Emerging Modification Technologies of Lignin-based Activated Carbon toward Advanced Applications

Chen, Kai; He, Zi‐Jing; Liu, Zhi‐Hua; Ragauskas, Arthur J.; Li, Bing‐Zhi; Yuan, Ying‐Jin

doi:10.1002/cssc.202201284

Title: Emerging Modification Technologies of Lignin-based Activated Carbon toward Advanced Applications

Journal Article · Mon Sep 12 00:00:00 UTC 2022 · ChemSusChem

DOI: https://doi.org/10.1002/cssc.202201284 · OSTI ID:2000344

Chen, Kai ^[1]; He, Zi‐Jing ^[1]; Liu, Zhi‐Hua ^[1];

^[2];

^[1]; Yuan, Ying‐Jin ^[1]

Tianjin Univ. (China)
Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Joint Institute for Biological Sciences (JIBS)

Lignin-based activated carbon (LAC) is a promising high-quality functional material due to high surface area, abundant porous structure, and various functional groups. Modification is the most important step to functionalize LAC by altering its porous and chemical properties. Here, this Review summarizes the state-of-the-art modification technologies of LAC toward advanced applications. Promising modification approaches are reviewed to display their effects on the preparation of LAC. The multiscale changes in the porosity and the surface chemistry of LAC are fully discussed. Advanced applications are then introduced to show the potential of LAC for supercapacitor electrode, catalyst support, hydrogen storage, and carbon dioxide capture. Finally, the mechanistic structure-function relationships of LAC are elaborated. These results highlight that modification technologies play a special role in altering the properties and defining the functionalities of LAC, which could be a promising porous carbon material toward industrial applications.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 2000344

Journal Information:: ChemSusChem, Journal Name: ChemSusChem Journal Issue: 21 Vol. 15; ISSN 1864-5631

Publisher:: ChemPubSoc EuropeCopyright Statement

Country of Publication:: United States

Language:: English

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Codesign of Combinatorial Organosolv Pretreatment (COP) and Lignin Nanoparticles (LNPs) in Biorefineries Liu, Zhi-Hua; Hao, Naijia; Shinde, Somnath ACS Sustainable Chemistry & Engineering, Vol. 7, Issue 2 https://doi.org/10.1021/acssuschemeng.8b05715	journal	December 2018
Toward Process-Resilient Lignin-Derived Activated Carbons for Hydrogen Storage Applications Rowlandson, Jemma L.; Edler, Karen J.; Tian, Mi ACS Sustainable Chemistry & Engineering, Vol. 8, Issue 5 https://doi.org/10.1021/acssuschemeng.9b05869	journal	January 2020
Transforming biorefinery designs with ‘Plug-In Processes of Lignin’ to enable economic waste valorization Liu, Zhi-Hua; Hao, Naijia; Wang, Yun-Yan Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-021-23920-4	journal	June 2021
Fabrication of Pd NPs-supported porous carbon by integrating the reducing reactivity and carbon-rich network of lignin Han, Guocheng; Jiang, Qimeng; Ye, Weijie Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-43840-0	journal	May 2019
The role of H₃PO₄in the preparation of activated carbon from NaOH-treated rice husk residue Li, Yaxin; Zhang, Xian; Yang, Ruiguang RSC Advances, Vol. 5, Issue 41 https://doi.org/10.1039/C5RA04634C	journal	January 2015
Synergistical enhancement of the electrochemical properties of lignin-based activated carbon using NH₃·H₂O dielectric barrier discharge plasma Chen, Weimin; Zhou, Xiaoyan; Shi, Shukai RSC Advances, Vol. 7, Issue 12 https://doi.org/10.1039/C6RA26010A	journal	January 2017
Latest advances in supercapacitors: from new electrode materials to novel device designs Wang, Faxing; Wu, Xiongwei; Yuan, Xinhai Chemical Society Reviews, Vol. 46, Issue 22 https://doi.org/10.1039/C7CS00205J	journal	January 2017
Chemicals from lignin: an interplay of lignocellulose fractionation, depolymerisation, and upgrading Schutyser, W.; Renders, T.; Van den Bosch, S. Chemical Society Reviews, Vol. 47, Issue 3 https://doi.org/10.1039/C7CS00566K	journal	January 2018
Enzymatic hydrolysis lignin derived hierarchical porous carbon for supercapacitors in ionic liquids with high power and energy densities Guo, Nannan; Li, Min; Sun, Xingkai Green Chemistry, Vol. 19, Issue 11 https://doi.org/10.1039/C7GC00506G	journal	January 2017
Defining lignin nanoparticle properties through tailored lignin reactivity by sequential organosolv fragmentation approach (SOFA) Liu, Zhi-Hua; Hao, Naijia; Shinde, Somnath Green Chemistry, Vol. 21, Issue 2 https://doi.org/10.1039/C8GC03290D	journal	January 2019
High-performance supercapacitor energy storage using a carbon material derived from lignin by bacterial activation before carbonization Zhang, Kejing; Liu, Mingren; Zhang, Tingzheng Journal of Materials Chemistry A, Vol. 7, Issue 47 https://doi.org/10.1039/C9TA04369A	journal	January 2019
Guidelines for performing lignin-first biorefining Abu-Omar, Mahdi M.; Barta, Katalin; Beckham, Gregg T. Energy & Environmental Science, Vol. 14, Issue 1 https://doi.org/10.1039/D0EE02870C	journal	January 2021
A comparative study of thermochemical and cold plasma treatment on lignin-based activated carbon for adsorbing Fe(III) Shi, Shukai; Wang, Xin; Chen, Weimin Materials Research Express, Vol. 5, Issue 5 https://doi.org/10.1088/2053-1591/aac232	journal	May 2018
Carbon-based supercapacitors for efficient energy storage Chen, Xuli; Paul, Rajib; Dai, Liming National Science Review, Vol. 4, Issue 3 https://doi.org/10.1093/nsr/nwx009	journal	March 2017
Composites from renewable and sustainable resources: Challenges and innovations Mohanty, Amar K.; Vivekanandhan, Singaravelu; Pin, Jean-Mathieu Science, Vol. 362, Issue 6414 https://doi.org/10.1126/science.aat9072	journal	November 2018
A heterogeneous microbial consortium producing short-chain fatty acids from lignocellulose Shahab, Robert L.; Brethauer, Simone; Davey, Matthew P. Science, Vol. 369, Issue 6507 https://doi.org/10.1126/science.abb1214	journal	August 2020
A Self-Assembled and Flexible Supercapacitor based on Redox-Active Lignin-Based Nitrogen-Doped Activated Carbon Functionalized Graphene Hydrogels Cui, Linlin; Li, Yue; Jia, Mengying Journal of The Electrochemical Society, Vol. 168, Issue 5 https://doi.org/10.1149/1945-7111/ac00f6	journal	May 2021
Preparation of Different Carbon Materials by Thermochemical Conversion of Lignin Rosas, Juana M.; Berenguer, RaÃºl; Valero-Romero, MarÃa JosÃ© Frontiers in Materials, Vol. 1 https://doi.org/10.3389/fmats.2014.00029	journal	December 2014
Effect of Co-solution of Carbon Precursor and Activating Agent on the Textural Properties of Highly Porous Activated Carbon Obtained by Chemical Activation of Lignin With H3PO4 Moulefera, Imane; García-Mateos, Francisco J.; Benyoucef, Abdelghani Frontiers in Materials, Vol. 7 https://doi.org/10.3389/fmats.2020.00153	journal	May 2020
Nitrogen Oxide Removal by Coal-Based Activated Carbon for a Marine Diesel Engine Wang, Zongyu; Kuang, Hailang; Zhang, Jifeng Applied Sciences, Vol. 9, Issue 8 https://doi.org/10.3390/app9081656	journal	April 2019
Preparation of Lignin-Based Carbon Materials and Its Application as a Sorbent Meng, Ling-Yan; Ma, Ming-Guo; Ji, Xing-Xiang Materials, Vol. 12, Issue 7 https://doi.org/10.3390/ma12071111	journal	April 2019
Lignin Based Activated Carbon Using H3PO4 Activation Yang, Zhongzhi; Gleisner, Roland; H. Mann, Doreen Polymers, Vol. 12, Issue 12 https://doi.org/10.3390/polym12122829	journal	November 2020
Activated carbon as catalyst support: precursors, preparation, modification and characterization Iwanow, Melanie; Gärtner, Tobias; Sieber, Volker Beilstein Journal of Organic Chemistry, Vol. 16 https://doi.org/10.3762/bjoc.16.104	journal	January 2020

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