Molecular-Modified Photocathodes for Applications in Artificial Photosynthesis and Solar-to-Fuel Technologies
Abstract
Nature offers inspiration for developing technologies that integrate the capture, conversion, and storage of solar energy. In this review article, we highlight principles of natural photosynthesis and artificial photosynthesis, drawing comparisons between solar energy transduction in biology and emerging solar-to-fuel technologies. Key features of the biological approach include use of earth-abundant elements and molecular interfaces for driving photoinduced charge separation reactions that power chemical transformations at global scales. Finally, for the artificial systems described in this review, emphasis is placed on advancements involving hybrid photocathodes that power fuel-forming reactions using molecular catalysts interfaced with visible-light-absorbing semiconductors.
- Authors:
-
- Arizona State Univ., Tempe, AZ (United States)
- Publication Date:
- Research Org.:
- Arizona State Univ., Tempe, AZ (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); Heiwa Nakajima Foundation; ARCS Foundation
- OSTI Identifier:
- 1906921
- Grant/Contract Number:
- SC0021186
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Chemical Reviews
- Additional Journal Information:
- Journal Volume: 122; Journal Issue: 21; Journal ID: ISSN 0009-2665
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; catalysts; charge transfer; electrical properties; electrodes; semiconductors
Citation Formats
Reyes Cruz, Edgar A., Nishiori, Daiki, Wadsworth, Brian L., Nguyen, Nghi P., Hensleigh, Lillian K., Khusnutdinova, Diana, Beiler, Anna M., and Moore, G. F. Molecular-Modified Photocathodes for Applications in Artificial Photosynthesis and Solar-to-Fuel Technologies. United States: N. p., 2022.
Web. doi:10.1021/acs.chemrev.2c00200.
Reyes Cruz, Edgar A., Nishiori, Daiki, Wadsworth, Brian L., Nguyen, Nghi P., Hensleigh, Lillian K., Khusnutdinova, Diana, Beiler, Anna M., & Moore, G. F. Molecular-Modified Photocathodes for Applications in Artificial Photosynthesis and Solar-to-Fuel Technologies. United States. https://doi.org/10.1021/acs.chemrev.2c00200
Reyes Cruz, Edgar A., Nishiori, Daiki, Wadsworth, Brian L., Nguyen, Nghi P., Hensleigh, Lillian K., Khusnutdinova, Diana, Beiler, Anna M., and Moore, G. F. Thu .
"Molecular-Modified Photocathodes for Applications in Artificial Photosynthesis and Solar-to-Fuel Technologies". United States. https://doi.org/10.1021/acs.chemrev.2c00200. https://www.osti.gov/servlets/purl/1906921.
@article{osti_1906921,
title = {Molecular-Modified Photocathodes for Applications in Artificial Photosynthesis and Solar-to-Fuel Technologies},
author = {Reyes Cruz, Edgar A. and Nishiori, Daiki and Wadsworth, Brian L. and Nguyen, Nghi P. and Hensleigh, Lillian K. and Khusnutdinova, Diana and Beiler, Anna M. and Moore, G. F.},
abstractNote = {Nature offers inspiration for developing technologies that integrate the capture, conversion, and storage of solar energy. In this review article, we highlight principles of natural photosynthesis and artificial photosynthesis, drawing comparisons between solar energy transduction in biology and emerging solar-to-fuel technologies. Key features of the biological approach include use of earth-abundant elements and molecular interfaces for driving photoinduced charge separation reactions that power chemical transformations at global scales. Finally, for the artificial systems described in this review, emphasis is placed on advancements involving hybrid photocathodes that power fuel-forming reactions using molecular catalysts interfaced with visible-light-absorbing semiconductors.},
doi = {10.1021/acs.chemrev.2c00200},
journal = {Chemical Reviews},
number = 21,
volume = 122,
place = {United States},
year = {Thu Sep 29 00:00:00 EDT 2022},
month = {Thu Sep 29 00:00:00 EDT 2022}
}
Figures / Tables:
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