Controlling condensation and frost growth with chemical micropatterns
Abstract
Frost growth on chilled hydrophobic surfaces is an inter-droplet phenomenon, where frozen droplets harvest water from supercooled liquid droplets to grow ice bridges that propagate across the surface in a chain reaction. To date, no surface has been able to passively prevent the in-plane growth of frost across the population of supercooled condensate. Here, we demonstrate that when the nucleation sites for supercooled condensate are properly controlled with chemical micropatterns, the speed of frost growth can be slowed and even halted entirely. This stoppage of frost growth is attributed to the large interdroplet separation between condensate upon the onset of freezing, which was controlled by the pitch of the chemical patterns and by deliberately triggering an early freezing event. Lastly, these findings reveal that frost growth can be passively suppressed by designing surfaces to spatially control nucleation sites and/or temporally control the onset of freezing events.
- Authors:
-
- Virginia Polytechnic Inst. and State Univ. (Virginia Tech), Blacksburg, VA (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
- Univ. of Tennessee, Knoxville, TN (United States); Kansas State Univ., Manhattan, KS (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Virginia Polytechnic Inst. and State Univ. (Virginia Tech), Blacksburg, VA (United States)
- Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1240546
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Volume: 6; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; applied physics; engineering; fluid dynamics; materials science
Citation Formats
Boreyko, Jonathan B., Hansen, Ryan R., Murphy, Kevin R., Nath, Saurabh, Retterer, Scott T., and Collier, C. Patrick. Controlling condensation and frost growth with chemical micropatterns. United States: N. p., 2016.
Web. doi:10.1038/srep19131.
Boreyko, Jonathan B., Hansen, Ryan R., Murphy, Kevin R., Nath, Saurabh, Retterer, Scott T., & Collier, C. Patrick. Controlling condensation and frost growth with chemical micropatterns. United States. https://doi.org/10.1038/srep19131
Boreyko, Jonathan B., Hansen, Ryan R., Murphy, Kevin R., Nath, Saurabh, Retterer, Scott T., and Collier, C. Patrick. Fri .
"Controlling condensation and frost growth with chemical micropatterns". United States. https://doi.org/10.1038/srep19131. https://www.osti.gov/servlets/purl/1240546.
@article{osti_1240546,
title = {Controlling condensation and frost growth with chemical micropatterns},
author = {Boreyko, Jonathan B. and Hansen, Ryan R. and Murphy, Kevin R. and Nath, Saurabh and Retterer, Scott T. and Collier, C. Patrick},
abstractNote = {Frost growth on chilled hydrophobic surfaces is an inter-droplet phenomenon, where frozen droplets harvest water from supercooled liquid droplets to grow ice bridges that propagate across the surface in a chain reaction. To date, no surface has been able to passively prevent the in-plane growth of frost across the population of supercooled condensate. Here, we demonstrate that when the nucleation sites for supercooled condensate are properly controlled with chemical micropatterns, the speed of frost growth can be slowed and even halted entirely. This stoppage of frost growth is attributed to the large interdroplet separation between condensate upon the onset of freezing, which was controlled by the pitch of the chemical patterns and by deliberately triggering an early freezing event. Lastly, these findings reveal that frost growth can be passively suppressed by designing surfaces to spatially control nucleation sites and/or temporally control the onset of freezing events.},
doi = {10.1038/srep19131},
journal = {Scientific Reports},
number = ,
volume = 6,
place = {United States},
year = {Fri Jan 22 00:00:00 EST 2016},
month = {Fri Jan 22 00:00:00 EST 2016}
}
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