo-sequestration
journal, January 2015

  • Iglauer, Stefan; Pentland, C. H.; Busch, A.
  • Water Resources Research, Vol. 51, Issue 1
  • DOI: 10.1002/2014WR015553

Modeling the velocity field during Haines jumps in porous media
journal, March 2015


Study of immiscible displacements in porous media using a color-gradient-based multiphase lattice Boltzmann method
journal, April 2014


Works referencing / citing this record:

Wettability and Flow Rate Impacts on Immiscible Displacement: A Theoretical Model
journal, April 2018

  • Hu, Ran; Wan, Jiamin; Yang, Zhibing
  • Geophysical Research Letters, Vol. 45, Issue 7
  • DOI: 10.1002/2017gl076600

Fundamental Understanding of Water Movement in Gas Diffusion Layer under Different Arrangements Using Combination of Direct Modeling and Experimental Visualization
journal, January 2018

  • Satjaritanun, P.; Hirano, S.; Shum, A. D.
  • Journal of The Electrochemical Society, Vol. 165, Issue 13
  • DOI: 10.1149/2.0201814jes

Visualizing and quantifying the crossover from capillary fingering to viscous fingering in a rough fracture: CROSSOVER CAPILLARY TO VISCOUS FINGERING
journal, September 2017

  • Chen, Yi-Feng; Fang, Shu; Wu, Dong-Sheng
  • Water Resources Research, Vol. 53, Issue 9
  • DOI: 10.1002/2017wr021051

The impact of drainage displacement patterns and Haines jumps on CO2 storage efficiency
journal, October 2018


Pore-scale numerical modeling of coupled fluid flow and medium geometrical deformations in an unconsolidated porous medium
journal, December 2019

  • Nasrollahzadeh, Behnam; Akhlaghi Amiri, Hossein Ali; Ghabezloo, Siavash
  • The European Physical Journal Plus, Vol. 134, Issue 12
  • DOI: 10.1140/epjp/i2019-12946-9

Energy Conversion Reveals Regime Transition of Imbibition in a Rough Fracture
journal, September 2018

  • Hu, Ran; Wu, Dong-Sheng; Yang, Zhibing
  • Geophysical Research Letters, Vol. 45, Issue 17
  • DOI: 10.1029/2018gl079302

Pore-scale characteristics of multiphase flow in heterogeneous porous media using the lattice Boltzmann method
journal, March 2019


Experimental study of drying effects during supercritical CO2 displacement in a pore network
journal, August 2018


Generalized three-dimensional lattice Boltzmann color-gradient method for immiscible two-phase pore-scale imbibition and drainage in porous media
journal, March 2017

  • Leclaire, Sébastien; Parmigiani, Andrea; Malaspinas, Orestis
  • Physical Review E, Vol. 95, Issue 3
  • DOI: 10.1103/physreve.95.033306

Preferential Paths of Air-water Two-phase Flow in Porous Structures with Special Consideration of Channel Thickness Effects
journal, November 2019