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Title: The Magnetic Genome of Two-Dimensional van der Waals Materials

Abstract

Magnetism in two-dimensional (2D) van der Waals (vdW) materials has recently emerged as one of the most promising areas in condensed matter research, with many exciting emerging properties and significant potential for applications ranging from topological magnonics to low-power spintronics, quantum computing, and optical communications. In the brief time after their discovery, 2D magnets have blossomed into a rich area for investigation, where fundamental concepts in magnetism are challenged by the behavior of spins that can develop at the single layer limit. However, much effort is still needed in multiple fronts before 2D magnets can be routinely used for practical implementations. In this comprehensive review, prominent authors with expertise in complementary fields of 2D magnetism (i.e., synthesis, device engineering, magneto-optics, imaging, transport, mechanics, spin excitations, and theory and simulations) have joined together to provide a genome of current knowledge and a guideline for future developments in 2D magnetic materials research.

Authors:
ORCiD logo [1]; ORCiD logo [2];  [1];  [3];  [4];  [5]; ORCiD logo [6]; ORCiD logo [7];  [8];  [9];  [10];  [11];  [12];  [13]; ORCiD logo [14];  [14];  [15]; ORCiD logo [16];  [17]; ORCiD logo [18] more »; ORCiD logo [19]; ORCiD logo [7]; ORCiD logo [20]; ORCiD logo [21]; ORCiD logo [22]; ORCiD logo [23];  [23];  [24]; ORCiD logo [3]; ORCiD logo [1];  [19];  [25];  [26];  [27];  [28];  [29];  [6];  [30]; ORCiD logo [31]; ORCiD logo [32] « less
  1. Materials Science and Engineering, School for Engineering of Matter, Transport and Energy, Arizona State University, Tempe, Arizona 85287, United States
  2. NISE Department, Max Planck Institute of Microstructure Physics, 06120 Halle, Germany, Instituto de Ciencia Molecular (ICMol), Universitat de València, 46980 Paterna, Spain
  3. Department of Chemistry, Columbia University, New York, New York 10027, United States
  4. Department of Physics, Harvard University, Cambridge, Massachusetts 02138, United States
  5. Twist Group, Faculty of Physics, University of Duisburg-Essen, Campus Duisburg, 47057 Duisburg, Germany
  6. Institute for Functional Intelligent Materials, National University of Singapore, 117544 Singapore
  7. Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, United States
  8. Physikalisches Institut, University of Stuttgart, 70569 Stuttgart, Germany
  9. Department of Chemistry, Columbia University, New York, New York 10027, United States, Department of Physics, Columbia University, New York, New York 10027, United States
  10. School of Materials Science and Engineering, Department of Energy Engineering Convergence, Kumoh National Institute of Technology, Gumi 39177, Korea
  11. Institute for Condensed Matter Physics and Complex Systems, School of Physics and Astronomy, The University of Edinburgh, Edinburgh, EH9 3FD, United Kingdom, Donostia International Physics Center (DIPC), 20018 Donostia-San Sebastián, Basque Country, Spain
  12. Department of Physics, Harvard University, Cambridge, Massachusetts 02138, United States, John Harvard Distinguished Science Fellows Program, Harvard University, Cambridge, Massachusetts 02138, United States
  13. Laboratory for Topological Quantum Matter and Spectroscopy, Department of Physics, Princeton University, Princeton, New Jersey 08544, United States
  14. Institute for Frontier Materials, Deakin University, Geelong Waurn Ponds Campus, Waurn Ponds, Victoria 3216, Australia
  15. Department of Physics, Columbia University, New York, New York 10027, United States
  16. CIC nanoGUNE BRTA, 20018 Donostia - San Sebastián, Basque Country, Spain, IKERBASQUE, Basque Foundation for Science, 48013 Bilbao, Basque Country, Spain
  17. Department of Physics, University of York, Heslington, York YO10 5DD, United Kingdom
  18. Université Grenoble Alpes, CEA, CNRS, Spintec, 38000 Grenoble, France, Institut Universitaire de France, 75231 Paris, France
  19. Department of Physics and Astronomy, University of Manchester, Manchester, M13 9PL, United Kingdom, National Graphene Institute, University of Manchester, Manchester, M13 9PL, United Kingdom
  20. Department of Electrical and Computer Engineering, Texas Tech University, 910 Boston Avenue, Lubbock, Texas 79409, United States
  21. Department of Physics, University of Michigan, 450 Church Street, Ann Arbor, Michigan 48109, United States
  22. Institute for Quantum Computing and Department of Chemistry, University of Waterloo, Waterloo, Ontario N2L 3G1, Canada
  23. SUPA, Institute of Photonics and Quantum Sciences, Heriot-Watt University, Edinburgh EH14 4AS, United Kingdom
  24. Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland
  25. Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States, Princeton Institute for Science and Technology of Materials, Princeton University, Princeton, New Jersey 08544, United States, National High Magnetic Field Laboratory, Florida State University, Tallahassee, Florida 32310, United States
  26. Physikalisches Institut, University of Stuttgart, 70569 Stuttgart, Germany, Max Planck Institute for Solid State Research, 70569 Stuttgart, Germany
  27. Department of Physics, Harvard University, Cambridge, Massachusetts 02138, United States, John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts 02138, United States
  28. Donostia International Physics Center (DIPC), 20018 Donostia-San Sebastián, Basque Country, Spain, Unité Mixte de Physique, CNRS, Thales, Université Paris-Saclay, 91767 Palaiseau, France, Department of Materials Physics UPV/EHU, 20018 Donostia - San Sebastián, Basque Country, Spain
  29. NISE Department, Max Planck Institute of Microstructure Physics, 06120 Halle, Germany
  30. Department of Physics and Astronomy, Rice University, Houston, Texas 77005, United States
  31. National High Magnetic Field Laboratory, Florida State University, Tallahassee, Florida 32310, United States, Department of Physics, Florida State University, Tallahassee, Florida 32306, United States
  32. Institute for Condensed Matter Physics and Complex Systems, School of Physics and Astronomy, The University of Edinburgh, Edinburgh, EH9 3FD, United Kingdom, Donostia International Physics Center (DIPC), 20018 Donostia-San Sebastián, Basque Country, Spain, Higgs Centre for Theoretical Physics, The University of Edinburgh, Edinburgh EH9 3FD, United Kingdom
Publication Date:
Research Org.:
Brookhaven National Laboratory (BNL), Upton, NY (United States); Florida State Univ., Tallahassee, FL (United States); Arizona State Univ., Tempe, AZ (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; US Army Research Office (ARO); US Air Force Office of Scientific Research (AFOSR); National Science Foundation (NSF); Engineering and Physical Sciences Research Council (EPSRC); National Research Foundation of Korea (NRF); Swiss National Science Foundation (SNSF); European Union Horizon 2020; French National Research Agency (ANR); Welch Foundation; Ministry of Education Singapore
OSTI Identifier:
1864055
Alternate Identifier(s):
OSTI ID: 1871296; OSTI ID: 1893761; OSTI ID: 1958292
Report Number(s):
BNL-223586-2022-JAAM
Journal ID: ISSN 1936-0851
Grant/Contract Number:  
SC0002613; SC0012704; SC0019443; DOE-SC0020653; SC0020653; W911NF-17-1-0023; FA9550- 21-1-0065; FA9550-18-1-0020; ECCS-2052527; DMR-1231319; DMR-1420634; DMR-174774; DMR-1904716; DMR-1906030; DMR-2011738; DMR-2100741; DMR-2111812; EP/N007131/1; EP/P029892/1; EP/T021578/1; IEC/R2/192001; URF/R1/211484; C-1839; ANR-18-CE24-0007; QLCI-CG-1936882; RTI2018094861-B-100; P2ZHP2-161980; P300P2-177832; GBMF 9468; EDUN C-33-18-279-V12, I-FIM; NRF-2021R1C1C1012394; 320163632/EV 196/2; FOR 2724; GRK 2642; 820394; AC02-05CH11231
Resource Type:
Published Article
Journal Name:
ACS Nano
Additional Journal Information:
Journal Name: ACS Nano Journal Volume: 16 Journal Issue: 5; Journal ID: ISSN 1936-0851
Publisher:
American Chemical Society
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE; magnetic properties; monolayers; order; quantum mechanics; theoretical models

Citation Formats

Wang, Qing Hua, Bedoya-Pinto, Amilcar, Blei, Mark, Dismukes, Avalon H., Hamo, Assaf, Jenkins, Sarah, Koperski, Maciej, Liu, Yu, Sun, Qi-Chao, Telford, Evan J., Kim, Hyun Ho, Augustin, Mathias, Vool, Uri, Yin, Jia-Xin, Li, Lu Hua, Falin, Alexey, Dean, Cory R., Casanova, Fèlix, Evans, Richard F. L., Chshiev, Mairbek, Mishchenko, Artem, Petrovic, Cedomir, He, Rui, Zhao, Liuyan, Tsen, Adam W., Gerardot, Brian D., Brotons-Gisbert, Mauro, Guguchia, Zurab, Roy, Xavier, Tongay, Sefaattin, Wang, Ziwei, Hasan, M. Zahid, Wrachtrup, Joerg, Yacoby, Amir, Fert, Albert, Parkin, Stuart, Novoselov, Kostya S., Dai, Pengcheng, Balicas, Luis, and Santos, Elton J. G. The Magnetic Genome of Two-Dimensional van der Waals Materials. United States: N. p., 2022. Web. doi:10.1021/acsnano.1c09150.
Wang, Qing Hua, Bedoya-Pinto, Amilcar, Blei, Mark, Dismukes, Avalon H., Hamo, Assaf, Jenkins, Sarah, Koperski, Maciej, Liu, Yu, Sun, Qi-Chao, Telford, Evan J., Kim, Hyun Ho, Augustin, Mathias, Vool, Uri, Yin, Jia-Xin, Li, Lu Hua, Falin, Alexey, Dean, Cory R., Casanova, Fèlix, Evans, Richard F. L., Chshiev, Mairbek, Mishchenko, Artem, Petrovic, Cedomir, He, Rui, Zhao, Liuyan, Tsen, Adam W., Gerardot, Brian D., Brotons-Gisbert, Mauro, Guguchia, Zurab, Roy, Xavier, Tongay, Sefaattin, Wang, Ziwei, Hasan, M. Zahid, Wrachtrup, Joerg, Yacoby, Amir, Fert, Albert, Parkin, Stuart, Novoselov, Kostya S., Dai, Pengcheng, Balicas, Luis, & Santos, Elton J. G. The Magnetic Genome of Two-Dimensional van der Waals Materials. United States. https://doi.org/10.1021/acsnano.1c09150
Wang, Qing Hua, Bedoya-Pinto, Amilcar, Blei, Mark, Dismukes, Avalon H., Hamo, Assaf, Jenkins, Sarah, Koperski, Maciej, Liu, Yu, Sun, Qi-Chao, Telford, Evan J., Kim, Hyun Ho, Augustin, Mathias, Vool, Uri, Yin, Jia-Xin, Li, Lu Hua, Falin, Alexey, Dean, Cory R., Casanova, Fèlix, Evans, Richard F. L., Chshiev, Mairbek, Mishchenko, Artem, Petrovic, Cedomir, He, Rui, Zhao, Liuyan, Tsen, Adam W., Gerardot, Brian D., Brotons-Gisbert, Mauro, Guguchia, Zurab, Roy, Xavier, Tongay, Sefaattin, Wang, Ziwei, Hasan, M. Zahid, Wrachtrup, Joerg, Yacoby, Amir, Fert, Albert, Parkin, Stuart, Novoselov, Kostya S., Dai, Pengcheng, Balicas, Luis, and Santos, Elton J. G. Wed . "The Magnetic Genome of Two-Dimensional van der Waals Materials". United States. https://doi.org/10.1021/acsnano.1c09150.
@article{osti_1864055,
title = {The Magnetic Genome of Two-Dimensional van der Waals Materials},
author = {Wang, Qing Hua and Bedoya-Pinto, Amilcar and Blei, Mark and Dismukes, Avalon H. and Hamo, Assaf and Jenkins, Sarah and Koperski, Maciej and Liu, Yu and Sun, Qi-Chao and Telford, Evan J. and Kim, Hyun Ho and Augustin, Mathias and Vool, Uri and Yin, Jia-Xin and Li, Lu Hua and Falin, Alexey and Dean, Cory R. and Casanova, Fèlix and Evans, Richard F. L. and Chshiev, Mairbek and Mishchenko, Artem and Petrovic, Cedomir and He, Rui and Zhao, Liuyan and Tsen, Adam W. and Gerardot, Brian D. and Brotons-Gisbert, Mauro and Guguchia, Zurab and Roy, Xavier and Tongay, Sefaattin and Wang, Ziwei and Hasan, M. Zahid and Wrachtrup, Joerg and Yacoby, Amir and Fert, Albert and Parkin, Stuart and Novoselov, Kostya S. and Dai, Pengcheng and Balicas, Luis and Santos, Elton J. G.},
abstractNote = {Magnetism in two-dimensional (2D) van der Waals (vdW) materials has recently emerged as one of the most promising areas in condensed matter research, with many exciting emerging properties and significant potential for applications ranging from topological magnonics to low-power spintronics, quantum computing, and optical communications. In the brief time after their discovery, 2D magnets have blossomed into a rich area for investigation, where fundamental concepts in magnetism are challenged by the behavior of spins that can develop at the single layer limit. However, much effort is still needed in multiple fronts before 2D magnets can be routinely used for practical implementations. In this comprehensive review, prominent authors with expertise in complementary fields of 2D magnetism (i.e., synthesis, device engineering, magneto-optics, imaging, transport, mechanics, spin excitations, and theory and simulations) have joined together to provide a genome of current knowledge and a guideline for future developments in 2D magnetic materials research.},
doi = {10.1021/acsnano.1c09150},
journal = {ACS Nano},
number = 5,
volume = 16,
place = {United States},
year = {Wed Apr 20 00:00:00 EDT 2022},
month = {Wed Apr 20 00:00:00 EDT 2022}
}

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https://doi.org/10.1021/acsnano.1c09150

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