Evolution of plasmon excitations across the phase diagram of the cuprate superconductor La 2 − x Sr x CuO 4

Hepting, M.; Boyko, T. D.; Zimmermann, V.; Bejas, M.; Suyolcu, Y. E.; Puphal, P.; Green, R. J.; Zinni, L.; Kim, J.; Casa, D.; Upton, M. H.; Wong, D.; Schulz, C.; Bartkowiak, M.; Habicht, K.; Pomjakushina, E.; Cristiani, G.; Logvenov, G.; Minola, M.; Yamase, H.; Greco, A.; Keimer, B.

doi:10.1103/PhysRevB.107.214516

Title: Evolution of plasmon excitations across the phase diagram of the cuprate superconductor ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$

Abstract

We use resonant inelastic x-ray scattering (RIXS) at the O K- and Cu K-edges to investigate the doping dependence and temperature dependence of low-energy plasmon excitations in La_2–xSr_xCuO₄. We observe a monotonic increase of the energy scale of the plasmons with increasing doping x in the underdoped regime, whereas a saturation occurs above optimal doping x ≳ 0.16 and persists at least up to x = 0.4. Furthermore, we find that the plasmon excitations show only a marginal temperature dependence, and possible effects due to the superconducting transition and the onset of strange metal behavior are either absent or below the detection limit of our experiment. Taking into account the strongly correlated character of the cuprates, we show that layered t – J – V model calculations accurately capture the increase of the plasmon energy in the underdoped regime. However, the computed plasmon energy continues to increase even for doping levels above x ≳ 0.16, which is distinct from the experimentally observed saturation and reaches a broad maximum around x = 0.55. We discuss whether possible lattice disorder in overdoped samples, a renormalization of the electronic correlation strength at high dopings, or an increasing relevance of nonplanar Cu and Omore »« less

Authors:

;

; Kim, J.; Casa, D.; Upton, M. H.; Wong, D.;

;

; Cristiani, G.; Logvenov, G.;

;

Publication Date:: Mon Jun 26 00:00:00 EDT 2023

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF); Japan Society for the Promotion of Science (JSPS) (KAKENHI)

OSTI Identifier:: 1986580

Alternate Identifier(s):: OSTI ID: 2229141

Grant/Contract Number:: AC02-06CH11357; JP20H01856

Resource Type:: Published Article

Journal Name:: Physical Review. B

Additional Journal Information:: Journal Name: Physical Review. B Journal Volume: 107 Journal Issue: 21; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Hepting, M., Boyko, T. D., Zimmermann, V., Bejas, M., Suyolcu, Y. E., Puphal, P., Green, R. J., Zinni, L., Kim, J., Casa, D., Upton, M. H., Wong, D., Schulz, C., Bartkowiak, M., Habicht, K., Pomjakushina, E., Cristiani, G., Logvenov, G., Minola, M., Yamase, H., Greco, A., and Keimer, B. Evolution of plasmon excitations across the phase diagram of the cuprate superconductor La 2 − x Sr x CuO 4.  United States: N. p., 2023. 
Web.  doi:10.1103/PhysRevB.107.214516.

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                    Hepting, M., Boyko, T. D., Zimmermann, V., Bejas, M., Suyolcu, Y. E., Puphal, P., Green, R. J., Zinni, L., Kim, J., Casa, D., Upton, M. H., Wong, D., Schulz, C., Bartkowiak, M., Habicht, K., Pomjakushina, E., Cristiani, G., Logvenov, G., Minola, M., Yamase, H., Greco, A., & Keimer, B. Evolution of plasmon excitations across the phase diagram of the cuprate superconductor La 2 − x Sr x CuO 4.  United States.  https://doi.org/10.1103/PhysRevB.107.214516

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                    Hepting, M., Boyko, T. D., Zimmermann, V., Bejas, M., Suyolcu, Y. E., Puphal, P., Green, R. J., Zinni, L., Kim, J., Casa, D., Upton, M. H., Wong, D., Schulz, C., Bartkowiak, M., Habicht, K., Pomjakushina, E., Cristiani, G., Logvenov, G., Minola, M., Yamase, H., Greco, A., and Keimer, B. Mon .  
"Evolution of plasmon excitations across the phase diagram of the cuprate superconductor La 2 − x Sr x CuO 4".  United States.  https://doi.org/10.1103/PhysRevB.107.214516.

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@article{osti_1986580,

  title        = {Evolution of plasmon excitations across the phase diagram of the cuprate superconductor La 2 − x Sr x CuO 4},

  author       = {Hepting, M. and Boyko, T. D. and Zimmermann, V. and Bejas, M. and Suyolcu, Y. E. and Puphal, P. and Green, R. J. and Zinni, L. and Kim, J. and Casa, D. and Upton, M. H. and Wong, D. and Schulz, C. and Bartkowiak, M. and Habicht, K. and Pomjakushina, E. and Cristiani, G. and Logvenov, G. and Minola, M. and Yamase, H. and Greco, A. and Keimer, B.},

  abstractNote = {We use resonant inelastic x-ray scattering (RIXS) at the O K- and Cu K-edges to investigate the doping dependence and temperature dependence of low-energy plasmon excitations in La2–xSrxCuO4. We observe a monotonic increase of the energy scale of the plasmons with increasing doping x in the underdoped regime, whereas a saturation occurs above optimal doping x ≳ 0.16 and persists at least up to x = 0.4. Furthermore, we find that the plasmon excitations show only a marginal temperature dependence, and possible effects due to the superconducting transition and the onset of strange metal behavior are either absent or below the detection limit of our experiment. Taking into account the strongly correlated character of the cuprates, we show that layered t – J – V model calculations accurately capture the increase of the plasmon energy in the underdoped regime. However, the computed plasmon energy continues to increase even for doping levels above x ≳ 0.16, which is distinct from the experimentally observed saturation and reaches a broad maximum around x = 0.55. We discuss whether possible lattice disorder in overdoped samples, a renormalization of the electronic correlation strength at high dopings, or an increasing relevance of nonplanar Cu and O orbitals could be responsible for the discrepancy between experiment and theory for doping levels above x = 0.16.},

  doi          = {10.1103/PhysRevB.107.214516},

  journal      = {Physical Review. B},

  number       = 21,

  volume       = 107,

  place        = {United States},

  year         = {Mon Jun 26 00:00:00 EDT 2023},

  month        = {Mon Jun 26 00:00:00 EDT 2023}

}

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Title: Evolution of plasmon excitations across the phase diagram of the cuprate superconductor La 2 − x Sr x CuO 4

Abstract

Citation Formats

Nonadiabatic and nonlocal electron-phonon interaction and phonon-plasmon mixing in the high-temperature superconductors journal, October 1994

Origin of the material dependence of T c in the single-layered cuprates journal, February 2012

Systematic evolution of temperature-dependent resistivity in La 2 − x Sr x CuO 4 journal, November 1992

Anomalous Criticality in the Electrical Resistivity of La2-xSrxCuO4 journal, January 2009

Imaging Doped Holes in a Cuprate Superconductor with High-Resolution Compton Scattering journal, April 2011

Hall coefficients and optical properties ofLa2−xSrxCuO4single-crystal thin films journal, February 1989

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Charge Excitations in Nd 2− x Ce x CuO 4 Observed with Resonant Inelastic X-ray Scattering: Comparison of Cu K -edge with Cu L 3 -edge journal, July 2019

Dispersion anomalies induced by the low-energy plasmon in the cuprates journal, January 2007

Superconductor-to-nonsuperconductor transition in ( La 1 − x Sr x ) 2 CuO 4 as investigated by transport and magnetic measurements journal, August 1989

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Low-energy plasmon excitations in infinite-layer nickelates journal, January 2023

Direct observation of orbital hybridisation in a cuprate superconductor journal, March 2018

Systematic derivation of a generalizedt-Jmodel journal, May 1994

Band-Structure Trend in Hole-Doped Cuprates and Correlation with T c max journal, July 2001

Resonant Inelastic X-Ray Scattering Study of Charge Excitations in L a 2 C u O 4 journal, October 2002

Design of Complex Oxide Interfaces by Oxide Molecular Beam Epitaxy journal, October 2019

Optical conductivity and superconductivity in highly overdoped La 2− x Ca x CuO 4 thin films journal, July 2021

Relevance of Cu – 3 d multiplet structure in models of high- T c cuprates journal, January 2020

Effective Hamiltonian for the superconducting Cu oxides journal, March 1988

Spatially modulated 'Mottness' in La2-xBaxCuO4 journal, December 2005

Magnetic, transport, and optical properties of monolayer copper oxides journal, July 1998

Unified theory of spin and charge excitations in high- Tc cuprate superconductors: A quantitative comparison with experiment and interpretation journal, July 2021

Acoustic plasmons and conducting carriers in hole-doped cuprate superconductors journal, June 2022

Renormalized band structure ofCuO2layers in superconducting compounds: A mean-field approach journal, October 1990

Scaling of the transition temperature of hole-doped cuprate superconductors with the charge-transfer energy journal, November 2012

Temperature-Dependent Ellipsometry Measurements of Partial Coulomb Energy in Superconducting Cuprates journal, August 2016

Effect of realistic out-of-plane dopant potentials on the superfluid density of overdoped cuprates journal, November 2022

Density and symmetry of unoccupied electronic states ofTl2Ba2CaCu2O8 journal, February 1990

Plasmons in cuprate superconductors journal, August 1990

Origin of high-energy charge excitations observed by resonant inelastic X-ray scattering in cuprate superconductors journal, January 2019

Optical conductivity of overdoped cuprate superconductors: Application to La 2 − x Sr x CuO 4 journal, August 2018

Electrodynamics of a layered electron gas. II. Periodic array journal, November 1974

Evidence for holes on oxygen sites in the high- T c superconductors La 2 − x Sr x CuO 4 and YBa 2 Cu 3 O 7 − y journal, April 1988

Layer plasmons and high- T c superconductivity journal, May 1988

Electronic collective modes and superconductivity in layered conductors journal, October 2003

Correlated electrons in high-temperature superconductors journal, July 1994

Non-Fermi-liquid states and pairing instability of a general model of copper oxide metals journal, June 1997

Probing the bulk plasmon continuum of layered materials through electron energy loss spectroscopy in a reflection geometry journal, October 2022

Phenomenology of the normal state of Cu-O high-temperature superconductors journal, October 1989

Many-Particle Physics book, January 1990

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Bimagnon studies in cuprates with resonant inelastic x-ray scattering at the O K edge. II. Doping effect in La 2 − x Sr x CuO 4 journal, June 2012

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Title: Evolution of plasmon excitations across the phase diagram of the cuprate superconductor ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$

Nonadiabatic and nonlocal electron-phonon interaction and phonon-plasmon mixing in the high-temperature superconductors
journal, October 1994

Origin of the material dependence of $T_{c}$ in the single-layered cuprates
journal, February 2012

Systematic evolution of temperature-dependent resistivity in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$
journal, November 1992

Anomalous Criticality in the Electrical Resistivity of La2-xSrxCuO4
journal, January 2009

Imaging Doped Holes in a Cuprate Superconductor with High-Resolution Compton Scattering
journal, April 2011

Hall coefficients and optical properties ofLa2−xSrxCuO4single-crystal thin films
journal, February 1989

Plasmon excitations in layered high- $T_{c}$ cuprates
journal, August 2016

Charge Excitations in Nd ₂₋ _x Ce _x CuO ₄ Observed with Resonant Inelastic X-ray Scattering: Comparison of Cu K -edge with Cu L ₃ -edge
journal, July 2019

Dispersion anomalies induced by the low-energy plasmon in the cuprates
journal, January 2007

Superconductor-to-nonsuperconductor transition in ( ${La}_{1 - x}$ ${Sr}_{x}$ $)_{2}$ ${CuO}_{4}$ as investigated by transport and magnetic measurements
journal, August 1989

Optical weights and waterfalls in doped charge-transfer insulators: A local density approximation and dynamical mean-field theory study of ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$
journal, October 2008

Low-energy plasmon excitations in infinite-layer nickelates
journal, January 2023

Direct observation of orbital hybridisation in a cuprate superconductor
journal, March 2018

Systematic derivation of a generalizedt-Jmodel
journal, May 1994

Band-Structure Trend in Hole-Doped Cuprates and Correlation with $T_{c \max}$
journal, July 2001

Resonant Inelastic X-Ray Scattering Study of Charge Excitations in $L a_{2} C u O_{4}$
journal, October 2002

Design of Complex Oxide Interfaces by Oxide Molecular Beam Epitaxy
journal, October 2019

Optical conductivity and superconductivity in highly overdoped La _{2− x} Ca _x CuO ₄ thin films
journal, July 2021

Relevance of $Cu - 3 d$ multiplet structure in models of high- $T_{c}$ cuprates
journal, January 2020

Effective Hamiltonian for the superconducting Cu oxides
journal, March 1988

Spatially modulated 'Mottness' in La2-xBaxCuO4
journal, December 2005

Magnetic, transport, and optical properties of monolayer copper oxides
journal, July 1998

Unified theory of spin and charge excitations in high- Tc cuprate superconductors: A quantitative comparison with experiment and interpretation
journal, July 2021

Acoustic plasmons and conducting carriers in hole-doped cuprate superconductors
journal, June 2022

Renormalized band structure ofCuO2layers in superconducting compounds: A mean-field approach
journal, October 1990

Scaling of the transition temperature of hole-doped cuprate superconductors with the charge-transfer energy
journal, November 2012

Temperature-Dependent Ellipsometry Measurements of Partial Coulomb Energy in Superconducting Cuprates
journal, August 2016

Effect of realistic out-of-plane dopant potentials on the superfluid density of overdoped cuprates
journal, November 2022

Density and symmetry of unoccupied electronic states ofTl2Ba2CaCu2O8
journal, February 1990

Plasmons in cuprate superconductors
journal, August 1990

Origin of high-energy charge excitations observed by resonant inelastic X-ray scattering in cuprate superconductors
journal, January 2019

Optical conductivity of overdoped cuprate superconductors: Application to ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$
journal, August 2018

Electrodynamics of a layered electron gas. II. Periodic array
journal, November 1974

Evidence for holes on oxygen sites in the high- $T_{c}$ superconductors ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$ and ${YBa}_{2}$ ${Cu}_{3}$ $O_{7 - y}$
journal, April 1988

Layer plasmons and high- $T_{c}$ superconductivity
journal, May 1988

Electronic collective modes and superconductivity in layered conductors
journal, October 2003

Correlated electrons in high-temperature superconductors
journal, July 1994

Non-Fermi-liquid states and pairing instability of a general model of copper oxide metals
journal, June 1997

Probing the bulk plasmon continuum of layered materials through electron energy loss spectroscopy in a reflection geometry
journal, October 2022

Phenomenology of the normal state of Cu-O high-temperature superconductors
journal, October 1989

Many-Particle Physics
book, January 1990

Bimagnon studies in cuprates with resonant inelastic x-ray scattering at the O $K$ edge. I. Assessment on La $_{2}$ CuO $_{4}$ and comparison with the excitation at Cu $L_{3}$ and Cu $K$ edges
journal, June 2012

Bimagnon studies in cuprates with resonant inelastic x-ray scattering at the O $K$ edge. II. Doping effect in La $_{2 - x}$ Sr $_{x}$ CuO $_{4}$
journal, June 2012

Two-Orbital Model Explains the Higher Transition Temperature of the Single-Layer Hg-Cuprate Superconductor Compared to That of the La-Cuprate Superconductor
journal, July 2010

Gapped Collective Charge Excitations and Interlayer Hopping in Cuprate Superconductors
journal, July 2022

Anisotropic Scattering Caused by Apical Oxygen Vacancies in Thin Films of Overdoped High-Temperature Cuprate Superconductors
journal, March 2022

Selective formation of apical oxygen vacancies in La2−xSrxCuO4
journal, October 2017

Doping a Mott insulator: Physics of high-temperature superconductivity
journal, January 2006

Anomalous attenuation of plasmons in strange metals and holography
journal, June 2019

Electronic states in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4 + δ}$ probed by soft-x-ray absorption
journal, January 1991

Close inspection of plasmon excitations in cuprate superconductors
journal, July 2020

A common thread: The pairing interaction for unconventional superconductors
journal, October 2012

Impact of dynamical screening on the phonon dynamics of metallic ${La}_{2} {CuO}_{4}$
journal, September 2009

The t – J model for the oxide high- T _c superconductors
journal, February 2008

Violation of the isotropic mean free path approximation for overdoped ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$
journal, June 2008

Three-dimensional collective charge excitations in electron-doped copper oxide superconductors
journal, October 2018

Apical oxygens and correlation strength in electron- and hole-doped copper oxides
journal, September 2010

Generalized plasma waves in layered superconductors: A unified approach
journal, May 2022

Symmetry of the3d9ligand hole induced by doping inYBa2Cu3O7−δ
journal, October 1988

Electronic correlations in solids, studied using electron energy-loss spectroscopy
journal, June 2001

Magnetic nature of the 500 meV peak in ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ observed with resonant inelastic x-ray scattering at the $Cu K$ -edge
journal, February 2010

Renormalization from density-functional theory to strong-coupling models for electronic states in Cu-O materials
journal, June 1990

Differences between the insulating limit quasiparticles of one-band and three-band cuprate models
journal, February 2016

Plasma Frequency of the Electron Gas in Layered Structures
journal, September 1973

Resonant inelastic x-ray scattering studies of elementary excitations
journal, June 2011

Self-consistent field approximation for the plasma frequencies of an electron gas in a layered thin film
journal, August 1975

Spin -Resolved Photoemission on Anti -Ferromagnets: Direct Observation of Zhang-Rice Singlets in CuO
journal, February 1997

Ab Initio determination of Cu 3d orbital energies in layered copper oxides
journal, August 2011

Detection of Acoustic Plasmons in Hole-Doped Lanthanum and Bismuth Cuprate Superconductors Using Resonant Inelastic X-Ray Scattering
journal, December 2020

Persistence of magnetic excitations in La2−xSrxCuO4 from the undoped insulator to the heavily overdoped non-superconducting metal
journal, August 2013

Extremely Overdoped Superconducting Cuprates via High Pressure Oxygenation Methods
journal, December 2021

Atomic-resolution two-dimensional mapping of holes in the cuprate superconductor La2−xSrxCuO4±δ
journal, May 2018

Charge-density waves and superconductivity as an alternative to phase separation in the infinite- U Hubbard-Holstein model
journal, November 1996

Electronic Phase Diagram of High- $T_{c}$ Cuprate Superconductors from a Mapping of the In-Plane Resistivity Curvature
journal, December 2004

Theory of high- $T_{c}$ superconductivity in oxides
journal, June 1987

Uncovering selective excitations using the resonant profile of indirect inelastic x-ray scattering in correlated materials: observing two-magnon scattering and relation to the dynamical structure factor
journal, November 2012

Orbital character of states at the Fermi level in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$ and $R_{2 - x}$ ${Ce}_{x}$ ${CuO}_{4}$ ( R =Nd,Sm)
journal, February 1993

Mott Gap Excitations in Twin-FreeYBa2Cu3O7−δ(Tc=93 K) Studied by Resonant Inelastic X-Ray Scattering
journal, May 2005

Progress and perspectives on electron-doped cuprates
journal, September 2010