Solution-Phase Synthesis of Cesium Lead Halide Perovskite Nanowires
Abstract
Halide perovskites have attracted much attention over the past 5 years as a promising class of materials for optoelectronic applications. However, compared to hybrid organic-inorganic perovskites, the study of their pure inorganic counterparts, like cesium lead halides (CsPbX3), lags far behind. Here, a catalyst-free, solution-phase synthesis of CsPbX3 nanowires (NWs) is reported. These NWs are single-crystalline, with uniform growth direction, and crystallize in the orthorhombic phase. Both CsPbBr3 and CsPbI3 are photoluminescence active, with composition-dependent temperature and self-trapping behavior. These NWs with a well-defined morphology could serve as an ideal platform for the investigation of fundamental properties and the development of future applications in nanoscale optoelectronic devices based on all-inorganic perovskites.
- Authors:
-
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States)
- Univ. of California, Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1832456
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of the American Chemical Society
- Additional Journal Information:
- Journal Volume: 137; Journal Issue: 29; Journal ID: ISSN 0002-7863
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; Crystallization; Physical and chemical processes; Transmission electron microscopy; Optoelectronics; Perovskites
Citation Formats
Zhang, Dandan, Eaton, Samuel W., Yu, Yi, Dou, Letian, and Yang, Peidong. Solution-Phase Synthesis of Cesium Lead Halide Perovskite Nanowires. United States: N. p., 2015.
Web. doi:10.1021/jacs.5b05404.
Zhang, Dandan, Eaton, Samuel W., Yu, Yi, Dou, Letian, & Yang, Peidong. Solution-Phase Synthesis of Cesium Lead Halide Perovskite Nanowires. United States. https://doi.org/10.1021/jacs.5b05404
Zhang, Dandan, Eaton, Samuel W., Yu, Yi, Dou, Letian, and Yang, Peidong. Thu .
"Solution-Phase Synthesis of Cesium Lead Halide Perovskite Nanowires". United States. https://doi.org/10.1021/jacs.5b05404. https://www.osti.gov/servlets/purl/1832456.
@article{osti_1832456,
title = {Solution-Phase Synthesis of Cesium Lead Halide Perovskite Nanowires},
author = {Zhang, Dandan and Eaton, Samuel W. and Yu, Yi and Dou, Letian and Yang, Peidong},
abstractNote = {Halide perovskites have attracted much attention over the past 5 years as a promising class of materials for optoelectronic applications. However, compared to hybrid organic-inorganic perovskites, the study of their pure inorganic counterparts, like cesium lead halides (CsPbX3), lags far behind. Here, a catalyst-free, solution-phase synthesis of CsPbX3 nanowires (NWs) is reported. These NWs are single-crystalline, with uniform growth direction, and crystallize in the orthorhombic phase. Both CsPbBr3 and CsPbI3 are photoluminescence active, with composition-dependent temperature and self-trapping behavior. These NWs with a well-defined morphology could serve as an ideal platform for the investigation of fundamental properties and the development of future applications in nanoscale optoelectronic devices based on all-inorganic perovskites.},
doi = {10.1021/jacs.5b05404},
journal = {Journal of the American Chemical Society},
number = 29,
volume = 137,
place = {United States},
year = {Thu Jul 16 00:00:00 EDT 2015},
month = {Thu Jul 16 00:00:00 EDT 2015}
}
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