Complex magnetic ordering in EuAl4–A 151Eu Mössbauer study
Abstract
151Eu Mössbauer spectroscopy has been used to investigate the behaviour of EuAl4 through the four magnetic transitions that occur below 16 K. We find clear evidence for the first transition (TN1, the onset of order) where an incommensurate modulated magnetic structure appears, and the third (TN3) where the modulation disappears at the tetragonal → orthorhombic structural transition. We see no changes at the lowest transition (TN4) but find that the modulation amplitude passes through a maximum at TN2. Data on the isostructural but magnetically simpler EuGa4 are also presented for comparison.
- Authors:
-
- McGill Univ., Montreal, QC (Canada)
- Ames Lab., and Iowa State Univ., Ames, IA (United States)
- Ames Lab., and Iowa State Univ., Ames, IA (United States); Univ. of Michigan, Ann Arbor, MI (United States)
- Publication Date:
- Research Org.:
- Ames Laboratory (AMES), Ames, IA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)
- OSTI Identifier:
- 2283157
- Report Number(s):
- IS-J-11250
Journal ID: ISSN 2158-3226
- Grant/Contract Number:
- AC02-07CH11358
- Resource Type:
- Accepted Manuscript
- Journal Name:
- AIP Advances
- Additional Journal Information:
- Journal Volume: 14; Journal Issue: 1; Journal ID: ISSN 2158-3226
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; magnetic ordering; crystal structure; Mossbauer spectroscopy; isomeric shift; Fourier analysis; hyperfine structure
Citation Formats
Ryan, Dominic H., Kuthanazhi, Brinda, Jo, Na Hyan, and Canfield, Paul C. Complex magnetic ordering in EuAl4–A 151Eu Mössbauer study. United States: N. p., 2024.
Web. doi:10.1063/9.0000621.
Ryan, Dominic H., Kuthanazhi, Brinda, Jo, Na Hyan, & Canfield, Paul C. Complex magnetic ordering in EuAl4–A 151Eu Mössbauer study. United States. https://doi.org/10.1063/9.0000621
Ryan, Dominic H., Kuthanazhi, Brinda, Jo, Na Hyan, and Canfield, Paul C. Tue .
"Complex magnetic ordering in EuAl4–A 151Eu Mössbauer study". United States. https://doi.org/10.1063/9.0000621. https://www.osti.gov/servlets/purl/2283157.
@article{osti_2283157,
title = {Complex magnetic ordering in EuAl4–A 151Eu Mössbauer study},
author = {Ryan, Dominic H. and Kuthanazhi, Brinda and Jo, Na Hyan and Canfield, Paul C.},
abstractNote = {151Eu Mössbauer spectroscopy has been used to investigate the behaviour of EuAl4 through the four magnetic transitions that occur below 16 K. We find clear evidence for the first transition (TN1, the onset of order) where an incommensurate modulated magnetic structure appears, and the third (TN3) where the modulation disappears at the tetragonal → orthorhombic structural transition. We see no changes at the lowest transition (TN4) but find that the modulation amplitude passes through a maximum at TN2. Data on the isostructural but magnetically simpler EuGa4 are also presented for comparison.},
doi = {10.1063/9.0000621},
journal = {AIP Advances},
number = 1,
volume = 14,
place = {United States},
year = {Tue Jan 23 00:00:00 EST 2024},
month = {Tue Jan 23 00:00:00 EST 2024}
}
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Works referenced in this record:
Magnetic phase transitions in Eu( single crystals
journal, August 2020
- Sangeetha, N. S.; Pakhira, Santanu; Ryan, D. H.
- Physical Review Materials, Vol. 4, Issue 8
Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples
journal, December 2015
- Canfield, Paul C.; Kong, Tai; Kaluarachchi, Udhara S.
- Philosophical Magazine, Vol. 96, Issue 1
A complete solution to the Mössbauer problem, all in one place
journal, December 2006
- Voyer, C. J.; Ryan, D. H.
- Hyperfine Interactions, Vol. 170, Issue 1-3
Lattice Modulation and Structural Phase Transition in the Antiferromagnet EuAl 4
journal, January 2019
- Shimomura, Susumu; Murao, Hiroki; Tsutsui, Satoshi
- Journal of the Physical Society of Japan, Vol. 88, Issue 1
EuNiGe 3 , an anisotropic antiferromagnet
journal, May 2014
- Maurya, A.; Bonville, P.; Thamizhavel, A.
- Journal of Physics: Condensed Matter, Vol. 26, Issue 21
New materials physics
journal, November 2019
- Canfield, Paul C.
- Reports on Progress in Physics, Vol. 83, Issue 1
Antiferromagnetic Order of EuGa4Probed by Mössbauer Spectroscopy
conference, June 2014
- Homma, Yoshiya; Nakamura, Ai; Hirose, Yusuke
- Proceedings of the International Conference on Strongly Correlated Electron Systems (SCES2013)
Magnetic and Fermi Surface Properties of EuGa 4
journal, October 2013
- Nakamura, Ai; Hiranaka, Yuichi; Hedo, Masato
- Journal of the Physical Society of Japan, Vol. 82, Issue 10
Transport and Magnetic Properties of EuAl 4 and EuGa 4
journal, December 2015
- Nakamura, Ai; Uejo, Taro; Honda, Fuminori
- Journal of the Physical Society of Japan, Vol. 84, Issue 12
Incommensurate modulated magnetic structure in orthorhombic EuPdSb
journal, June 2001
- Bonville, P.; Hodges, J. A.; Shirakawa, M.
- The European Physical Journal B, Vol. 21, Issue 3
Modulated ferromagnetic ordering and the magnetocaloric response of Eu 4 PdMg
journal, May 2015
- Ryan, D. H.; Legros, Anaëlle; Niehaus, Oliver
- Journal of Applied Physics, Vol. 117, Issue 17
Magnetic Structure of Divalent Europium Compound EuGa 4 Studied by Single-Crystal Time-of-Flight Neutron Diffraction
journal, November 2016
- Kawasaki, Takuro; Kaneko, Koji; Nakamura, Ai
- Journal of the Physical Society of Japan, Vol. 85, Issue 11
Charge-Density-Wave Order and Multiple Magnetic Transitions in Divalent Europium Compound EuAl 4
journal, June 2021
- Kaneko, Koji; Kawasaki, Takuro; Nakamura, Ai
- Journal of the Physical Society of Japan, Vol. 90, Issue 6