Amorphization due to electronic energy deposition in defective strontium titanate

Xue, Haizhou; Zarkadoula, Eva; Liu, Peng; Jin, Ke; Zhang, Yanwen; Weber, William J.

doi:10.1016/j.actamat.2017.01.051

Title: Amorphization due to electronic energy deposition in defective strontium titanate

Abstract

The synergistic interaction of electronic energy loss by ions with ion-induced defects created by elastic nuclear scattering processes has been investigated for single crystal SrTiO₃. An initial pre-damaged defect state corresponding to a relative disorder level of 0.10–0.15 sensitizes the SrTiO₃ to amorphous track formation along the ion path of 12 and 20 MeV Ti, 21 MeV Cl and 21 MeV Ni ions, where Ti, Cl and Ni ions otherwise do not produce amorphous or damage tracks in pristine SrTiO₃. The electronic stopping power threshold for amorphous ion track formation is found to be 6.7 keV/nm for the pre-damaged defect state studied in this work. Lastly, these results suggest the possibility of selectively producing nanometer scale, amorphous ion tracks in thin films of epitaxial SrTiO₃.

Authors:

Xue, Haizhou ^[1];

^[2]; Liu, Peng ^[3]; Jin, Ke ^[2]; Zhang, Yanwen ^[2];

^[4]

Univ. of Tennessee, Knoxville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States); Shandong Univ., Jinan (China)
Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Publication Date:: Fri Jan 27 00:00:00 EST 2017

Research Org.:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1342693

Alternate Identifier(s):: OSTI ID: 1418379

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Acta Materialia

Additional Journal Information:: Journal Volume: 127; Journal Issue: C; Journal ID: ISSN 1359-6454

Publisher:: Elsevier

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; strontium titanante; ion tracks; electronic stopping; SrTiO3; energy dissipation; stopping power; amorphization

Citation Formats


                    Xue, Haizhou, Zarkadoula, Eva, Liu, Peng, Jin, Ke, Zhang, Yanwen, and Weber, William J. Amorphization due to electronic energy deposition in defective strontium titanate.  United States: N. p., 2017. 
Web.  doi:10.1016/j.actamat.2017.01.051.

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                    Xue, Haizhou, Zarkadoula, Eva, Liu, Peng, Jin, Ke, Zhang, Yanwen, & Weber, William J. Amorphization due to electronic energy deposition in defective strontium titanate.  United States.  https://doi.org/10.1016/j.actamat.2017.01.051

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                    Xue, Haizhou, Zarkadoula, Eva, Liu, Peng, Jin, Ke, Zhang, Yanwen, and Weber, William J. Fri .  
"Amorphization due to electronic energy deposition in defective strontium titanate".  United States.  https://doi.org/10.1016/j.actamat.2017.01.051.  https://www.osti.gov/servlets/purl/1342693.

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@article{osti_1342693,

  title        = {Amorphization due to electronic energy deposition in defective strontium titanate},

  author       = {Xue, Haizhou and Zarkadoula, Eva and Liu, Peng and Jin, Ke and Zhang, Yanwen and Weber, William J.},

  abstractNote = {The synergistic interaction of electronic energy loss by ions with ion-induced defects created by elastic nuclear scattering processes has been investigated for single crystal SrTiO3. An initial pre-damaged defect state corresponding to a relative disorder level of 0.10–0.15 sensitizes the SrTiO3 to amorphous track formation along the ion path of 12 and 20 MeV Ti, 21 MeV Cl and 21 MeV Ni ions, where Ti, Cl and Ni ions otherwise do not produce amorphous or damage tracks in pristine SrTiO3. The electronic stopping power threshold for amorphous ion track formation is found to be 6.7 keV/nm for the pre-damaged defect state studied in this work. Lastly, these results suggest the possibility of selectively producing nanometer scale, amorphous ion tracks in thin films of epitaxial SrTiO3.},

  doi          = {10.1016/j.actamat.2017.01.051},

  journal      = {Acta Materialia},

  number       = C,

  volume       = 127,

  place        = {United States},

  year         = {Fri Jan 27 00:00:00 EST 2017},

  month        = {Fri Jan 27 00:00:00 EST 2017}

}

Copy to clipboard

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Works referencing / citing this record:

Synergistic effects of nuclear and electronic energy deposition on damage production in KTaO ₃
journal, July 2018

Jin, Ke; Zhang, Yanwen; Weber, William J.
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Amorphization kinetics in strontium titanate at 16 and 300 K under argon ion irradiation
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Two-stage synergy of electronic energy loss with defects in LiTaO 3 under ion irradiation
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Sellami, Neila; Crespillo, Miguel L.; Zhang, Yanwen
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Latent tracks and novel infrared waveguide formation in lithium tantalate irradiated with swift heavy ions
journal, February 2019

Liu, Yong; Crespillo, Miguel L.; Huang, Qing
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DOI: 10.1088/1361-6463/ab0534

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Title: Amorphization due to electronic energy deposition in defective strontium titanate

Abstract

Citation Formats

The role of electronic energy loss in ion beam modification of materials journal, February 2015

Additive effects of electronic and nuclear energy losses in irradiation-induced amorphization of zircon journal, December 2015

Competing effects of electronic and nuclear energy loss on microstructural evolution in ionic-covalent materials journal, May 2014

Combined effects of nuclear and electronic energy losses in solids irradiated with a dual-ion beam journal, April 2013

Synergy of elastic and inelastic energy loss on ion track formation in SrTiO3 journal, January 2015

Synergy of inelastic and elastic energy loss: Temperature effects and electronic stopping power dependence journal, January 2016

Energy threshold for the creation of nanodots on SrTiO 3 by swift heavy ions journal, April 2010

In situ radiation damage studies of LaxSr1−3x∕2TiO3 perovskites journal, April 2008

Materials Science of High-Level Nuclear Waste Immobilization journal, January 2009

Switching the electrical resistance of individual dislocations in single-crystalline SrTiO3 journal, March 2006

Oxide Interfaces--An Opportunity for Electronics journal, March 2010

Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching journal, July 2005

Theory of spin-orbit coupling at LaAlO 3 /SrTiO 3 interfaces and SrTiO 3 surfaces journal, April 2013

High Mobility in LaAlO3/SrTiO3 Heterostructures: Origin, Dimensionality, and Perspectives journal, May 2007

Interface-induced superconductivity and strain-dependent spin density waves in FeSe/SrTiO3 thin films journal, May 2013

Metallic and Insulating Interfaces of Amorphous SrTiO 3 -Based Oxide Heterostructures journal, September 2011

New ion beam materials laboratory for materials modification and irradiation effects research journal, November 2014

The radial distribution of dose around the path of a heavy ion in liquid water journal, January 1986

Experimental determination of track cross-section in Gd3Ga5O12 and comparison to the inelastic thermal spike model applied to several materials journal, August 2005

Triple sign reversal of the Hall effect in HgBa 2 CaCu 2 O 6 thin films after heavy-ion irradiation journal, January 2000

Response of strontium titanate to ion and electron irradiation journal, May 2009

Non-linear damage accumulation in Au-irradiated SrTiO3 journal, September 2006

Ion-induced damage accumulation and electron-beam-enhanced recrystallization in Sr Ti O 3 journal, September 2005

Ion implantation in semiconductors—Part II: Damage production and annealing journal, January 1972

Models and mechanisms of irradiation-induced amorphization in ceramics journal, May 2000

Towards new applications of ion tracks journal, August 2004

Wet and vapor etching of tracks produced in SiO2 by Ti ion irradiation journal, April 2007

Effect of nanosized surfactant molecules on the etching of ion tracks: New degrees of freedom in design of pore shape journal, August 2003

The effect of annealing environments on the epitaxial recrystallization of ion-beam-amorphized SrTiO 3 journal, March 1992

Synergistic effects of nuclear and electronic energy deposition on damage production in KTaO 3 journal, July 2018

Amorphization kinetics in strontium titanate at 16 and 300 K under argon ion irradiation journal, January 2019

Swift heavy ion tracks in alkali tantalate crystals: a combined experimental and computational study journal, December 2019

Two-stage synergy of electronic energy loss with defects in LiTaO 3 under ion irradiation journal, March 2018

Latent tracks and novel infrared waveguide formation in lithium tantalate irradiated with swift heavy ions journal, February 2019

The role of electronic energy loss in ion beam modification of materials
journal, February 2015

Additive effects of electronic and nuclear energy losses in irradiation-induced amorphization of zircon
journal, December 2015

Competing effects of electronic and nuclear energy loss on microstructural evolution in ionic-covalent materials
journal, May 2014

Combined effects of nuclear and electronic energy losses in solids irradiated with a dual-ion beam
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Synergy of elastic and inelastic energy loss on ion track formation in SrTiO3
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Synergy of inelastic and elastic energy loss: Temperature effects and electronic stopping power dependence
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Energy threshold for the creation of nanodots on SrTiO ₃ by swift heavy ions
journal, April 2010

In situ radiation damage studies of LaxSr1−3x∕2TiO3 perovskites
journal, April 2008

Materials Science of High-Level Nuclear Waste Immobilization
journal, January 2009

Switching the electrical resistance of individual dislocations in single-crystalline SrTiO3
journal, March 2006

Oxide Interfaces--An Opportunity for Electronics
journal, March 2010

Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching
journal, July 2005

Theory of spin-orbit coupling at LaAlO $_{3}$ /SrTiO $_{3}$ interfaces and SrTiO $_{3}$ surfaces
journal, April 2013

High Mobility in ${LaAlO}_{3} / {SrTiO}_{3}$ Heterostructures: Origin, Dimensionality, and Perspectives
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Interface-induced superconductivity and strain-dependent spin density waves in FeSe/SrTiO3 thin films
journal, May 2013

Metallic and Insulating Interfaces of Amorphous SrTiO ₃ -Based Oxide Heterostructures
journal, September 2011

New ion beam materials laboratory for materials modification and irradiation effects research
journal, November 2014

The radial distribution of dose around the path of a heavy ion in liquid water
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Experimental determination of track cross-section in Gd3Ga5O12 and comparison to the inelastic thermal spike model applied to several materials
journal, August 2005

Triple sign reversal of the Hall effect in ${HgBa}_{2} {CaCu}_{2} O_{6}$ thin films after heavy-ion irradiation
journal, January 2000

Response of strontium titanate to ion and electron irradiation
journal, May 2009

Non-linear damage accumulation in Au-irradiated SrTiO3
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Ion-induced damage accumulation and electron-beam-enhanced recrystallization in $Sr Ti O_{3}$
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Ion implantation in semiconductors—Part II: Damage production and annealing
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Models and mechanisms of irradiation-induced amorphization in ceramics
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Towards new applications of ion tracks
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Wet and vapor etching of tracks produced in SiO2 by Ti ion irradiation
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Effect of nanosized surfactant molecules on the etching of ion tracks: New degrees of freedom in design of pore shape
journal, August 2003

The effect of annealing environments on the epitaxial recrystallization of ion-beam-amorphized SrTiO ₃
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Synergistic effects of nuclear and electronic energy deposition on damage production in KTaO ₃
journal, July 2018

Amorphization kinetics in strontium titanate at 16 and 300 K under argon ion irradiation
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Swift heavy ion tracks in alkali tantalate crystals: a combined experimental and computational study
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Two-stage synergy of electronic energy loss with defects in LiTaO 3 under ion irradiation
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