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Title: Non-monotonic resonance in a spatially forced Lengyel-Epstein model

Abstract

Here, we study resonant spatially periodic solutions of the Lengyel-Epstein model modified to describe the chlorine dioxide-iodine-malonic acid reaction under spatially periodic illumination. Using multiple-scale analysis and numerical simulations, we obtain the stability ranges of 2:1 resonant solutions, i.e., solutions with wavenumbers that are exactly half of the forcing wavenumber. We show that the width of resonant wavenumber response is a non-monotonic function of the forcing strength, and diminishes to zero at sufficiently strong forcing. Furthermore, we show that strong forcing may result in a π/2 phase shift of the resonant solutions, and argue that the nonequilibrium Ising-Bloch front bifurcation can be reversed. Finally, we attribute these behaviors to an inherent property of forcing by periodic illumination, namely, the increase of the mean spatial illumination as the forcing amplitude is increased.

Authors:
 [1];  [2];  [3]
  1. Ben-Gurion Univ. of Negev, Beer-Sheva (Israel). Physics Dept.; Soroka Univ. Medical Center, Beer-Sheva (Israel)
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Center for Nonlinear Studies
  3. Ben-Gurion Univ. of Negev, Beer-Sheva (Israel). Physics Dept.; Ben-Gurion Univ. of Negev, Midreshet Ben-Gurion (Israel)
Publication Date:
Research Org.:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1329575
Report Number(s):
LA-UR-15-21321
Journal ID: ISSN 1054-1500; CHAOEH
Grant/Contract Number:  
AC52-06NA25396; 2008241
Resource Type:
Accepted Manuscript
Journal Name:
Chaos: An Interdisciplinary Journal of Nonlinear Science
Additional Journal Information:
Journal Volume: 25; Journal Issue: 6; Journal ID: ISSN 1054-1500
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Mathematics

Citation Formats

Haim, Lev, Hagberg, Aric, and Meron, Ehud. Non-monotonic resonance in a spatially forced Lengyel-Epstein model. United States: N. p., 2015. Web. doi:10.1063/1.4921768.
Haim, Lev, Hagberg, Aric, & Meron, Ehud. Non-monotonic resonance in a spatially forced Lengyel-Epstein model. United States. https://doi.org/10.1063/1.4921768
Haim, Lev, Hagberg, Aric, and Meron, Ehud. Tue . "Non-monotonic resonance in a spatially forced Lengyel-Epstein model". United States. https://doi.org/10.1063/1.4921768. https://www.osti.gov/servlets/purl/1329575.
@article{osti_1329575,
title = {Non-monotonic resonance in a spatially forced Lengyel-Epstein model},
author = {Haim, Lev and Hagberg, Aric and Meron, Ehud},
abstractNote = {Here, we study resonant spatially periodic solutions of the Lengyel-Epstein model modified to describe the chlorine dioxide-iodine-malonic acid reaction under spatially periodic illumination. Using multiple-scale analysis and numerical simulations, we obtain the stability ranges of 2:1 resonant solutions, i.e., solutions with wavenumbers that are exactly half of the forcing wavenumber. We show that the width of resonant wavenumber response is a non-monotonic function of the forcing strength, and diminishes to zero at sufficiently strong forcing. Furthermore, we show that strong forcing may result in a π/2 phase shift of the resonant solutions, and argue that the nonequilibrium Ising-Bloch front bifurcation can be reversed. Finally, we attribute these behaviors to an inherent property of forcing by periodic illumination, namely, the increase of the mean spatial illumination as the forcing amplitude is increased.},
doi = {10.1063/1.4921768},
journal = {Chaos: An Interdisciplinary Journal of Nonlinear Science},
number = 6,
volume = 25,
place = {United States},
year = {Tue Jun 02 00:00:00 EDT 2015},
month = {Tue Jun 02 00:00:00 EDT 2015}
}

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Works referenced in this record:

Stripe-hexagon competition in forced pattern-forming systems with broken up-down symmetry
journal, April 2005


Pattern Forming System in the Presence of Different Symmetry-Breaking Mechanisms
journal, November 2008


Rayleigh–Bénard convection in the presence of spatial temperature modulations
journal, February 2011


Locking of Turing patterns in the chlorine dioxide–iodine–malonic acid reaction with one-dimensional spatial periodic forcing
journal, January 2011

  • Dolnik, Milos; Bánsági, Tamás; Ansari, Sama
  • Physical Chemistry Chemical Physics, Vol. 13, Issue 27
  • DOI: 10.1039/c1cp20949c

Wave-number locking in spatially forced pattern-forming systems
journal, June 2008


Spatial Periodic Forcing Can Displace Patterns It Is Intended to Control
journal, July 2012


Wavenumber locking and pattern formation in spatially forced systems
journal, June 2009


Instabilities of natural convection in a periodically heated layer
journal, September 2013


Competing resonances in spatially forced pattern-forming systems
journal, September 2013


Resonance patterns in spatially forced Rayleigh–Bénard convection
journal, September 2014

  • Weiss, S.; Seiden, G.; Bodenschatz, E.
  • Journal of Fluid Mechanics, Vol. 756
  • DOI: 10.1017/jfm.2014.456

Spatial forcing of pattern-forming systems that lack inversion symmetry
journal, August 2014


Spatial localization in heterogeneous systems
journal, January 2014


Reversing desertification as a spatial resonance problem
journal, January 2015


Frequency Locking in Spatially Extended Systems
journal, February 2001


Development of Standing-Wave Labyrinthine Patterns
journal, January 2002

  • Yochelis, Arik; Hagberg, Aric; Meron, Ehud
  • SIAM Journal on Applied Dynamical Systems, Vol. 1, Issue 2
  • DOI: 10.1137/S1111111101397111

Two-phase resonant patterns in forced oscillatory systems: boundaries, mechanisms and forms
journal, December 2004

  • Yochelis, Arik; Elphick, Christian; Hagberg, Aric
  • Physica D: Nonlinear Phenomena, Vol. 199, Issue 1-2
  • DOI: 10.1016/j.physd.2004.08.015

Bloch-Front Turbulence in a Periodically Forced Belousov-Zhabotinsky Reaction
journal, September 2004


Classification of Spatially Localized Oscillations in Periodically Forced Dissipative Systems
journal, January 2008

  • Burke, J.; Yochelis, A.; Knobloch, E.
  • SIAM Journal on Applied Dynamical Systems, Vol. 7, Issue 3
  • DOI: 10.1137/070698191

Control of waves, patterns and turbulence in chemical systems
journal, March 2006


Breaking chirality in nonequilibrium systems
journal, September 1990


On the origin of traveling pulses in bistable systems
journal, June 1997


Complexes of stationary domain walls in the resonantly forced Ginsburg-Landau equation
journal, February 2005


Symmetry breaking in nonequilibrium systems: Interaction of defects
journal, December 1992


Fronts and patterns in a spatially forced CDIMA reaction
journal, January 2014

  • Haim, Lev; Hagberg, Aric; Nagao, Raphael
  • Phys. Chem. Chem. Phys., Vol. 16, Issue 47
  • DOI: 10.1039/C4CP04261A

Control of the Chlorine Dioxide−Iodine−Malonic Acid Oscillating Reaction by Illumination
journal, September 1999

  • Muñuzuri, Alberto P.; Dolnik, Milos; Zhabotinsky, Anatol M.
  • Journal of the American Chemical Society, Vol. 121, Issue 35
  • DOI: 10.1021/ja9910457

Experimental and modeling study of oscillations in the chlorine dioxide-iodine-malonic acid reaction
journal, December 1990

  • Lengyel, Istvan; Rabai, Gyula; Epstein, Irving R.
  • Journal of the American Chemical Society, Vol. 112, Issue 25
  • DOI: 10.1021/ja00181a011

The Dynamics of Curved Fronts: Beyond Geometry
journal, February 1997


Pattern formation outside of equilibrium
journal, July 1993


Nonlinear Physics of Ecosystems
journal, April 2015


Works referencing / citing this record:

From one pattern into another: analysis of Turing patterns in heterogeneous domains via WKBJ
journal, January 2020

  • Krause, Andrew L.; Klika, Václav; Woolley, Thomas E.
  • Journal of The Royal Society Interface, Vol. 17, Issue 162
  • DOI: 10.1098/rsif.2019.0621

From One Pattern into Another: Analysis of Turing Patterns in Heterogeneous Domains via WKBJ
preprint, January 2019


Turing Patterning in Stratified Domains
preprint, January 2020