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Oxide– and Silicate–Water Interfaces and Their Roles in Technology and the Environment
Abstract
Interfacial reactions drive all elemental cycling on Earth and play a pivotal role in human life such as agriculture, water purification, energy production, environmental contaminant remediation, and nuclear waste repository management. Chemistry at such interfaces has been a focus of research for several decades, with the most recent comprehensive review published in 1999 (Brown et al., Chemical Reviews). Here we critically review research advances on structure, reactivity, and dynamic and coupled processes at oxide- and silicate-water interfaces in the last 20+ years and discuss the future opportunities. First, since the onset of the 21st century, strides towards a detailed understanding of interfaces submerged in aqueous solutions have been enabled by the development techniques with near-atomic measurement resolution utilizing tunable highflux focused ultrafast laser and X-ray sources, as well as nano-fabrication approaches that enable transmission electron microscopy in a liquid cell. This leap into atomic- and nm-scale measurements uncovered scale-dependent chemical phenomena, with reaction thermodynamics, kinetics, and pathways deviating from previous observations made on the larger systems. The second key advance is new experimental evidence for what scientists have hypothesized but could not test previously: namely that interfacial chemical reactions are frequently driven by “anomalies”, or “non-idealities” - such as defects,more »
- Authors:
-
more »
- Univ. of Texas at El Paso, TX (United States)
- Temple Univ., Philadelphia, PA (United States)
- Stanford Univ., CA (United States)
- Texas A & M Univ., College Station, TX (United States)
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Virginia Polytechnic Inst. and State Univ. (Virginia Tech), Blacksburg, VA (United States)
- Univ. Paris-Saclay, Evry-Courcouronnes (France)
- Northwestern Univ., Evanston, IL (United States)
- Univ. of Alberta, Edmonton, AB (Canada)
- Univ. of California, San Diego, CA (United States)
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Washington Univ., St. Louis, MO (United States)
- Georgia State Univ., Atlanta, GA (United States)
- Univ. of Texas, Austin, TX (United States)
- Karlsruhe Inst. of Technology (KIT) (Germany)
- University of Münster (Germany)
- Rutgers Univ., Piscataway, NJ (United States)
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Ruhr Univ., Bochum (Germany)
- Univ. Nacional Autonoma de Mexico (UNAM), Mexico City (Mexico)
- Case Western Reserve Univ., Cleveland, OH (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division (CSGB); USDOE National Nuclear Security Administration (NNSA); National Science Foundation (NSF); American Chemical Society; US Army Research Office (ARO); US Army Research Laboratory (USARL)
- OSTI Identifier:
- 1975377
- Alternate Identifier(s):
- OSTI ID: 1985975
- Report Number(s):
- PNNL-SA-169484
Journal ID: ISSN 0009-2665
- Grant/Contract Number:
- AC05-00OR22725; FG02-00ER15112; SC0012186; SC0023390; NA0003525; CHE-1905077; 62756-ND5; W911NF-19-1-0078; 21-015452; FWP #56674; AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Chemical Reviews
- Additional Journal Information:
- Journal Volume: 123; Journal Issue: 10; Journal ID: ISSN 0009-2665
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; Interfaces; Layers; Minerals; Nanoparticles; Oxides
Citation Formats
Bañuelos, José Leobardo, Borguet, Eric, Brown, Gordon E., Cygan, Randall T., DeYoreo, James J., Dove, Patricia M., Gaigeot, Marie-Pierre, Geiger, Franz M., Gibbs, Julianne M., Grassian, Vicki H., Ilgen, Anastasia G., Jun, Young-Shin, Kabengi, Nadine, Katz, Lynn, Kubicki, James D., Lützenkirchen, Johannes, Putnis, Christine V., Remsing, Richard C., Rosso, Kevin M., Rother, Gernot, Sulpizi, Marialore, Villalobos, Mario, and Zhang, Huichun. Oxide– and Silicate–Water Interfaces and Their Roles in Technology and the Environment. United States: N. p., 2023.
Web. doi:10.1021/acs.chemrev.2c00130.
Bañuelos, José Leobardo, Borguet, Eric, Brown, Gordon E., Cygan, Randall T., DeYoreo, James J., Dove, Patricia M., Gaigeot, Marie-Pierre, Geiger, Franz M., Gibbs, Julianne M., Grassian, Vicki H., Ilgen, Anastasia G., Jun, Young-Shin, Kabengi, Nadine, Katz, Lynn, Kubicki, James D., Lützenkirchen, Johannes, Putnis, Christine V., Remsing, Richard C., Rosso, Kevin M., Rother, Gernot, Sulpizi, Marialore, Villalobos, Mario, & Zhang, Huichun. Oxide– and Silicate–Water Interfaces and Their Roles in Technology and the Environment. United States. https://doi.org/10.1021/acs.chemrev.2c00130
Bañuelos, José Leobardo, Borguet, Eric, Brown, Gordon E., Cygan, Randall T., DeYoreo, James J., Dove, Patricia M., Gaigeot, Marie-Pierre, Geiger, Franz M., Gibbs, Julianne M., Grassian, Vicki H., Ilgen, Anastasia G., Jun, Young-Shin, Kabengi, Nadine, Katz, Lynn, Kubicki, James D., Lützenkirchen, Johannes, Putnis, Christine V., Remsing, Richard C., Rosso, Kevin M., Rother, Gernot, Sulpizi, Marialore, Villalobos, Mario, and Zhang, Huichun. Mon .
"Oxide– and Silicate–Water Interfaces and Their Roles in Technology and the Environment". United States. https://doi.org/10.1021/acs.chemrev.2c00130.
@article{osti_1975377,
title = {Oxide– and Silicate–Water Interfaces and Their Roles in Technology and the Environment},
author = {Bañuelos, José Leobardo and Borguet, Eric and Brown, Gordon E. and Cygan, Randall T. and DeYoreo, James J. and Dove, Patricia M. and Gaigeot, Marie-Pierre and Geiger, Franz M. and Gibbs, Julianne M. and Grassian, Vicki H. and Ilgen, Anastasia G. and Jun, Young-Shin and Kabengi, Nadine and Katz, Lynn and Kubicki, James D. and Lützenkirchen, Johannes and Putnis, Christine V. and Remsing, Richard C. and Rosso, Kevin M. and Rother, Gernot and Sulpizi, Marialore and Villalobos, Mario and Zhang, Huichun},
abstractNote = {Interfacial reactions drive all elemental cycling on Earth and play a pivotal role in human life such as agriculture, water purification, energy production, environmental contaminant remediation, and nuclear waste repository management. Chemistry at such interfaces has been a focus of research for several decades, with the most recent comprehensive review published in 1999 (Brown et al., Chemical Reviews). Here we critically review research advances on structure, reactivity, and dynamic and coupled processes at oxide- and silicate-water interfaces in the last 20+ years and discuss the future opportunities. First, since the onset of the 21st century, strides towards a detailed understanding of interfaces submerged in aqueous solutions have been enabled by the development techniques with near-atomic measurement resolution utilizing tunable highflux focused ultrafast laser and X-ray sources, as well as nano-fabrication approaches that enable transmission electron microscopy in a liquid cell. This leap into atomic- and nm-scale measurements uncovered scale-dependent chemical phenomena, with reaction thermodynamics, kinetics, and pathways deviating from previous observations made on the larger systems. The second key advance is new experimental evidence for what scientists have hypothesized but could not test previously: namely that interfacial chemical reactions are frequently driven by “anomalies”, or “non-idealities” - such as defects, nanoconfinement, and unanticipated chemical structures. Third, advances in computational chemistry have allowed insight to move beyond simple schematics and gain a molecular model of these complex interfaces. These advances were facilitated by our ability to simulate with greater accuracy systems in concert with their corresponding high-resolution experimental observations. In combination with surface-sensitive measurements, we have gained knowledge of the interfacial structure and dynamics, including the underlying oxide surface and the immediately adjacent water and aqueous ions, which enable us to better define what constitutes the oxide-water interface. This critical review discusses how science is progressing from understanding the ideal oxide- and silicate-water interfaces to more realistic systems, focusing on accomplishments in the last 20 years, and identifying the remaining unknowns, outstanding challenges, and future opportunities for the community to address and/or to seek in the decades to come. We anticipate that the next 20 years will focus on understanding and predicting dynamic transient and reactive structures over greater spatial and temporal ranges as well as systems of greater structural and chemical complexity. Closer collaborations of theoretical and experimental experts across disciplines are critical to achieving this great aspiration.},
doi = {10.1021/acs.chemrev.2c00130},
journal = {Chemical Reviews},
number = 10,
volume = 123,
place = {United States},
year = {Mon May 15 00:00:00 EDT 2023},
month = {Mon May 15 00:00:00 EDT 2023}
}
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