Minimizing Interfacial Recombination in 1.8 eV Triple‐Halide Perovskites for 27.5% Efficient All‐Perovskite Tandems
Abstract
Abstract All‐perovskite tandem solar cells show great potential to enable the highest performance at reasonable costs for a viable market entry in the near future. In particular, wide‐bandgap (WBG) perovskites with higher open‐circuit voltage ( V OC ) are essential to further improve the tandem solar cells’ performance. Here, a new 1.8 eV bandgap triple‐halide perovskite composition in conjunction with a piperazinium iodide (PI) surface treatment is developed. With structural analysis, it is found that the PI modifies the surface through a reduction of excess lead iodide in the perovskite and additionally penetrates the bulk. Constant light‐induced magneto‐transport measurements are applied to separately resolve charge carrier properties of electrons and holes. These measurements reveal a reduced deep trap state density, and improved steady‐state carrier lifetime (factor 2.6) and diffusion lengths (factor 1.6). As a result, WBG PSCs achieve 1.36 V V OC , reaching 90% of the radiative limit. Combined with a 1.26 eV narrow bandgap (NBG) perovskite with a rubidium iodide additive, this enables a tandem cell with a certified scan efficiency of 27.5%.
- Authors:
-
[2];
more »
- Division Solar Energy Helmholtz‐Zentrum Berlin für Materialien und Energie GmbH 12489 Berlin Germany, National Renewable Energy Laboratory Golden Colorado 80401 USA
- Division Solar Energy Helmholtz‐Zentrum Berlin für Materialien und Energie GmbH 12489 Berlin Germany
- Institute of Physics and Astronomy University of Potsdam 14476 Potsdam‐Golm Germany
- POLYMAT University of the Basque Country UPV/EHU Av. Tolosa 72 Donostia‐San Sebastián 20018 Spain, IKERBASQUE Basque Foundation for Science Bilbao 48009 Spain, POLYKEY s.l. Av. Tolosa 72 Donostia‐San Sebastián 20018 Spain
- Institute of Applied Physics University of Tübingen 72076 Tübingen Germany
- Materials, Chemical and Computational Sciences (MCCS) National Renewable Energy Laboratory Golden CO 80401 USA
- Clarendon Laboratory Department of Advanced Materials and Interfaces for Photovoltaic Solar Cells University of Oxford Parks Road Oxford OX1 3PU UK
- Institute of Electronic Devices University of Wuppertal 42119 Wuppertal Germany, Wuppertal Center for Smart Materials &, Systems University of Wuppertal 42119 Wuppertal Germany
- Institute of Physics and Astronomy University of Potsdam 14476 Potsdam‐Golm Germany, Electronic Engineering Department The Chinese University of Hong Kong Hong Kong SAR China
- Division Solar Energy Helmholtz‐Zentrum Berlin für Materialien und Energie GmbH 12489 Berlin Germany, Faculty of Electrical Engineering and Computer Science Technische Universität Berlin Berlin Germany
- Publication Date:
- Research Org.:
- National Renewable Energy Laboratory (NREL), Golden, CO (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office; German Research Foundation (DFG); Engineering and Physical Sciences Research Council (EPSRC); Federal Ministry of Education and Research (BMBF); European Union (EU); Volkswagen Foundation
- OSTI Identifier:
- 2228988
- Alternate Identifier(s):
- OSTI ID: 2229792; OSTI ID: 2274824
- Report Number(s):
- NREL/JA-5900-88317
Journal ID: ISSN 0935-9648; 2307743
- Grant/Contract Number:
- AC3608GO28308; AC36-08GO28308; 03SF0540; 03SF0631; SPP2196; RI 1551/15-2
- Resource Type:
- Published Article
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Name: Advanced Materials Journal Volume: 36 Journal Issue: 6; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley Blackwell (John Wiley & Sons)
- Country of Publication:
- Germany
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; all-perovskite tandem solar cells; piperazinium iodide; recombination losses; triple-halide wide-bandgap perovskite
Citation Formats
Yang, Fengjiu, Tockhorn, Philipp, Musiienko, Artem, Lang, Felix, Menzel, Dorothee, Macqueen, Rowan, Köhnen, Eike, Xu, Ke, Mariotti, Silvia, Mantione, Daniele, Merten, Lena, Hinderhofer, Alexander, Li, Bor, Wargulski, Dan R., Harvey, Steven P., Zhang, Jiahuan, Scheler, Florian, Berwig, Sebastian, Roß, Marcel, Thiesbrummel, Jarla, Al‐Ashouri, Amran, Brinkmann, Kai O., Riedl, Thomas, Schreiber, Frank, Abou‐Ras, Daniel, Snaith, Henry, Neher, Dieter, Korte, Lars, Stolterfoht, Martin, and Albrecht, Steve. Minimizing Interfacial Recombination in 1.8 eV Triple‐Halide Perovskites for 27.5% Efficient All‐Perovskite Tandems. Germany: N. p., 2023.
Web. doi:10.1002/adma.202307743.
Yang, Fengjiu, Tockhorn, Philipp, Musiienko, Artem, Lang, Felix, Menzel, Dorothee, Macqueen, Rowan, Köhnen, Eike, Xu, Ke, Mariotti, Silvia, Mantione, Daniele, Merten, Lena, Hinderhofer, Alexander, Li, Bor, Wargulski, Dan R., Harvey, Steven P., Zhang, Jiahuan, Scheler, Florian, Berwig, Sebastian, Roß, Marcel, Thiesbrummel, Jarla, Al‐Ashouri, Amran, Brinkmann, Kai O., Riedl, Thomas, Schreiber, Frank, Abou‐Ras, Daniel, Snaith, Henry, Neher, Dieter, Korte, Lars, Stolterfoht, Martin, & Albrecht, Steve. Minimizing Interfacial Recombination in 1.8 eV Triple‐Halide Perovskites for 27.5% Efficient All‐Perovskite Tandems. Germany. https://doi.org/10.1002/adma.202307743
Yang, Fengjiu, Tockhorn, Philipp, Musiienko, Artem, Lang, Felix, Menzel, Dorothee, Macqueen, Rowan, Köhnen, Eike, Xu, Ke, Mariotti, Silvia, Mantione, Daniele, Merten, Lena, Hinderhofer, Alexander, Li, Bor, Wargulski, Dan R., Harvey, Steven P., Zhang, Jiahuan, Scheler, Florian, Berwig, Sebastian, Roß, Marcel, Thiesbrummel, Jarla, Al‐Ashouri, Amran, Brinkmann, Kai O., Riedl, Thomas, Schreiber, Frank, Abou‐Ras, Daniel, Snaith, Henry, Neher, Dieter, Korte, Lars, Stolterfoht, Martin, and Albrecht, Steve. Wed .
"Minimizing Interfacial Recombination in 1.8 eV Triple‐Halide Perovskites for 27.5% Efficient All‐Perovskite Tandems". Germany. https://doi.org/10.1002/adma.202307743.
@article{osti_2228988,
title = {Minimizing Interfacial Recombination in 1.8 eV Triple‐Halide Perovskites for 27.5% Efficient All‐Perovskite Tandems},
author = {Yang, Fengjiu and Tockhorn, Philipp and Musiienko, Artem and Lang, Felix and Menzel, Dorothee and Macqueen, Rowan and Köhnen, Eike and Xu, Ke and Mariotti, Silvia and Mantione, Daniele and Merten, Lena and Hinderhofer, Alexander and Li, Bor and Wargulski, Dan R. and Harvey, Steven P. and Zhang, Jiahuan and Scheler, Florian and Berwig, Sebastian and Roß, Marcel and Thiesbrummel, Jarla and Al‐Ashouri, Amran and Brinkmann, Kai O. and Riedl, Thomas and Schreiber, Frank and Abou‐Ras, Daniel and Snaith, Henry and Neher, Dieter and Korte, Lars and Stolterfoht, Martin and Albrecht, Steve},
abstractNote = {Abstract All‐perovskite tandem solar cells show great potential to enable the highest performance at reasonable costs for a viable market entry in the near future. In particular, wide‐bandgap (WBG) perovskites with higher open‐circuit voltage ( V OC ) are essential to further improve the tandem solar cells’ performance. Here, a new 1.8 eV bandgap triple‐halide perovskite composition in conjunction with a piperazinium iodide (PI) surface treatment is developed. With structural analysis, it is found that the PI modifies the surface through a reduction of excess lead iodide in the perovskite and additionally penetrates the bulk. Constant light‐induced magneto‐transport measurements are applied to separately resolve charge carrier properties of electrons and holes. These measurements reveal a reduced deep trap state density, and improved steady‐state carrier lifetime (factor 2.6) and diffusion lengths (factor 1.6). As a result, WBG PSCs achieve 1.36 V V OC , reaching 90% of the radiative limit. Combined with a 1.26 eV narrow bandgap (NBG) perovskite with a rubidium iodide additive, this enables a tandem cell with a certified scan efficiency of 27.5%.},
doi = {10.1002/adma.202307743},
journal = {Advanced Materials},
number = 6,
volume = 36,
place = {Germany},
year = {Wed Dec 06 00:00:00 EST 2023},
month = {Wed Dec 06 00:00:00 EST 2023}
}
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