Search Menu
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information
Search Scholarly Publications

Title: 3D velocity map imaging of electrons with TPX3CAM

Abstract

In this report we demonstrate three-dimensional velocity map imaging of low energy electrons using a TPX3CAM, where the three-dimensional momentum information [$$p_x, p_y, p_z$$] is encoded in position and timing [x, y, t] of hits on the camera sensor. We make use of the camera sensor for the [x, y] information and a constant fraction discriminator and fast time to digital converter in the camera for the time information. We illustrate the capabilities of our apparatus by presenting above threshold ionization measurements of xenon, which produces well defined structures in the momentum resolved photoelectron yield.

Authors:
 [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [2];  [3]
+ Show Author Affiliations
  1. Stony Brook Univ., NY (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Univ. of Connecticut, Storrs, CT (United States)
Publication Date:
Research Org.:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Laboratory Directed Research and Development (LDRD) Program; US Air Force Office of Scientific Research (AFOSR)
OSTI Identifier:
1845416
Alternate Identifier(s):
OSTI ID: 1838384
Report Number(s):
BNL-222755-2022-JAAM
Journal ID: ISSN 0034-6748; TRN: US2302444
Grant/Contract Number:  
SC0012704; G02-08ER15983; FA9550-17-1-0369; DEF-G02-08ER15983; 19-30
Resource Type:
Accepted Manuscript
Journal Name:
Review of Scientific Instruments
Additional Journal Information:
Journal Volume: 93; Journal Issue: 1; Journal ID: ISSN 0034-6748
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
79 ASTRONOMY AND ASTROPHYSICS; data streams; integral transforms; time-to-digital converter; pump probe experiments; electron diffraction; stereoscopy; optical materials; femtosecond lasers; field desorption; velocity map imaging

Citation Formats

Cheng, Chuan, Mogol, Gonenc, Weinacht, Thomas, Nomerotski, Andrei, and Trallero-Herrero, Carlos. 3D velocity map imaging of electrons with TPX3CAM. United States: N. p., 2022. Web. doi:10.1063/5.0071804.
Copy to clipboard
Cheng, Chuan, Mogol, Gonenc, Weinacht, Thomas, Nomerotski, Andrei, & Trallero-Herrero, Carlos. 3D velocity map imaging of electrons with TPX3CAM. United States. https://doi.org/10.1063/5.0071804
Copy to clipboard
Cheng, Chuan, Mogol, Gonenc, Weinacht, Thomas, Nomerotski, Andrei, and Trallero-Herrero, Carlos. Wed . "3D velocity map imaging of electrons with TPX3CAM". United States. https://doi.org/10.1063/5.0071804. https://www.osti.gov/servlets/purl/1845416.
Copy to clipboard
@article{osti_1845416,
title = {3D velocity map imaging of electrons with TPX3CAM},
author = {Cheng, Chuan and Mogol, Gonenc and Weinacht, Thomas and Nomerotski, Andrei and Trallero-Herrero, Carlos},
abstractNote = {In this report we demonstrate three-dimensional velocity map imaging of low energy electrons using a TPX3CAM, where the three-dimensional momentum information [$p_x, p_y, p_z$] is encoded in position and timing [x, y, t] of hits on the camera sensor. We make use of the camera sensor for the [x, y] information and a constant fraction discriminator and fast time to digital converter in the camera for the time information. We illustrate the capabilities of our apparatus by presenting above threshold ionization measurements of xenon, which produces well defined structures in the momentum resolved photoelectron yield.},
doi = {10.1063/5.0071804},
journal = {Review of Scientific Instruments},
number = 1,
volume = 93,
place = {United States},
year = {Wed Jan 05 00:00:00 EST 2022},
month = {Wed Jan 05 00:00:00 EST 2022}
}
Copy to clipboard
Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1063/5.0071804
Copyright Statement
Other availability
Search WorldCat Search WorldCat to find libraries that may hold this journal
Save / Share:
Export Metadata
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.

Works referenced in this record:

Absolute ion detection efficiencies of microchannel plates and funnel microchannel plates for multi-coincidence detection
journal, April 2018

  • Fehre, K.; Trojanowskaja, D.; Gatzke, J.
  • Review of Scientific Instruments, Vol. 89, Issue 4
  • DOI: 10.1063/1.5022564

Two‐dimensional imaging of state‐selected photodissociation products detected by multiphoton ionization
journal, July 1987

  • Chandler, David W.; Houston, Paul L.
  • The Journal of Chemical Physics, Vol. 87, Issue 2
  • DOI: 10.1063/1.453276

Timepix3: a 65K channel hybrid pixel readout chip with simultaneous ToA/ToT and sparse readout
journal, May 2014

Communication: Time- and space-sliced velocity map electron imaging
journal, December 2014

  • Lee, Suk Kyoung; Lin, Yun Fei; Lingenfelter, Steven
  • The Journal of Chemical Physics, Vol. 141, Issue 22
  • DOI: 10.1063/1.4903744

Velocity map imaging of ions and electrons using electrostatic lenses: Application in photoelectron and photofragment ion imaging of molecular oxygen
journal, September 1997

  • Eppink, André T. J. B.; Parker, David H.
  • Review of Scientific Instruments, Vol. 68, Issue 9
  • DOI: 10.1063/1.1148310

A photoelectron-photoion coincidence imaging apparatus for femtosecond time-resolved molecular dynamics with electron time-of-flight resolution of σ=18ps and energy resolution ΔE∕E=3.5%
journal, June 2008

  • Vredenborg, Arno; Roeterdink, Wim G.; Janssen, Maurice H. M.
  • Review of Scientific Instruments, Vol. 79, Issue 6
  • DOI: 10.1063/1.2949142

Coincidence velocity map imaging using a single detector
journal, July 2017

  • Zhao, Arthur; Sándor, Péter; Weinacht, Thomas
  • The Journal of Chemical Physics, Vol. 147, Issue 1
  • DOI: 10.1063/1.4981917

Imaging ultrafast molecular dynamics with laser-induced electron diffraction
journal, March 2012

  • Blaga, Cosmin I.; Xu, Junliang; DiChiara, Anthony D.
  • Nature, Vol. 483, Issue 7388
  • DOI: 10.1038/nature10820

Direct current slice imaging
journal, April 2003

  • Townsend, Dave; Minitti, Michael P.; Suits, Arthur G.
  • Review of Scientific Instruments, Vol. 74, Issue 4
  • DOI: 10.1063/1.1544053

Thick-lens velocity-map imaging spectrometer with high resolution for high-energy charged particles
journal, May 2014

Coincidence velocity map imaging using Tpx3Cam, a time stamping optical camera with 1.5 ns timing resolution
journal, November 2017

  • Zhao, Arthur; van Beuzekom, Martin; Bouwens, Bram
  • Review of Scientific Instruments, Vol. 88, Issue 11
  • DOI: 10.1063/1.4996888

Femtosecond Time-Resolved Photoelectron Spectroscopy
journal, April 2004

  • Stolow, Albert; Bragg, Arthur E.; Neumark, Daniel M.
  • Chemical Reviews, Vol. 104, Issue 4
  • DOI: 10.1021/cr020683w

Excited state dynamics of CH 2 I 2 and CH 2 BrI studied with UV pump VUV probe photoelectron spectroscopy
journal, May 2019

  • Horton, Spencer L.; Liu, Yusong; Forbes, Ruaridh
  • The Journal of Chemical Physics, Vol. 150, Issue 17
  • DOI: 10.1063/1.5086665

Recoil-ion and electron momentum spectroscopy: reaction-microscopes
journal, August 2003

Slice imaging: A new approach to ion imaging and velocity mapping
journal, October 2001

  • Gebhardt, Christoph R.; Rakitzis, T. Peter; Samartzis, Peter C.
  • Review of Scientific Instruments, Vol. 72, Issue 10
  • DOI: 10.1063/1.1403010

Recoil-ion momentum spectroscopy
journal, July 1997

  • Ullrich, J.; Moshammer, R.; Dörner, R.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 30, Issue 13
  • DOI: 10.1088/0953-4075/30/13/006

Laser-induced electron diffraction: a new tool for probing ultrafast molecular dynamics
journal, September 1996

Imaging and time stamping of photons with nanosecond resolution in Timepix based optical cameras
journal, September 2019

  • Nomerotski, Andrei
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 937
  • DOI: 10.1016/j.nima.2019.05.034

Slicing Using a Conventional Velocity Map Imaging Setup:  O 2 , I 2 , and I 2 + Photodissociation †
journal, September 2004

  • Chestakov, Dmitri A.; Wu, Shiou-Min; Wu, Guorong
  • The Journal of Physical Chemistry A, Vol. 108, Issue 39
  • DOI: 10.1021/jp0491111

A direct comparison of high-speed methods for the numerical Abel transform
journal, June 2019

  • Hickstein, Daniel D.; Gibson, Stephen T.; Yurchak, Roman
  • Review of Scientific Instruments, Vol. 90, Issue 6
  • DOI: 10.1063/1.5092635

Excited-state dynamics of CH 2 I 2 and CH 2 IBr studied with UV-pump VUV-probe momentum-resolved photoion spectroscopy
journal, November 2020

  • Liu, Yusong; Rozgonyi, Tamás; Marquetand, Philipp
  • The Journal of Chemical Physics, Vol. 153, Issue 18
  • DOI: 10.1063/5.0026177
    Sort by:
    [ × clear filter / sort ]

    Similar Records in DOE PAGES and OSTI.GOV collections: