Designer Nanomaterials through Programmable Assembly
Abstract
Nanoparticles have long been recognized for their unique properties, leading to exciting potential applications across optics, electronics, magnetism, and catalysis. These specific functions often require a designed organization of particles, which includes the type of order as well as placement and relative orientation of particles of the same or different kinds. DNA nanotechnology offers the ability to introduce highly addressable bonds, tailor particle interactions, and control the geometry of bindings motifs. Here, we discuss how developments in structural DNA nanotechnology have enabled greater control over 1D, 2D, and 3D particle organizations through programmable assembly. This Review focuses on how the use of DNA binding between nanocomponents and DNA structural motifs has progressively allowed the rational formation of prescribed particle organizations. Here, we offer insight into how DNA-based motifs and elements can be further developed to control particle organizations and how particles and DNA can be integrated into nanoscale building blocks, so-called “material voxels”, to realize designer nanomaterials with desired functions.
- Authors:
-
- Columbia Univ., New York, NY (United States); Brookhaven National Lab. (BNL), Upton, NY (United States)
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1854500
- Report Number(s):
- BNL-222832-2022-JAAM
Journal ID: ISSN 0044-8249
- Grant/Contract Number:
- SC0012704; SC0008772
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Angewandte Chemie
- Additional Journal Information:
- Journal Volume: 134; Journal Issue: 3; Journal ID: ISSN 0044-8249
- Publisher:
- German Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; DNA-based nanomaterials; crystal engineering; designed nanomaterials; DNA structures; nanoparticles; self-assembly
Citation Formats
Kahn, Jason S., and Gang, Oleg. Designer Nanomaterials through Programmable Assembly. United States: N. p., 2021.
Web. doi:10.1002/ange.202105678.
Kahn, Jason S., & Gang, Oleg. Designer Nanomaterials through Programmable Assembly. United States. https://doi.org/10.1002/ange.202105678
Kahn, Jason S., and Gang, Oleg. Mon .
"Designer Nanomaterials through Programmable Assembly". United States. https://doi.org/10.1002/ange.202105678. https://www.osti.gov/servlets/purl/1854500.
@article{osti_1854500,
title = {Designer Nanomaterials through Programmable Assembly},
author = {Kahn, Jason S. and Gang, Oleg},
abstractNote = {Nanoparticles have long been recognized for their unique properties, leading to exciting potential applications across optics, electronics, magnetism, and catalysis. These specific functions often require a designed organization of particles, which includes the type of order as well as placement and relative orientation of particles of the same or different kinds. DNA nanotechnology offers the ability to introduce highly addressable bonds, tailor particle interactions, and control the geometry of bindings motifs. Here, we discuss how developments in structural DNA nanotechnology have enabled greater control over 1D, 2D, and 3D particle organizations through programmable assembly. This Review focuses on how the use of DNA binding between nanocomponents and DNA structural motifs has progressively allowed the rational formation of prescribed particle organizations. Here, we offer insight into how DNA-based motifs and elements can be further developed to control particle organizations and how particles and DNA can be integrated into nanoscale building blocks, so-called “material voxels”, to realize designer nanomaterials with desired functions.},
doi = {10.1002/ange.202105678},
journal = {Angewandte Chemie},
number = 3,
volume = 134,
place = {United States},
year = {Mon Jun 14 00:00:00 EDT 2021},
month = {Mon Jun 14 00:00:00 EDT 2021}
}
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