DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Space-and-time resolved spectroscopy of single GaN nanowires

Abstract

Gallium nitridenanowires have garnered much attention in recent years due to their attractive optical and electrical properties. An understanding of carrier transport, relaxation, and recombination in these quasi-one-dimensional nanosystems is therefore important in optimizing them for various applications. We present ultrafast optical microscopic measurements on single GaNnanowires. Furthermore, our experiments, performed while varying the light polarization,excitation fluence, and position, give insight into the mechanisms governing carrier dynamics in these nanosystems.

Authors:
 [1];  [2];  [3];  [3];  [3];  [4];  [4]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Indian Space Research Organization, Bangalor (India)
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); New Mexico State Univ., Las Cruces, NM (United States)
  3. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  4. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1235285
Alternate Identifier(s):
OSTI ID: 1226766; OSTI ID: 1239536
Report Number(s):
SAND-2015-5890J; LA-UR-15-24825
Journal ID: ISSN 0003-6951; 598503
Grant/Contract Number:  
AC04-94AL85000; AC52-06NA25396
Resource Type:
Accepted Manuscript
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 106; Journal Issue: 26; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; III-V semiconductors; carrier relaxation times; nanowires; polarization; ultrafast measurements; 77 NANOSCIENCE AND NANOTECHNOLOGY

Citation Formats

Upadhya, Prashanth C., Martinez, Julio A., Li, Qiming, Wang, George T., Swartzentruber, Brian S., Taylor, Antoinette J., and Prasankumar, Rohit P. Space-and-time resolved spectroscopy of single GaN nanowires. United States: N. p., 2015. Web. doi:10.1063/1.4923273.
Upadhya, Prashanth C., Martinez, Julio A., Li, Qiming, Wang, George T., Swartzentruber, Brian S., Taylor, Antoinette J., & Prasankumar, Rohit P. Space-and-time resolved spectroscopy of single GaN nanowires. United States. https://doi.org/10.1063/1.4923273
Upadhya, Prashanth C., Martinez, Julio A., Li, Qiming, Wang, George T., Swartzentruber, Brian S., Taylor, Antoinette J., and Prasankumar, Rohit P. Tue . "Space-and-time resolved spectroscopy of single GaN nanowires". United States. https://doi.org/10.1063/1.4923273. https://www.osti.gov/servlets/purl/1235285.
@article{osti_1235285,
title = {Space-and-time resolved spectroscopy of single GaN nanowires},
author = {Upadhya, Prashanth C. and Martinez, Julio A. and Li, Qiming and Wang, George T. and Swartzentruber, Brian S. and Taylor, Antoinette J. and Prasankumar, Rohit P.},
abstractNote = {Gallium nitridenanowires have garnered much attention in recent years due to their attractive optical and electrical properties. An understanding of carrier transport, relaxation, and recombination in these quasi-one-dimensional nanosystems is therefore important in optimizing them for various applications. We present ultrafast optical microscopic measurements on single GaNnanowires. Furthermore, our experiments, performed while varying the light polarization,excitation fluence, and position, give insight into the mechanisms governing carrier dynamics in these nanosystems.},
doi = {10.1063/1.4923273},
journal = {Applied Physics Letters},
number = 26,
volume = 106,
place = {United States},
year = {Tue Jun 30 00:00:00 EDT 2015},
month = {Tue Jun 30 00:00:00 EDT 2015}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 8 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Nanowire photonics
journal, October 2009


GaN based nanorods for solid state lighting
journal, April 2012

  • Li, Shunfeng; Waag, Andreas
  • Journal of Applied Physics, Vol. 111, Issue 7
  • DOI: 10.1063/1.3694674

Review of recent progress of III-nitride nanowire lasers
journal, January 2013

  • Arafin, Shamsul; Liu, Xianhe; Mi, Zetian
  • Journal of Nanophotonics, Vol. 7, Issue 1
  • DOI: 10.1117/1.JNP.7.074599

Coaxial Group III−Nitride Nanowire Photovoltaics
journal, April 2009

  • Dong, Yajie; Tian, Bozhi; Kempa, Thomas J.
  • Nano Letters, Vol. 9, Issue 5, p. 2183-2187
  • DOI: 10.1021/nl900858v

III-nitride core–shell nanowire arrayed solar cells
journal, April 2012


Gallium Nitride Nanowire Nanodevices
journal, February 2002

  • Huang, Yu; Duan, Xiangfeng; Cui, Yi
  • Nano Letters, Vol. 2, Issue 2
  • DOI: 10.1021/nl015667d

Nanoscale Effects on Heterojunction Electron Gases in GaN/AlGaN Core/Shell Nanowires
journal, August 2011

  • Wong, Bryan M.; Léonard, François; Li, Qiming
  • Nano Letters, Vol. 11, Issue 8
  • DOI: 10.1021/nl200981x

Probing Quantum Confinement within Single Core–Multishell Nanowires
journal, October 2012

  • Martínez-Criado, Gema; Homs, Alejandro; Alén, Benito
  • Nano Letters, Vol. 12, Issue 11
  • DOI: 10.1021/nl303178u

Gigahertz Coherent Guided Acoustic Phonons in AlN/GaN Nanowire Superlattices
journal, February 2013

  • Mante, Pierre-Adrien; Wu, Yueh-Chun; Lin, Yuan-Ting
  • Nano Letters, Vol. 13, Issue 3
  • DOI: 10.1021/nl3044986

Single-mode GaN nanowire lasers
journal, January 2012

  • Li, Qiming; Wright, Jeremy B.; Chow, Weng W.
  • Optics Express, Vol. 20, Issue 16
  • DOI: 10.1364/OE.20.017873

Franz−Keldysh Effect in GaN Nanowires
journal, July 2007

  • Cavallini, A.; Polenta, L.; Rossi, M.
  • Nano Letters, Vol. 7, Issue 7
  • DOI: 10.1021/nl070954o

Luminescence properties of defects in GaN
journal, March 2005

  • Reshchikov, Michael A.; Morkoç, Hadis
  • Journal of Applied Physics, Vol. 97, Issue 6
  • DOI: 10.1063/1.1868059

Depletion-Mode Photoconductivity Study of Deep Levels in GaN Nanowires
journal, October 2008


GaN nanowire surface state observed using deep level optical spectroscopy
journal, April 2010

  • Armstrong, A.; Li, Q.; Lin, Y.
  • Applied Physics Letters, Vol. 96, Issue 16
  • DOI: 10.1063/1.3404182

Deep level optical spectroscopy of GaN nanorods
journal, September 2009

  • Armstrong, A.; Li, Q.; Bogart, K. H. A.
  • Journal of Applied Physics, Vol. 106, Issue 5
  • DOI: 10.1063/1.3211317

Highly aligned, template-free growth and characterization of vertical GaN nanowires on sapphire by metal–organic chemical vapour deposition
journal, November 2006


Polarized Raman scattering from single GaN nanowires
journal, July 2006


Correlation of growth temperature, photoluminescence, and resistivity in GaN nanowires
journal, March 2008

  • Talin, A. Alec; Wang, George T.; Lai, Elaine
  • Applied Physics Letters, Vol. 92, Issue 9
  • DOI: 10.1063/1.2889941

Yellow Luminescence of Polar and Nonpolar GaN Nanowires on r -Plane Sapphire by Metal Organic Chemical Vapor Deposition
journal, July 2013

  • Xu, Shengrui; Hao, Yue; Zhang, Jincheng
  • Nano Letters, Vol. 13, Issue 8
  • DOI: 10.1021/nl4015205

Origin of Yellow-Band Emission in Epitaxially Grown GaN Nanowire Arrays
journal, August 2014

  • Liu, Baodan; Yuan, Fang; Dierre, Benjamin
  • ACS Applied Materials & Interfaces, Vol. 6, Issue 16
  • DOI: 10.1021/am5034878

Transport imaging for contact-free measurements of minority carrier diffusion in GaN, GaN/AlGaN, and GaN/InGaN core-shell nanowires
journal, March 2011

  • Baird, Lee; Ong, C. P.; Cole, R. Adam
  • Applied Physics Letters, Vol. 98, Issue 13
  • DOI: 10.1063/1.3573832

Spatial Distribution of Defect Luminescence in GaN Nanowires
journal, May 2010


Ultrafast carrier dynamics in semiconductor nanowires
journal, September 2009

  • Prasankumar, Rohit P.; Upadhya, Prashanth C.; Taylor, Antoinette J.
  • physica status solidi (b), Vol. 246, Issue 9
  • DOI: 10.1002/pssb.200945128

Ultrafast Carrier Relaxation in InN Nanowires Grown by Reactive Vapor Transport
journal, November 2008

  • Othonos, Andreas; Zervos, Matthew; Pervolaraki, Maria
  • Nanoscale Research Letters, Vol. 4, Issue 2
  • DOI: 10.1007/s11671-008-9211-8

Noncontact Measurement of Charge Carrier Lifetime and Mobility in GaN Nanowires
journal, January 2012

  • Parkinson, Patrick; Dodson, Christopher; Joyce, Hannah J.
  • Nano Letters, Vol. 12, Issue 9
  • DOI: 10.1021/nl301898m

Ultrafast carrier dynamics in GaN nanorods
journal, November 2014

  • Yang, Chi-Yuan; Chia, Chih-Ta; Chen, Hung-Ying
  • Applied Physics Letters, Vol. 105, Issue 21
  • DOI: 10.1063/1.4902927

Defect states of chemical vapor deposition grown GaN nanowires: Effects and mechanisms in the relaxation of carriers
journal, September 2009

  • Tsokkou, Demetra; Othonos, Andreas; Zervos, Matthew
  • Journal of Applied Physics, Vol. 106, Issue 5
  • DOI: 10.1063/1.3212989

The influence of radial heterostructuring on carrier dynamics in gallium nitride nanowires
journal, October 2012

  • Kar, Ayan; Li, Qiming; Upadhya, Prashanth C.
  • Applied Physics Letters, Vol. 101, Issue 14
  • DOI: 10.1063/1.4756915

The influence of defect states on non-equilibrium carrier dynamics in GaN nanowires
journal, January 2010


Ultrafast Transient Absorption Measurements of Charge Carrier Dynamics in Single II−VI Nanowires
journal, October 2009

  • Carey, Christopher R.; Yu, Yanghai; Kuno, Masaru
  • The Journal of Physical Chemistry C, Vol. 113, Issue 44
  • DOI: 10.1021/jp907147y

Carrier Thermalization Dynamics in Single Zincblende and Wurtzite InP Nanowires
journal, November 2014

  • Wang, Yuda; Jackson, Howard E.; Smith, Leigh M.
  • Nano Letters, Vol. 14, Issue 12
  • DOI: 10.1021/nl503747h

Ultrafast Spectroscopy of Quantum Confined States in a Single CdSe Nanowire
journal, March 2013

  • Schumacher, Thorsten; Giessen, Harald; Lippitz, Markus
  • Nano Letters, Vol. 13, Issue 4
  • DOI: 10.1021/nl400259f

Charge Carrier Trapping and Acoustic Phonon Modes in Single CdTe Nanowires
journal, May 2012

  • Lo, Shun Shang; Major, Todd A.; Petchsang, Nattasamon
  • ACS Nano, Vol. 6, Issue 6
  • DOI: 10.1021/nn3010526

Ultrafast optical wide field microscopy
journal, January 2013


Direct Imaging of Free Carrier and Trap Carrier Motion in Silicon Nanowires by Spatially-Separated Femtosecond Pump–Probe Microscopy
journal, February 2013

  • Gabriel, Michelle M.; Kirschbrown, Justin R.; Christesen, Joseph D.
  • Nano Letters, Vol. 13, Issue 3
  • DOI: 10.1021/nl400265b

Ultrafast Carrier Dynamics in Individual Silicon Nanowires: Characterization of Diameter-Dependent Carrier Lifetime and Surface Recombination with Pump–Probe Microscopy
journal, April 2014

  • Grumstrup, Erik M.; Gabriel, Michelle M.; Cating, Emma M.
  • The Journal of Physical Chemistry C, Vol. 118, Issue 16
  • DOI: 10.1021/jp502737e

Reversible Strain-Induced Electron–Hole Recombination in Silicon Nanowires Observed with Femtosecond Pump–Probe Microscopy
journal, October 2014

  • Grumstrup, Erik M.; Gabriel, Michelle M.; Pinion, Christopher W.
  • Nano Letters, Vol. 14, Issue 11
  • DOI: 10.1021/nl5026166

Understanding ultrafast carrier dynamics in single quasi-one-dimensional Si nanowires
journal, February 2012

  • Seo, M. A.; Dayeh, S. A.; Upadhya, P. C.
  • Applied Physics Letters, Vol. 100, Issue 7
  • DOI: 10.1063/1.3685487

Mapping Carrier Diffusion in Single Silicon Core–Shell Nanowires with Ultrafast Optical Microscopy
journal, February 2012

  • Seo, M. A.; Yoo, J.; Dayeh, S. A.
  • Nano Letters, Vol. 12, Issue 12
  • DOI: 10.1021/nl303502f

Carrier recombination dynamics in individual CdSe nanowires
journal, March 2011


Transient Rayleigh Scattering: A New Probe of Picosecond Carrier Dynamics in a Single Semiconductor Nanowire
journal, September 2012

  • Montazeri, Mohammad; Jackson, Howard E.; Smith, Leigh M.
  • Nano Letters, Vol. 12, Issue 10
  • DOI: 10.1021/nl302767u

Strain influenced indium composition distribution in GaN/InGaN core-shell nanowires
journal, November 2010

  • Li, Qiming; Wang, George T.
  • Applied Physics Letters, Vol. 97, Issue 18
  • DOI: 10.1063/1.3513345

Exciton Recombination Dynamics in CdSe Nanowires:  Bimolecular to Three-Carrier Auger Kinetics
journal, July 2006

  • Robel, István; Bunker, Bruce A.; Kamat, Prashant V.
  • Nano Letters, Vol. 6, Issue 7
  • DOI: 10.1021/nl060199z

Works referencing / citing this record:

Ultrafast measurements of the dynamics of single nanostructures: a review
journal, November 2018

  • Beane, Gary; Devkota, Tuphan; Brown, Brendan S.
  • Reports on Progress in Physics, Vol. 82, Issue 1
  • DOI: 10.1088/1361-6633/aaea4b