High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]
Abstract
High-harmonic generation (HHG) in bulk solids permits the exploration of materials in a new regime of strong fields and attosecond timescales. The generation process has been discussed in the context of strongly driven electron dynamics in single-particle bands. Two-dimensional materials exhibit distinctive electronic properties compared to the bulk that could significantly modify the HHG process, including different symmetries, access to individual valleys and enhanced many-body interactions. Here we demonstrate non-perturbative HHG from a monolayer MoS2 crystal, with even and odd harmonics extending to the 13th order. The even orders are predominantly polarized perpendicular to the pump and are compatible with the anomalous transverse intraband current arising from the material’s Berry curvature, while the weak parallel component suggests the importance of interband transitions. The odd harmonics exhibit a significant enhancement in efficiency per layer compared to the bulk, which is attributed to correlation effects. In conclusion, the combination of strong many-body Coulomb interactions and widely tunable electronic properties in two-dimensional materials offers a new platform for attosecond physics.
- Authors:
-
- SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States)
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1353193
- Grant/Contract Number:
- AC02-76SF00515
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Physics
- Additional Journal Information:
- Journal Volume: 13; Journal Issue: 3; Journal ID: ISSN 1745-2473
- Publisher:
- Nature Publishing Group (NPG)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Liu, Hanzhe, Li, Yilei, You, Yong Sing, Ghimire, Shambhu, Heinz, Tony F., and Reis, David A. High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]. United States: N. p., 2016.
Web. doi:10.1038/NPHYS3946.
Liu, Hanzhe, Li, Yilei, You, Yong Sing, Ghimire, Shambhu, Heinz, Tony F., & Reis, David A. High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]. United States. https://doi.org/10.1038/NPHYS3946
Liu, Hanzhe, Li, Yilei, You, Yong Sing, Ghimire, Shambhu, Heinz, Tony F., and Reis, David A. Mon .
"High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]". United States. https://doi.org/10.1038/NPHYS3946. https://www.osti.gov/servlets/purl/1353193.
@article{osti_1353193,
title = {High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]},
author = {Liu, Hanzhe and Li, Yilei and You, Yong Sing and Ghimire, Shambhu and Heinz, Tony F. and Reis, David A.},
abstractNote = {High-harmonic generation (HHG) in bulk solids permits the exploration of materials in a new regime of strong fields and attosecond timescales. The generation process has been discussed in the context of strongly driven electron dynamics in single-particle bands. Two-dimensional materials exhibit distinctive electronic properties compared to the bulk that could significantly modify the HHG process, including different symmetries, access to individual valleys and enhanced many-body interactions. Here we demonstrate non-perturbative HHG from a monolayer MoS2 crystal, with even and odd harmonics extending to the 13th order. The even orders are predominantly polarized perpendicular to the pump and are compatible with the anomalous transverse intraband current arising from the material’s Berry curvature, while the weak parallel component suggests the importance of interband transitions. The odd harmonics exhibit a significant enhancement in efficiency per layer compared to the bulk, which is attributed to correlation effects. In conclusion, the combination of strong many-body Coulomb interactions and widely tunable electronic properties in two-dimensional materials offers a new platform for attosecond physics.},
doi = {10.1038/NPHYS3946},
journal = {Nature Physics},
number = 3,
volume = 13,
place = {United States},
year = {Mon Nov 14 00:00:00 EST 2016},
month = {Mon Nov 14 00:00:00 EST 2016}
}
Web of Science
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Ultrafast modification of Hubbard $U$ in a strongly correlated material: ab initio high-harmonic generation in NiO
text, January 2017
- Tancogne-Dejean, Nicolas; Sentef, Michael A.; Rubio, Angel
- arXiv
High-Harmonic Generation in Mott Insulators
text, January 2017
- Murakami, Yuta; Eckstein, Martin; Werner, Philipp
- arXiv
Strain-controlled high harmonic generation with Dirac fermions in silicene
text, January 2018
- Qin, Rui; Chen, Zi-Yu
- arXiv
Circularly polarized extreme ultraviolet high harmonic generation in graphene
text, January 2018
- Chen, Zi-Yu; Qin, Rui
- arXiv
Optical harmonic generation in monolayer group-VI transition metal dichalcogenides
text, January 2018
- Autere, Anton; Jussila, Henri; Marini, Andrea
- arXiv
Coherent electron trajectory control in graphene
text, January 2018
- Heide, Christian; Higuchi, Takuya; Weber, Heiko B.
- arXiv
Interband resonant high-harmonic generation by valley polarized electron-hole pairs
text, January 2019
- Yoshikawa, Naotaka; Nagai, Kohei; Uchida, Kento
- arXiv
All-optical measurement of high-order fractional molecular echoes by high-order harmonic generation
text, January 2019
- Wang, Baoning; He, Lixin; He, Yanqing
- arXiv