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Title: Doping evolution of the second magnetization peak and magnetic relaxation in ( B a 1 - x K x ) F e 2 A s 2 single crystals

Here, we present a thorough study of doping dependent magnetic hysteresis and relaxation characteristics in single crystals of (Ba 1-xK x) Fe 2As 2 (0.18 ≤ x ≤ 1). The critical current density J c reaches maximum in the underdoped sample x = 0.26 and then decreases in the optimally doped and overdoped samples. Meanwhile, the magnetic relaxation rate S rapidly increases and the flux creep activation barrier U 0 sharply decreases in the overdoped sample x = 0.70. These results suggest that vortex pinning is very strong in the underdoped regime, but it is greatly reduced in the optimally doped and overdoped regime. Transmission electron microscope (TEM) measurements reveal the existence of dislocations and inclusions in all three studied samples x = 0.38, 0.46, and 0.65. An investigation of the paramagnetic Meissner effect (PME) suggests that spatial variations in T c become small in the samples x = 0.43 and 0.46, slightly above the optimal doping levels. Our results support that two types of pinning sources dominate the (Ba 1-xK x) Fe 2As 2 crystals: (i) strong δl pinning, which results from the fluctuations in the mean free path l and δT c pinning from the spatial variations inmore » T c in the underdoped regime, and (ii) weak δT c pinning in the optimally doped and overdoped regime.« less
Authors:
 [1] ;  [1] ;  [1] ;  [1] ;  [2] ;  [2] ;  [3]
  1. Ames Lab., Ames, IA (United States). Division of Materials Sciences and Engineering
  2. Ames Lab. and Iowa State Univ., Ames, IA (United States). Division of Materials Sciences and Engineering and Dept. of Physics and Astronomy
  3. Ames Lab. and Iowa State Univ., Ames, IA (United States). Dept. of Materials Science and Engineering
Publication Date:
Report Number(s):
IS-J-9358
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1801652
Grant/Contract Number:
AC02-07CH11358
Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 97; Journal Issue: 5; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Research Org:
Ames Laboratory (AMES), Ames, IA (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE
OSTI Identifier:
1422753
Alternate Identifier(s):
OSTI ID: 1421577