Growth and Post-Deposition Treatments of SrTiO3 Films for Dye-Sensitized Photoelectrosynthesis Cell Applications
Abstract
Sensitized SrTiO3 films were observed as potential photoanodes for dye-sensitized photoelectrosynthesis cells (DSPECs). The SrTiO3 films were grown via pulsed laser deposition (PLD) on a transparent conducting oxide (fluorine-doped tin oxide, FTO) substrate, annealed, and then loaded with zinc(II) 5,10,15-tris(mesityl)-20-[(dihydroxyphosphoryl)phenyl] porphyrin (MPZnP). When paired with a platinum wire counter electrode and an Ag/AgCl reference electrode these sensitized films exhibited photocurrent densities on the order of 350 nA/cm2 under 0 V applied bias conditions versus a normal hydrogen electrode (NHE) and 75 mW/cm2 illumination at a wavelength of 445 nm. The conditions of the post-deposition annealing step—namely, a high-temperature reducing atmosphere—proved to be the most vital growth parameters for increasing photocurrent in these electrodes.
- Authors:
-
- Univ. of North Carolina, Chapel Hill, NC (United States)
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Center for Solar Fuels (UNC EFRC)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1371423
- Grant/Contract Number:
- SC0001011
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ACS Applied Materials and Interfaces
- Additional Journal Information:
- Journal Volume: 8; Journal Issue: 19; Related Information: UNC partners with University of North Carolina (lead); Duke University; University of Florida; Georgia Institute of Technology; University; North Carolina Central University; Research Triangle Institute; Journal ID: ISSN 1944-8244
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; SrTiO3; pulsed laser deposition; post-deposition annealing; dye-sensitized photoelectrosynthesis cell; transient absorption
Citation Formats
Call, Robert W., Alibabaei, Leila, Dillon, Robert J., Knauf, Robin R., Nayak, Animesh, Dempsey, Jillian L., Papanikolas, John M., and Lopez, Rene. Growth and Post-Deposition Treatments of SrTiO3 Films for Dye-Sensitized Photoelectrosynthesis Cell Applications. United States: N. p., 2016.
Web. doi:10.1021/acsami.6b01289.
Call, Robert W., Alibabaei, Leila, Dillon, Robert J., Knauf, Robin R., Nayak, Animesh, Dempsey, Jillian L., Papanikolas, John M., & Lopez, Rene. Growth and Post-Deposition Treatments of SrTiO3 Films for Dye-Sensitized Photoelectrosynthesis Cell Applications. United States. https://doi.org/10.1021/acsami.6b01289
Call, Robert W., Alibabaei, Leila, Dillon, Robert J., Knauf, Robin R., Nayak, Animesh, Dempsey, Jillian L., Papanikolas, John M., and Lopez, Rene. Fri .
"Growth and Post-Deposition Treatments of SrTiO3 Films for Dye-Sensitized Photoelectrosynthesis Cell Applications". United States. https://doi.org/10.1021/acsami.6b01289. https://www.osti.gov/servlets/purl/1371423.
@article{osti_1371423,
title = {Growth and Post-Deposition Treatments of SrTiO3 Films for Dye-Sensitized Photoelectrosynthesis Cell Applications},
author = {Call, Robert W. and Alibabaei, Leila and Dillon, Robert J. and Knauf, Robin R. and Nayak, Animesh and Dempsey, Jillian L. and Papanikolas, John M. and Lopez, Rene},
abstractNote = {Sensitized SrTiO3 films were observed as potential photoanodes for dye-sensitized photoelectrosynthesis cells (DSPECs). The SrTiO3 films were grown via pulsed laser deposition (PLD) on a transparent conducting oxide (fluorine-doped tin oxide, FTO) substrate, annealed, and then loaded with zinc(II) 5,10,15-tris(mesityl)-20-[(dihydroxyphosphoryl)phenyl] porphyrin (MPZnP). When paired with a platinum wire counter electrode and an Ag/AgCl reference electrode these sensitized films exhibited photocurrent densities on the order of 350 nA/cm2 under 0 V applied bias conditions versus a normal hydrogen electrode (NHE) and 75 mW/cm2 illumination at a wavelength of 445 nm. The conditions of the post-deposition annealing step—namely, a high-temperature reducing atmosphere—proved to be the most vital growth parameters for increasing photocurrent in these electrodes.},
doi = {10.1021/acsami.6b01289},
journal = {ACS Applied Materials and Interfaces},
number = 19,
volume = 8,
place = {United States},
year = {Fri Apr 29 00:00:00 EDT 2016},
month = {Fri Apr 29 00:00:00 EDT 2016}
}
Web of Science
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