Advancements in rationally designed PGM-free fuel cell catalysts derived from metal–organic frameworks
Abstract
Over the past several years, metal-organic framework (MOF)-derived platinum group metal free (PGM-free) electrocatalysts have gained considerable attention due to their high efficiency and low cost as potential replacement for platinum in catalyzing oxygen reduction reaction (ORR). In this review, we summarize the recent advancements in design, synthesis and characterization of MOF-derived ORR catalysts and their performances in acidic and alkaline media. As a result, we also discuss the key challenges such as durability and activity enhancement critical in moving forward this emerging electrocatalyst science.
- Authors:
-
- Argonne National Lab. (ANL), Lemont, IL (United States); Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Argonne National Lab. (ANL), Lemont, IL (United States)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Sustainable Transportation Office. Hydrogen Fuel Cell Technologies Office (HFTO); USDOE Office of Science (SC)
- OSTI Identifier:
- 1373936
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Materials Horizons
- Additional Journal Information:
- Journal Volume: 4; Journal Issue: 1; Journal ID: ISSN 2051-6347
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 36 MATERIALS SCIENCE; MOF; PGM-free; catalyst; fuel cell
Citation Formats
Barkholtz, Heather M., and Liu, Di -Jia. Advancements in rationally designed PGM-free fuel cell catalysts derived from metal–organic frameworks. United States: N. p., 2016.
Web. doi:10.1039/c6mh00344c.
Barkholtz, Heather M., & Liu, Di -Jia. Advancements in rationally designed PGM-free fuel cell catalysts derived from metal–organic frameworks. United States. https://doi.org/10.1039/c6mh00344c
Barkholtz, Heather M., and Liu, Di -Jia. Mon .
"Advancements in rationally designed PGM-free fuel cell catalysts derived from metal–organic frameworks". United States. https://doi.org/10.1039/c6mh00344c. https://www.osti.gov/servlets/purl/1373936.
@article{osti_1373936,
title = {Advancements in rationally designed PGM-free fuel cell catalysts derived from metal–organic frameworks},
author = {Barkholtz, Heather M. and Liu, Di -Jia},
abstractNote = {Over the past several years, metal-organic framework (MOF)-derived platinum group metal free (PGM-free) electrocatalysts have gained considerable attention due to their high efficiency and low cost as potential replacement for platinum in catalyzing oxygen reduction reaction (ORR). In this review, we summarize the recent advancements in design, synthesis and characterization of MOF-derived ORR catalysts and their performances in acidic and alkaline media. As a result, we also discuss the key challenges such as durability and activity enhancement critical in moving forward this emerging electrocatalyst science.},
doi = {10.1039/c6mh00344c},
journal = {Materials Horizons},
number = 1,
volume = 4,
place = {United States},
year = {Mon Nov 14 00:00:00 EST 2016},
month = {Mon Nov 14 00:00:00 EST 2016}
}
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