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Title: High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]

Abstract

High-harmonic generation (HHG) in bulk solids permits the exploration of materials in a new regime of strong fields and attosecond timescales. The generation process has been discussed in the context of strongly driven electron dynamics in single-particle bands. Two-dimensional materials exhibit distinctive electronic properties compared to the bulk that could significantly modify the HHG process, including different symmetries, access to individual valleys and enhanced many-body interactions. Here we demonstrate non-perturbative HHG from a monolayer MoS2 crystal, with even and odd harmonics extending to the 13th order. The even orders are predominantly polarized perpendicular to the pump and are compatible with the anomalous transverse intraband current arising from the material’s Berry curvature, while the weak parallel component suggests the importance of interband transitions. The odd harmonics exhibit a significant enhancement in efficiency per layer compared to the bulk, which is attributed to correlation effects. In conclusion, the combination of strong many-body Coulomb interactions and widely tunable electronic properties in two-dimensional materials offers a new platform for attosecond physics.

Authors:
 [1];  [1];  [2];  [2];  [1];  [1]
  1. SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States)
  2. SLAC National Accelerator Lab., Menlo Park, CA (United States)
Publication Date:
Research Org.:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1353193
Grant/Contract Number:  
AC02-76SF00515
Resource Type:
Accepted Manuscript
Journal Name:
Nature Physics
Additional Journal Information:
Journal Volume: 13; Journal Issue: 3; Journal ID: ISSN 1745-2473
Publisher:
Nature Publishing Group (NPG)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE

Citation Formats

Liu, Hanzhe, Li, Yilei, You, Yong Sing, Ghimire, Shambhu, Heinz, Tony F., and Reis, David A. High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]. United States: N. p., 2016. Web. doi:10.1038/NPHYS3946.
Liu, Hanzhe, Li, Yilei, You, Yong Sing, Ghimire, Shambhu, Heinz, Tony F., & Reis, David A. High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]. United States. https://doi.org/10.1038/NPHYS3946
Liu, Hanzhe, Li, Yilei, You, Yong Sing, Ghimire, Shambhu, Heinz, Tony F., and Reis, David A. Mon . "High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]". United States. https://doi.org/10.1038/NPHYS3946. https://www.osti.gov/servlets/purl/1353193.
@article{osti_1353193,
title = {High-harmonic generation from an atomically thin semiconductor [Observation of high harmonics from an atomically thin semiconductor]},
author = {Liu, Hanzhe and Li, Yilei and You, Yong Sing and Ghimire, Shambhu and Heinz, Tony F. and Reis, David A.},
abstractNote = {High-harmonic generation (HHG) in bulk solids permits the exploration of materials in a new regime of strong fields and attosecond timescales. The generation process has been discussed in the context of strongly driven electron dynamics in single-particle bands. Two-dimensional materials exhibit distinctive electronic properties compared to the bulk that could significantly modify the HHG process, including different symmetries, access to individual valleys and enhanced many-body interactions. Here we demonstrate non-perturbative HHG from a monolayer MoS2 crystal, with even and odd harmonics extending to the 13th order. The even orders are predominantly polarized perpendicular to the pump and are compatible with the anomalous transverse intraband current arising from the material’s Berry curvature, while the weak parallel component suggests the importance of interband transitions. The odd harmonics exhibit a significant enhancement in efficiency per layer compared to the bulk, which is attributed to correlation effects. In conclusion, the combination of strong many-body Coulomb interactions and widely tunable electronic properties in two-dimensional materials offers a new platform for attosecond physics.},
doi = {10.1038/NPHYS3946},
journal = {Nature Physics},
number = 3,
volume = 13,
place = {United States},
year = {Mon Nov 14 00:00:00 EST 2016},
month = {Mon Nov 14 00:00:00 EST 2016}
}

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