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Title: Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause

Abstract

The MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition was the largest Arctic field campaign ever conducted. MOSAiC offered the unique opportunity to monitor and characterize aerosols and clouds with high vertical resolution up to 30 km height at latitudes from 80 to 90 °N over an entire year (October 2019 to September 2020). Without a clear knowledge of the complex aerosol layering, vertical structures, and dominant aerosol types and their impact on cloud formation, a full understanding of the meteorological processes in the Arctic, and thus advanced climate change research, is impossible. Widespread ground-based in situ observations in the Arctic are insufficient to provide these required aerosol and cloud data. In this article, a summary of our MOSAiC observations of tropospheric aerosol profiles with a state-of-the-art multiwavelength polarization Raman lidar aboard the icebreaker Polarstern is presented. Particle optical properties, i.e., light-extinction profiles and aerosol optical thickness (AOT), and estimates of cloud-relevant aerosol properties such as the number concentration of cloud condensation nuclei (CCN) and ice-nucleating particles (INPs) are discussed, separately for the lowest part of the troposphere (atmospheric boundary layer, ABL), within the lower free troposphere (around 2000 m height), and at the cirrus level closemore » to the tropopause. In situ observations of the particle number concentration and INPs aboard Polarstern are included in the study. A strong decrease in the aerosol amount with height in winter and moderate vertical variations in summer were observed in terms of the particle extinction coefficient. The 532 nm light-extinction values dropped from >50 Mm-1 close to the surface to <5 Mm-1 at 4–6 km height in the winter months. Lofted, aged wildfire smoke layers caused a re-increase in the aerosol concentration towards the tropopause. In summer (June to August 2020), much lower particle extinction coefficients, frequently as low as 1–5 Mm-1, were observed in the ABL. Aerosol removal, controlled by in-cloud and below-cloud scavenging processes (widely suppressed in winter and very efficient in summer) in the lowermost 1–2 km of the atmosphere, seems to be the main reason for the strong differences between winter and summer aerosol conditions. A complete annual cycle of the AOT in the central Arctic could be measured. This is a valuable addition to the summertime observations with the sun photometers of the Arctic Aerosol Robotic Network (AERONET). In line with the pronounced annual cycle in the aerosol optical properties, typical CCN number concentrations (0.2 % supersaturation level) ranged from 50–500 cm-3 in winter to 10–100 cm-3 in summer in the ABL. In the lower free troposphere (at 2000 m), however, the CCN level was roughly constant throughout the year, with values mostly from 30 to 100 cm-3. A strong contrast between winter and summer was also given in terms of ABL INPs which control ice production in low-level clouds. While soil dust (from surrounding continents) is probably the main INP type during the autumn, winter, and spring months, local sea spray aerosol (with a biogenic aerosol component) seems to dominate the ice nucleation in the ABL during the summer months (June–August). The strong winter vs. summer contrast in the INP number concentration by roughly 2–3 orders of magnitude in the lower troposphere is, however, mainly caused by the strong cloud temperature contrast. A unique event of the MOSAiC expedition was the occurrence of a long-lasting wildfire smoke layer in the upper troposphere and lower stratosphere. Our observations suggest that the smoke particles frequently triggered cirrus formation close to the tropopause from October 2019 to May 2020.« less

Authors:
; ; ORCiD logo; ORCiD logo; ORCiD logo; ORCiD logo; ORCiD logo; ORCiD logo; ; ORCiD logo; ORCiD logo; ORCiD logo; ; ORCiD logo; ORCiD logo; ORCiD logo; ORCiD logo
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Atmospheric Radiation Measurement (ARM) Data Center; Colorado State Univ., Fort Collins, CO (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Biological and Environmental Research (BER); German Federal Ministry for Education and Research (BMBF); Alfred Wegener Institute; European Union's Horizon 2020; German Research Foundation (DFG)
OSTI Identifier:
2067671
Alternate Identifier(s):
OSTI ID: 2229260
Grant/Contract Number:  
AC05-76RL01830; DESC0021034; SC0019745; SC002204; SC0021034; N-2014-H-060_Dethloff; AFMOSAiC-1_00; AWI_PS122_00; 654109
Resource Type:
Published Article
Journal Name:
Atmospheric Chemistry and Physics (Online)
Additional Journal Information:
Journal Name: Atmospheric Chemistry and Physics (Online) Journal Volume: 23 Journal Issue: 19; Journal ID: ISSN 1680-7324
Publisher:
Copernicus GmbH
Country of Publication:
Germany
Language:
English
Subject:
54 ENVIRONMENTAL SCIENCES

Citation Formats

Ansmann, Albert, Ohneiser, Kevin, Engelmann, Ronny, Radenz, Martin, Griesche, Hannes, Hofer, Julian, Althausen, Dietrich, Creamean, Jessie M., Boyer, Matthew C., Knopf, Daniel A., Dahlke, Sandro, Maturilli, Marion, Gebauer, Henriette, Bühl, Johannes, Jimenez, Cristofer, Seifert, Patric, and Wandinger, Ulla. Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause. Germany: N. p., 2023. Web. doi:10.5194/acp-23-12821-2023.
Ansmann, Albert, Ohneiser, Kevin, Engelmann, Ronny, Radenz, Martin, Griesche, Hannes, Hofer, Julian, Althausen, Dietrich, Creamean, Jessie M., Boyer, Matthew C., Knopf, Daniel A., Dahlke, Sandro, Maturilli, Marion, Gebauer, Henriette, Bühl, Johannes, Jimenez, Cristofer, Seifert, Patric, & Wandinger, Ulla. Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause. Germany. https://doi.org/10.5194/acp-23-12821-2023
Ansmann, Albert, Ohneiser, Kevin, Engelmann, Ronny, Radenz, Martin, Griesche, Hannes, Hofer, Julian, Althausen, Dietrich, Creamean, Jessie M., Boyer, Matthew C., Knopf, Daniel A., Dahlke, Sandro, Maturilli, Marion, Gebauer, Henriette, Bühl, Johannes, Jimenez, Cristofer, Seifert, Patric, and Wandinger, Ulla. Thu . "Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause". Germany. https://doi.org/10.5194/acp-23-12821-2023.
@article{osti_2067671,
title = {Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause},
author = {Ansmann, Albert and Ohneiser, Kevin and Engelmann, Ronny and Radenz, Martin and Griesche, Hannes and Hofer, Julian and Althausen, Dietrich and Creamean, Jessie M. and Boyer, Matthew C. and Knopf, Daniel A. and Dahlke, Sandro and Maturilli, Marion and Gebauer, Henriette and Bühl, Johannes and Jimenez, Cristofer and Seifert, Patric and Wandinger, Ulla},
abstractNote = {The MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition was the largest Arctic field campaign ever conducted. MOSAiC offered the unique opportunity to monitor and characterize aerosols and clouds with high vertical resolution up to 30 km height at latitudes from 80 to 90 °N over an entire year (October 2019 to September 2020). Without a clear knowledge of the complex aerosol layering, vertical structures, and dominant aerosol types and their impact on cloud formation, a full understanding of the meteorological processes in the Arctic, and thus advanced climate change research, is impossible. Widespread ground-based in situ observations in the Arctic are insufficient to provide these required aerosol and cloud data. In this article, a summary of our MOSAiC observations of tropospheric aerosol profiles with a state-of-the-art multiwavelength polarization Raman lidar aboard the icebreaker Polarstern is presented. Particle optical properties, i.e., light-extinction profiles and aerosol optical thickness (AOT), and estimates of cloud-relevant aerosol properties such as the number concentration of cloud condensation nuclei (CCN) and ice-nucleating particles (INPs) are discussed, separately for the lowest part of the troposphere (atmospheric boundary layer, ABL), within the lower free troposphere (around 2000 m height), and at the cirrus level close to the tropopause. In situ observations of the particle number concentration and INPs aboard Polarstern are included in the study. A strong decrease in the aerosol amount with height in winter and moderate vertical variations in summer were observed in terms of the particle extinction coefficient. The 532 nm light-extinction values dropped from >50 Mm-1 close to the surface to <5 Mm-1 at 4–6 km height in the winter months. Lofted, aged wildfire smoke layers caused a re-increase in the aerosol concentration towards the tropopause. In summer (June to August 2020), much lower particle extinction coefficients, frequently as low as 1–5 Mm-1, were observed in the ABL. Aerosol removal, controlled by in-cloud and below-cloud scavenging processes (widely suppressed in winter and very efficient in summer) in the lowermost 1–2 km of the atmosphere, seems to be the main reason for the strong differences between winter and summer aerosol conditions. A complete annual cycle of the AOT in the central Arctic could be measured. This is a valuable addition to the summertime observations with the sun photometers of the Arctic Aerosol Robotic Network (AERONET). In line with the pronounced annual cycle in the aerosol optical properties, typical CCN number concentrations (0.2 % supersaturation level) ranged from 50–500 cm-3 in winter to 10–100 cm-3 in summer in the ABL. In the lower free troposphere (at 2000 m), however, the CCN level was roughly constant throughout the year, with values mostly from 30 to 100 cm-3. A strong contrast between winter and summer was also given in terms of ABL INPs which control ice production in low-level clouds. While soil dust (from surrounding continents) is probably the main INP type during the autumn, winter, and spring months, local sea spray aerosol (with a biogenic aerosol component) seems to dominate the ice nucleation in the ABL during the summer months (June–August). The strong winter vs. summer contrast in the INP number concentration by roughly 2–3 orders of magnitude in the lower troposphere is, however, mainly caused by the strong cloud temperature contrast. A unique event of the MOSAiC expedition was the occurrence of a long-lasting wildfire smoke layer in the upper troposphere and lower stratosphere. Our observations suggest that the smoke particles frequently triggered cirrus formation close to the tropopause from October 2019 to May 2020.},
doi = {10.5194/acp-23-12821-2023},
journal = {Atmospheric Chemistry and Physics (Online)},
number = 19,
volume = 23,
place = {Germany},
year = {Thu Oct 12 00:00:00 EDT 2023},
month = {Thu Oct 12 00:00:00 EDT 2023}
}

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Retrieval of ice-nucleating particle concentrations from lidar observations and comparison with UAV in situ measurements
journal, January 2019

  • Marinou, Eleni; Tesche, Matthias; Nenes, Athanasios
  • Atmospheric Chemistry and Physics, Vol. 19, Issue 17
  • DOI: 10.5194/acp-19-11315-2019

Microphysical investigation of the seeder and feeder region of an Alpine mixed-phase cloud
journal, January 2021

  • Ramelli, Fabiola; Henneberger, Jan; David, Robert O.
  • Atmospheric Chemistry and Physics, Vol. 21, Issue 9
  • DOI: 10.5194/acp-21-6681-2021

Processes Controlling the Composition and Abundance of Arctic Aerosol
journal, November 2018

  • Willis, Megan D.; Leaitch, W. Richard; Abbatt, Jonathan P. D.
  • Reviews of Geophysics, Vol. 56, Issue 4
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Marine and terrestrial influences on ice nucleating particles during continuous springtime measurements in an Arctic oilfield location
journal, January 2018

  • Creamean, Jessie M.; Kirpes, Rachel M.; Pratt, Kerri A.
  • Atmospheric Chemistry and Physics, Vol. 18, Issue 24
  • DOI: 10.5194/acp-18-18023-2018

The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review
journal, January 2018


Automated time–height-resolved air mass source attribution for profiling remote sensing applications
journal, March 2021

  • Radenz, Martin; Seifert, Patric; Baars, Holger
  • Atmospheric Chemistry and Physics, Vol. 21, Issue 4
  • DOI: 10.5194/acp-21-3015-2021

Long-term profiling of mineral dust and pollution aerosol with multiwavelength polarization Raman lidar at the Central Asian site of Dushanbe, Tajikistan: case studies
journal, December 2017

  • Hofer, Julian; Althausen, Dietrich; Abdullaev, Sabur F.
  • Atmospheric Chemistry and Physics, Vol. 17, Issue 23
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Heterogeneous nucleation of ice particles on glassy aerosols under cirrus conditions
journal, March 2010

  • Murray, Benjamin J.; Wilson, Theodore W.; Dobbie, Steven
  • Nature Geoscience, Vol. 3, Issue 4
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The automated multiwavelength Raman polarization and water-vapor lidar PollyXT: the neXT generation
journal, January 2016

  • Engelmann, Ronny; Kanitz, Thomas; Baars, Holger
  • Atmospheric Measurement Techniques, Vol. 9, Issue 4
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The characterization of long-range transported North American biomass burning plumes: what can a multi-wavelength Mie–Raman-polarization-fluorescence lidar provide?
journal, April 2022

  • Hu, Qiaoyun; Goloub, Philippe; Veselovskii, Igor
  • Atmospheric Chemistry and Physics, Vol. 22, Issue 8
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Contrasting the impact of aerosols at northern and southern midlatitudes on heterogeneous ice formation: AEROSOL EFFECT ON ICE FORMATION
journal, September 2011

  • Kanitz, T.; Seifert, P.; Ansmann, A.
  • Geophysical Research Letters, Vol. 38, Issue 17
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Ice-nucleating particles in northern Greenland: annual cycles, biological contribution and parameterizations
journal, April 2023

  • Sze, Kevin C. H.; Wex, Heike; Hartmann, Markus
  • Atmospheric Chemistry and Physics, Vol. 23, Issue 8
  • DOI: 10.5194/acp-23-4741-2023

Real-time Environmental Applications and Display sYstem: READY
journal, September 2017


Evaluation of aerosol number concentrations from CALIPSO with ATom airborne in situ measurements
journal, June 2022

  • Choudhury, Goutam; Ansmann, Albert; Tesche, Matthias
  • Atmospheric Chemistry and Physics, Vol. 22, Issue 11
  • DOI: 10.5194/acp-22-7143-2022

AERONET—A Federated Instrument Network and Data Archive for Aerosol Characterization
journal, October 1998


Wildfire smoke, Arctic haze, and aerosol effects on mixed-phase and cirrus clouds over the North Pole region during MOSAiC: an introduction
journal, January 2021

  • Engelmann, Ronny; Ansmann, Albert; Ohneiser, Kevin
  • Atmospheric Chemistry and Physics, Vol. 21, Issue 17
  • DOI: 10.5194/acp-21-13397-2021

The immersion mode ice nucleation behavior of mineral dusts: A comparison of different pure and surface modified dusts
journal, October 2014

  • Augustin-Bauditz, S.; Wex, H.; Kanter, S.
  • Geophysical Research Letters, Vol. 41, Issue 20
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Heterogeneous ice nucleation properties of natural desert dust particles coated with a surrogate of secondary organic aerosol
journal, January 2019

  • Kanji, Zamin A.; Sullivan, Ryan C.; Niemand, Monika
  • Atmospheric Chemistry and Physics, Vol. 19, Issue 7
  • DOI: 10.5194/acp-19-5091-2019

Integrating laboratory and field data to quantify the immersion freezing ice nucleation activity of mineral dust particles
journal, January 2015

  • DeMott, P. J.; Prenni, A. J.; McMeeking, G. R.
  • Atmospheric Chemistry and Physics, Vol. 15, Issue 1
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Arctic Air Pollution: New Insights from POLARCAT-IPY
journal, December 2014

  • Law, Katharine S.; Stohl, Andreas; Quinn, Patricia K.
  • Bulletin of the American Meteorological Society, Vol. 95, Issue 12
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Ambient aerosol properties in the remote atmosphere from global-scale in situ measurements
journal, January 2021

  • Brock, Charles A.; Froyd, Karl D.; Dollner, Maximilian
  • Atmospheric Chemistry and Physics, Vol. 21, Issue 19
  • DOI: 10.5194/acp-21-15023-2021

Sources of carbonaceous aerosols and deposited black carbon in the Arctic in winter-spring: implications for radiative forcing
journal, January 2011


NOAA’s HYSPLIT Atmospheric Transport and Dispersion Modeling System
journal, December 2015

  • Stein, A. F.; Draxler, R. R.; Rolph, G. D.
  • Bulletin of the American Meteorological Society, Vol. 96, Issue 12
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A Stochastic Representation of Temperature Fluctuations Induced by Mesoscale Gravity Waves
journal, November 2019

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  • Journal of Geophysical Research: Atmospheres, Vol. 124, Issue 21
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Heterogeneous ice nucleation on particles composed of humic-like substances impacted by O 3
journal, January 2011

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Aerosol remote sensing in polar regions
journal, January 2015


Application of the shipborne remote sensing supersite OCEANET for profiling of Arctic aerosols and clouds during Polarstern cruise PS106
journal, January 2020

  • Griesche, Hannes J.; Seifert, Patric; Ansmann, Albert
  • Atmospheric Measurement Techniques, Vol. 13, Issue 10
  • DOI: 10.5194/amt-13-5335-2020

A unified synergistic retrieval of clouds, aerosols, and precipitation from EarthCARE: the ACM-CAP product
journal, July 2023

  • Mason, Shannon L.; Hogan, Robin J.; Bozzo, Alessio
  • Atmospheric Measurement Techniques, Vol. 16, Issue 13
  • DOI: 10.5194/amt-16-3459-2023

The unexpected smoke layer in the High Arctic winter stratosphere during MOSAiC 2019–2020
journal, January 2021

  • Ohneiser, Kevin; Ansmann, Albert; Chudnovsky, Alexandra
  • Atmospheric Chemistry and Physics, Vol. 21, Issue 20
  • DOI: 10.5194/acp-21-15783-2021

Tropospheric and stratospheric wildfire smoke profiling with lidar: mass, surface area, CCN, and INP retrieval
journal, January 2021

  • Ansmann, Albert; Ohneiser, Kevin; Mamouri, Rodanthi-Elisavet
  • Atmospheric Chemistry and Physics, Vol. 21, Issue 12
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Ice Nucleating Particles Carried From Below a Phytoplankton Bloom to the Arctic Atmosphere
journal, July 2019

  • Creamean, J. M.; Cross, J. N.; Pickart, R.
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Spaceborne Evidence That Ice‐Nucleating Particles Influence High‐Latitude Cloud Phase
journal, July 2022

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Atmospheric ice nucleation
journal, March 2023


Ship-borne aerosol profiling with lidar over the Atlantic Ocean: from pure marine conditions to complex dust–smoke mixtures
journal, July 2018

  • Bohlmann, Stephanie; Baars, Holger; Radenz, Martin
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The CALIPSO Mission: A Global 3D View of Aerosols and Clouds
journal, September 2010

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Black carbon lofts wildfire smoke high into the stratosphere to form a persistent plume
journal, August 2019


Meteorological conditions during the MOSAiC expedition
journal, January 2021

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Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 1: Climatology and trend
journal, August 2022

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Ice nucleation of bare and sulfuric acid-coated mineral dust particles and implication for cloud properties: Ice formation on dust particles
journal, August 2014

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  • Journal of Geophysical Research: Atmospheres, Vol. 119, Issue 16
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Characteristics of atmospheric transport into the Arctic troposphere
journal, January 2006


Sea spray aerosol as a unique source of ice nucleating particles
journal, December 2015

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An update on polar aerosol optical properties using POLAR-AOD and other measurements performed during the International Polar Year
journal, June 2012


Quantifying the low bias of CALIPSO's column aerosol optical depth due to undetected aerosol layers: Undetected Aerosols in CALIPSO AOD
journal, January 2017

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Aerosols in current and future Arctic climate
journal, February 2021


An overview of the first decade of Polly NET : an emerging network of automated Raman-polarization lidars for continuous aerosol profiling
journal, January 2016

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Ice nucleation by fertile soil dusts: relative importance of mineral and biogenic components
journal, January 2014

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Annual cycle observations of aerosols capable of ice formation in central Arctic clouds
journal, June 2022


Potential of polarization lidar to provide profiles of CCN- and INP-relevant aerosol parameters
journal, January 2016

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Study of polar thin ice clouds and aerosols seen by CloudSat and CALIPSO during midwinter 2007
journal, January 2009

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Terrestrial or marine – indications towards the origin of ice-nucleating particles during melt season in the European Arctic up to 83.7° N
journal, January 2021

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  • DOI: 10.5194/acp-21-11613-2021

Overview of Ice Nucleating Particles
journal, January 2017