Halide Perovskites and Their Derivatives for Efficient, High‐Resolution Direct Radiation Detection: Design Strategies and Applications
Abstract
Abstract The past decade has witnessed a rapid rise in the performance of optoelectronic devices based on lead‐halide perovskites (LHPs). The large mobility‐lifetime products and defect tolerance of these materials, essential for optoelectronics, also make them well‐suited for radiation detectors, especially given the heavy elements present, which is essential for strong X‐ray and γ‐ray attenuation. Over the past decade, LHP thick films, wafers, and single crystals have given rise to direct radiation detectors that have outperformed incumbent technologies in terms of sensitivity (reported values up to 3.5 × 10 6 µC Gy air −1 cm −2 ), limit of detection (directly measured values down to 1.5 nGy air s −1 ), along with competitive energy and imaging resolution at room temperature. At the same time, lead‐free perovskite‐inspired materials (e.g., methylammonium bismuth iodide), which have underperformed in solar cells, have recently matched and, in some areas (e.g., in polarization stability), surpassed the performance of LHP detectors. These advances open up opportunities to achieve devices for safer medical imaging, as well as more effective non‐invasive analysis for security, nuclear safety, or product inspection applications. Herein, the principles behind the rapid rises in performance of LHP and perovskite‐inspired material detectors, and how their properties andmore »
- Authors:
-
[2];
[2];
[1]
- Inorganic Chemistry Laboratory University of Oxford Oxford OX1 3QR UK
- Center for Integrated Nanotechnologies Los Alamos National Laboratory Los Alamos NM 87545 USA
- Publication Date:
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 2228978
- Alternate Identifier(s):
- OSTI ID: 2229766
- Resource Type:
- Published Article
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Name: Advanced Materials Journal Volume: 36 Journal Issue: 8; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley Blackwell (John Wiley & Sons)
- Country of Publication:
- Germany
- Language:
- English
Citation Formats
Dudipala, Kavya Reddy, Le, Thanh‐Hai, Nie, Wanyi, and Hoye, Robert L. Z. Halide Perovskites and Their Derivatives for Efficient, High‐Resolution Direct Radiation Detection: Design Strategies and Applications. Germany: N. p., 2023.
Web. doi:10.1002/adma.202304523.
Dudipala, Kavya Reddy, Le, Thanh‐Hai, Nie, Wanyi, & Hoye, Robert L. Z. Halide Perovskites and Their Derivatives for Efficient, High‐Resolution Direct Radiation Detection: Design Strategies and Applications. Germany. https://doi.org/10.1002/adma.202304523
Dudipala, Kavya Reddy, Le, Thanh‐Hai, Nie, Wanyi, and Hoye, Robert L. Z. Wed .
"Halide Perovskites and Their Derivatives for Efficient, High‐Resolution Direct Radiation Detection: Design Strategies and Applications". Germany. https://doi.org/10.1002/adma.202304523.
@article{osti_2228978,
title = {Halide Perovskites and Their Derivatives for Efficient, High‐Resolution Direct Radiation Detection: Design Strategies and Applications},
author = {Dudipala, Kavya Reddy and Le, Thanh‐Hai and Nie, Wanyi and Hoye, Robert L. Z.},
abstractNote = {Abstract The past decade has witnessed a rapid rise in the performance of optoelectronic devices based on lead‐halide perovskites (LHPs). The large mobility‐lifetime products and defect tolerance of these materials, essential for optoelectronics, also make them well‐suited for radiation detectors, especially given the heavy elements present, which is essential for strong X‐ray and γ‐ray attenuation. Over the past decade, LHP thick films, wafers, and single crystals have given rise to direct radiation detectors that have outperformed incumbent technologies in terms of sensitivity (reported values up to 3.5 × 10 6 µC Gy air −1 cm −2 ), limit of detection (directly measured values down to 1.5 nGy air s −1 ), along with competitive energy and imaging resolution at room temperature. At the same time, lead‐free perovskite‐inspired materials (e.g., methylammonium bismuth iodide), which have underperformed in solar cells, have recently matched and, in some areas (e.g., in polarization stability), surpassed the performance of LHP detectors. These advances open up opportunities to achieve devices for safer medical imaging, as well as more effective non‐invasive analysis for security, nuclear safety, or product inspection applications. Herein, the principles behind the rapid rises in performance of LHP and perovskite‐inspired material detectors, and how their properties and performance link with critical applications in non‐invasive diagnostics are discussed. The key strategies to engineer the performance of these materials, and the important challenges to overcome to commercialize these new technologies are also discussed.},
doi = {10.1002/adma.202304523},
journal = {Advanced Materials},
number = 8,
volume = 36,
place = {Germany},
year = {Wed Dec 06 00:00:00 EST 2023},
month = {Wed Dec 06 00:00:00 EST 2023}
}
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