Highly compressible 3D periodic graphene aerogel microlattices
Abstract
Graphene is a two-dimensional material that offers a unique combination of low density, exceptional mechanical properties, large surface area and excellent electrical conductivity. Recent progress has produced bulk 3D assemblies of graphene, such as graphene aerogels, but they possess purely stochastic porous networks, which limit their performance compared with the potential of an engineered architecture. Here we report the fabrication of periodic graphene aerogel microlattices, possessing an engineered architecture via a 3D printing technique known as direct ink writing. The 3D printed graphene aerogels are lightweight, highly conductive and exhibit supercompressibility (up to 90% compressive strain). Moreover, the Young’s moduli of the 3D printed graphene aerogels show an order of magnitude improvement over bulk graphene materials with comparable geometric density and possess large surface areas. Ultimately, adapting the 3D printing technique to graphene aerogels realizes the possibility of fabricating a myriad of complex aerogel architectures for a broad range of applications.
- Publication Date:
- Research Org.:
- Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
- Sponsoring Org.:
- USDOE Laboratory Directed Research and Development (LDRD) Program
- OSTI Identifier:
- 1259507
- Alternate Identifier(s):
- OSTI ID: 1410001
- Report Number(s):
- LLNL-JRNL-665510
Journal ID: ISSN 2041-1723; ncomms7962
- Grant/Contract Number:
- AC52-07NA27344; 14-SI-004; 13-LW-099
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 6; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 77 NANOSCIENCE AND NANOTECHNOLOGY
Citation Formats
Zhu, Cheng, Han, T. Yong-Jin, Duoss, Eric B., Golobic, Alexandra M., Kuntz, Joshua D., Spadaccini, Christopher M., and Worsley, Marcus A. Highly compressible 3D periodic graphene aerogel microlattices. United States: N. p., 2015.
Web. doi:10.1038/ncomms7962.
Zhu, Cheng, Han, T. Yong-Jin, Duoss, Eric B., Golobic, Alexandra M., Kuntz, Joshua D., Spadaccini, Christopher M., & Worsley, Marcus A. Highly compressible 3D periodic graphene aerogel microlattices. United States. https://doi.org/10.1038/ncomms7962
Zhu, Cheng, Han, T. Yong-Jin, Duoss, Eric B., Golobic, Alexandra M., Kuntz, Joshua D., Spadaccini, Christopher M., and Worsley, Marcus A. Wed .
"Highly compressible 3D periodic graphene aerogel microlattices". United States. https://doi.org/10.1038/ncomms7962. https://www.osti.gov/servlets/purl/1259507.
@article{osti_1259507,
title = {Highly compressible 3D periodic graphene aerogel microlattices},
author = {Zhu, Cheng and Han, T. Yong-Jin and Duoss, Eric B. and Golobic, Alexandra M. and Kuntz, Joshua D. and Spadaccini, Christopher M. and Worsley, Marcus A.},
abstractNote = {Graphene is a two-dimensional material that offers a unique combination of low density, exceptional mechanical properties, large surface area and excellent electrical conductivity. Recent progress has produced bulk 3D assemblies of graphene, such as graphene aerogels, but they possess purely stochastic porous networks, which limit their performance compared with the potential of an engineered architecture. Here we report the fabrication of periodic graphene aerogel microlattices, possessing an engineered architecture via a 3D printing technique known as direct ink writing. The 3D printed graphene aerogels are lightweight, highly conductive and exhibit supercompressibility (up to 90% compressive strain). Moreover, the Young’s moduli of the 3D printed graphene aerogels show an order of magnitude improvement over bulk graphene materials with comparable geometric density and possess large surface areas. Ultimately, adapting the 3D printing technique to graphene aerogels realizes the possibility of fabricating a myriad of complex aerogel architectures for a broad range of applications.},
doi = {10.1038/ncomms7962},
journal = {Nature Communications},
number = ,
volume = 6,
place = {United States},
year = {Wed Apr 22 00:00:00 EDT 2015},
month = {Wed Apr 22 00:00:00 EDT 2015}
}
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