Multimodal (Non)Linear Optical Nanoimaging and Nanospectroscopy
Abstract
This article highlights recent advances in linear and nonlinear spectral nanoimaging. The described developments are motivated by the need to characterize molecular and material systems noninvasively with nanometer spatial and femtosecond temporal resolution. Indeed, the ability to image and chemically characterize heterogeneous interfaces with joint nano–femto resolution is a prerequisite to advancing our fundamental understanding of processes as diverse as heterogeneous catalysis, microbial communication, and energy flow in pristine/defect-containing low-dimensional quantum materials, to name a few. We describe pioneering work and recent demonstrations of (non)linear optical nanoimaging and nanospectroscopy, with an emphasis on high spatial resolution measurements conducted under ambient laboratory conditions.
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE Laboratory Directed Research and Development (LDRD) Program
- OSTI Identifier:
- 1916456
- Report Number(s):
- PNNL-SA-174591
Journal ID: ISSN 1948-7185
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Physical Chemistry Letters
- Additional Journal Information:
- Journal Volume: 13; Journal Issue: 31; Journal ID: ISSN 1948-7185
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; Light; Nanocubes; Plasmonics; Probes; Raman spectroscopy
Citation Formats
Wang, Chih-Feng, and El-Khoury, Patrick Z. Multimodal (Non)Linear Optical Nanoimaging and Nanospectroscopy. United States: N. p., 2022.
Web. doi:10.1021/acs.jpclett.2c01993.
Wang, Chih-Feng, & El-Khoury, Patrick Z. Multimodal (Non)Linear Optical Nanoimaging and Nanospectroscopy. United States. https://doi.org/10.1021/acs.jpclett.2c01993
Wang, Chih-Feng, and El-Khoury, Patrick Z. Wed .
"Multimodal (Non)Linear Optical Nanoimaging and Nanospectroscopy". United States. https://doi.org/10.1021/acs.jpclett.2c01993. https://www.osti.gov/servlets/purl/1916456.
@article{osti_1916456,
title = {Multimodal (Non)Linear Optical Nanoimaging and Nanospectroscopy},
author = {Wang, Chih-Feng and El-Khoury, Patrick Z.},
abstractNote = {This article highlights recent advances in linear and nonlinear spectral nanoimaging. The described developments are motivated by the need to characterize molecular and material systems noninvasively with nanometer spatial and femtosecond temporal resolution. Indeed, the ability to image and chemically characterize heterogeneous interfaces with joint nano–femto resolution is a prerequisite to advancing our fundamental understanding of processes as diverse as heterogeneous catalysis, microbial communication, and energy flow in pristine/defect-containing low-dimensional quantum materials, to name a few. We describe pioneering work and recent demonstrations of (non)linear optical nanoimaging and nanospectroscopy, with an emphasis on high spatial resolution measurements conducted under ambient laboratory conditions.},
doi = {10.1021/acs.jpclett.2c01993},
journal = {Journal of Physical Chemistry Letters},
number = 31,
volume = 13,
place = {United States},
year = {Wed Aug 03 00:00:00 EDT 2022},
month = {Wed Aug 03 00:00:00 EDT 2022}
}
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