Title: Vertical Variations of Cloud Microphysical Relationships in Marine Stratocumulus Clouds Observed During the ACE‐ENA Campaign

Journal Article · · Journal of Geophysical Research: Atmospheres
ORCiD logo [1]; ORCiD logo [2];  [3];  [2];  [4]; ORCiD logo [5]; ORCiD logo [6]; ORCiD logo [7]; ORCiD logo [7]; ORCiD logo [7]
  1. Department of Physics Michigan Technological University MI USA, Department of Atmospheric Sciences Yonsei University Seoul Korea
  2. Department of Atmospheric Sciences Yonsei University Seoul Korea
  3. Department of Physics Michigan Technological University MI USA
  4. Department of Energy Environmental and Chemical Engineering Center for Aerosol Science and Engineering University of Washington St. Louis WA USA
  5. Key Laboratory for Aerosol‐Cloud‐Precipitation of China Meteorological Administration/Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters (CIC‐FEMD) Nanjing University of Information Science &, Technology Nanjing China
  6. Environmental and Climate Sciences Department Brookhaven National Laboratory Upton NY USA
  7. Pacific Northwest National Laboratory Richland WA USA

Abstract This study examines the vertical variations of cloud microphysical relationships and their implications to cloud microphysical processes in marine stratocumulus clouds using in‐situ aircraft observations during the Aerosol and Cloud Experiments in Eastern North Atlantic (ACE‐ENA) field campaign. A new diagram with a coordinate system based on cloud droplet liquid water content (L c ) and phase relaxation time scale is proposed to investigate mixing mechanisms. This new diagram analysis shows that the inhomogeneous mixing trait is dominant near the cloud top, but homogeneous mixing trait is stronger at lower altitudes. The relevant scale parameters (i.e., transition length scale and transition scale number) also indicate a high likelihood of inhomogeneous mixing. The relationship between L c and standard deviation of droplet radius (σ R ) clearly shows the vertical transition: the correlation between L c and σ R is positive at lower cloud altitudes, but it becomes negative as altitude increases. Such a vertical transition is consistent with the vertical circulation mixing, modulating the cloud microphysical relationships to suggest homogeneous mixing at a significant depth from the cloud top.

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Atmospheric Radiation Measurement (ARM) Data Center; Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
Korea government (MSIT); National Natural Science Foundation of China (NSFC); National Research Foundation of Korea (NRF); USDOE; USDOE Office of Science (SC), Biological and Environmental Research (BER)
Contributing Organization:
Argonne National Lab. (ANL), Argonne, IL (United States)
Grant/Contract Number:
AC05-76RL01830; SC0012704; SC0020052; SC0020053
OSTI ID:
1835384
Report Number(s):
BNL-222437-2021-JAAM; PNNL-SA-159750; e2021JD034700
Journal Information:
Journal of Geophysical Research: Atmospheres, Journal Name: Journal of Geophysical Research: Atmospheres Journal Issue: 24 Vol. 126; ISSN 2169-897X
Publisher:
American Geophysical Union (AGU)Copyright Statement
Country of Publication:
United States
Language:
English

References (51)

Improvement of cloud microphysics in the aerosol-climate model BCC_AGCM2.0.1_CUACE/Aero, evaluation against observations, and updated aerosol indirect effect journal July 2014
Scale dependence of entrainment-mixing mechanisms in cumulus clouds: Scale dependence of mixing mechanisms journal December 2014
Cloud microphysical relationships and their implication on entrainment and mixing mechanism for the stratocumulus clouds measured during the VOCALS project: CLOUD MICROPHYSICS - ENTRAINMENT, MIXING journal May 2015
Evaporative cooling amplification of the entrainment velocity in radiatively driven stratocumulus journal September 2015
On the size distribution of cloud holes in stratocumulus and their relationship to cloud-top entrainment: ENTRAINMENT IN STRATOCUMLUS CLOUD HOLES journal May 2013
Entrainment rates and microphysics in POST stratocumulus: ENTRAINMENT RATES IN STRATOCUMULUS journal November 2013
Simple approach to dynamics of entrainment interface layers and cloud holes in stratocumulus clouds journal January 2009
Models of cloud-topped mixed layers under a strong inversion journal July 1968
Laboratory studies of the effects of mixing on the evolution of cloud droplet spectra journal April 1977
The influence of entrainment on the evolution of cloud droplet spectra: I. A model of inhomogeneous mixing journal July 1980
Small scale mixing processes at the top of a marine stratocumulus—a case study
  • Haman, Krzysztof E.; Malinowski, Szymon P.; Kurowski, Marcin J.
  • Quarterly Journal of the Royal Meteorological Society, Vol. 133, Issue 622 https://doi.org/10.1002/qj.5
journal January 2007
Do stratocumulus clouds detrain? FIRE I data revisited journal October 2006
Microphysical properties of stratocumulus clouds journal September 2000
Statistical analysis of microphysical properties and the parameterization of effective radius of warm clouds in Beijing area journal August 2009
A study on the entrainment and mixing process in the continental stratocumulus clouds measured during the RACORO campaign journal September 2017
Impact of secondary droplet activation on the contrasting cloud microphysical relationships during the wet and dry seasons in the Amazon journal December 2019
Cloud transitions and decoupling in shear-free stratocumulus-topped boundary layers journal August 2000
Observations of marine stratocumulus microphysics and implications for processes controlling droplet spectra: Results from the Marine Stratus/Stratocumulus Experiment journal January 2009
Examination of turbulent entrainment-mixing mechanisms using a combined approach journal January 2011
Dispersion Aerosol Indirect Effect in Turbulent Clouds: Laboratory Measurements of Effective Radius journal October 2018
Search for Microphysical Signatures of Stochastic Condensation in Marine Boundary Layer Clouds Using Airborne Digital Holography journal March 2019
Contrasting Scale Dependence of Entrainment‐Mixing Mechanisms in Stratocumulus Clouds journal May 2020
Contribution to the cloud droplet effective radius parameterization journal November 1992
Open-path airborne tunable diode laser hygrometer
  • Diskin, Glenn S.; Podolske, James R.; Sachse, Glen W.
  • International Symposium on Optical Science and Technology, SPIE Proceedings https://doi.org/10.1117/12.453736
conference September 2002
Interpretation of Cloud-Climate Feedback as Produced by 14 Atmospheric General Circulation Models journal August 1989
Holographic measurements of inhomogeneous cloud mixing at the centimeter scale journal October 2015
Cloud-Top Entrainment in Stratocumulus Clouds journal January 2017
The Effect of Cloud Type on Earth's Energy Balance: Global Analysis journal November 1992
Turbulent Characteristics of Some Canadian Cumulus Clouds journal January 1977
Overestimates of Entrainment From Wetting of Aircraft Temperature Sensors in Cloud journal January 1979
The Microstructure of Cumulus Cloud: Part IV. The Effect on the Droplet Spectrum of Mixing Between Cloud and Environment journal March 1973
Conditional Instability of the First Kind Upside-Down journal January 1980
Cloud Top Entrainment Instability journal January 1980
A Simple Model of Droplet Spectral Evolution during Turbulent Mixing journal September 1989
Linear Eddy Modeling of Entrainment and Mixing in Stratus Clouds journal September 1993
Supersaturation of Water Vapor in Clouds journal December 2003
Large-Eddy Simulation of Evaporatively Driven Entrainment in Cloud-Topped Mixed Layers journal May 2008
Estimating the Evaporative Cooling Bias of an Airborne Reverse Flow Thermometer journal January 2009
Homogeneous and Inhomogeneous Mixing in Cumulus Clouds: Dependence on Local Turbulence Structure journal December 2009
The DOE ARM Aerial Facility journal May 2014
Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) journal February 2022
Holes and Entrainment in Stratocumulus journal February 2005
Cooling of Entrained Parcels in a Large-Eddy Simulation journal March 2012
A New Mechanism of Droplet Size Distribution Broadening during Diffusional Growth journal July 2013
Reduction of the Entrainment Velocity by Cloud Droplet Sedimentation in Stratocumulus journal March 2017
Influence of Microphysical Variability on Stochastic Condensation in a Turbulent Laboratory Cloud journal January 2018
Entrainment and Mixing in Stratocumulus: Effects of a New Explicit Subgrid-Scale Scheme for Large-Eddy Simulations with Particle-Based Microphysics journal July 2019
Observational Study of the Entrainment-Mixing Process in Warm Convective Clouds journal June 2007
Stratocumulus Clouds journal August 2012
Entrainment, Mixing, and Microphysics in Trade-Wind Cumulus journal January 2008
Physics of Stratocumulus Top (POST): turbulent mixing across capping inversion journal January 2013