Strategies towards enabling lithium metal in batteries: interphases and electrodes
Abstract
Despite the continuous increase in capacity, lithium-ion intercalation batteries are approaching their performance limits. As a result, research is intensifying on next-generation battery technologies. The use of a lithium metal anode promises the highest theoretical energy density and enables use of lithium-free or novel high-energy cathodes. However, the lithium metal anode suffers from poor morphological stability and Coulombic efficiency during cycling, especially in liquid electrolytes. In contrast to solid electrolytes, liquid electrolytes have the advantage of high ionic conductivity and good wetting of the anode, despite the lithium metal volume change during cycling. Rapid capacity fade due to inhomogeneous deposition and dissolution of lithium is the main hindrance to the successful utilization of the lithium metal anode in combination with liquid electrolytes. In this perspective, we discuss how experimental and theoretical insights can provide possible pathways for reversible cycling of two-dimensional lithium metal. Therefore, we discuss improvements in the understanding of lithium metal nucleation, deposition, and stripping on the nanoscale. As the solid–electrolyte interphase (SEI) plays a key role in the lithium morphology, we discuss how the proper SEI design might allow stable cycling. We highlight recent advances in conventional and (localized) highly concentrated electrolytes in view of their respectivemore »
- Authors:
-
more »
- Helmholtz Institute Ulm (HIU), Ulm 89081, Germany, German Aerospace Center (DLR), Stuttgart 70569, Germany
- Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL 60439, USA
- Material Sciences Division, Argonne National Laboratory, Lemont, IL 60439, USA
- Energy Storage and Distributed Resources Division, Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA 94720, USA
- Energy and Environment Directorate, Pacific Northwest National Laboratory (PNNL), Richland, WA 99354, USA
- Institute of Energy and Climate Research IEK-9, Forschungszentrum Jülich GmbH, Jülich, Germany
- Helmholtz-Institute Münster (HI MS), IEK-12, Forschungszentrum Jülich GmbH, Münster, 48149, Germany
- University of Münster, MEET Battery Research Center, Münster, 48149, Germany
- Research Laboratory of Electronics, Massachusetts Institute of Technology (MIT), Cambridge, Massachusetts 02139, USA
- Department of Chemical Engineering, Texas A&M University, College Station, TX 77843, USA
- Institute for Applied Materials – Electrochemical Technologies (IAM-ET), Karlsruhe Institute of Technology (KIT), Karlsruhe 76021, Germany
- Helmholtz Institute Ulm (HIU), Ulm 89081, Germany, Karlsruhe Institute of Technology (KIT), Karlsruhe 76021, Germany
- Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory (PNNL), Richland, WA 99354, USA
- Research Laboratory of Electronics, Massachusetts Institute of Technology (MIT), Cambridge, Massachusetts 02139, USA, Department of Mechanical Engineering, Massachusetts Institute of Technology (MIT), Cambridge, MA 02139, USA, Department of Materials Science and Engineering, Massachusetts Institute of Technology (MIT), Cambridge, MA 02139, USA
- Helmholtz-Institute Münster (HI MS), IEK-12, Forschungszentrum Jülich GmbH, Münster, 48149, Germany, University of Münster, MEET Battery Research Center, Münster, 48149, Germany
- Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL 60439, USA, Material Science and Engineering, Stanford University, Stanford, CA 94305, USA
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- OSTI Identifier:
- 1811080
- Alternate Identifier(s):
- OSTI ID: 1819859; OSTI ID: 1830505; OSTI ID: 1840906
- Report Number(s):
- PNNL-SA-160592
Journal ID: ISSN 1754-5692; EESNBY
- Grant/Contract Number:
- AC02-05CH11231; AC05-76RL01830; AC02-06CH11357
- Resource Type:
- Published Article
- Journal Name:
- Energy & Environmental Science
- Additional Journal Information:
- Journal Name: Energy & Environmental Science Journal Volume: 14 Journal Issue: 10; Journal ID: ISSN 1754-5692
- Publisher:
- Royal Society of Chemistry (RSC)
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- 25 ENERGY STORAGE
Citation Formats
Horstmann, Birger, Shi, Jiayan, Amine, Rachid, Werres, Martin, He, Xin, Jia, Hao, Hausen, Florian, Cekic-Laskovic, Isidora, Wiemers-Meyer, Simon, Lopez, Jeffrey, Galvez-Aranda, Diego, Baakes, Florian, Bresser, Dominic, Su, Chi-Cheung, Xu, Yaobin, Xu, Wu, Jakes, Peter, Eichel, Rüdiger-A., Figgemeier, Egbert, Krewer, Ulrike, Seminario, Jorge M., Balbuena, Perla B., Wang, Chongmin, Passerini, Stefano, Shao-Horn, Yang, Winter, Martin, Amine, Khalil, Kostecki, Robert, and Latz, Arnulf. Strategies towards enabling lithium metal in batteries: interphases and electrodes. United Kingdom: N. p., 2021.
Web. doi:10.1039/D1EE00767J.
Horstmann, Birger, Shi, Jiayan, Amine, Rachid, Werres, Martin, He, Xin, Jia, Hao, Hausen, Florian, Cekic-Laskovic, Isidora, Wiemers-Meyer, Simon, Lopez, Jeffrey, Galvez-Aranda, Diego, Baakes, Florian, Bresser, Dominic, Su, Chi-Cheung, Xu, Yaobin, Xu, Wu, Jakes, Peter, Eichel, Rüdiger-A., Figgemeier, Egbert, Krewer, Ulrike, Seminario, Jorge M., Balbuena, Perla B., Wang, Chongmin, Passerini, Stefano, Shao-Horn, Yang, Winter, Martin, Amine, Khalil, Kostecki, Robert, & Latz, Arnulf. Strategies towards enabling lithium metal in batteries: interphases and electrodes. United Kingdom. https://doi.org/10.1039/D1EE00767J
Horstmann, Birger, Shi, Jiayan, Amine, Rachid, Werres, Martin, He, Xin, Jia, Hao, Hausen, Florian, Cekic-Laskovic, Isidora, Wiemers-Meyer, Simon, Lopez, Jeffrey, Galvez-Aranda, Diego, Baakes, Florian, Bresser, Dominic, Su, Chi-Cheung, Xu, Yaobin, Xu, Wu, Jakes, Peter, Eichel, Rüdiger-A., Figgemeier, Egbert, Krewer, Ulrike, Seminario, Jorge M., Balbuena, Perla B., Wang, Chongmin, Passerini, Stefano, Shao-Horn, Yang, Winter, Martin, Amine, Khalil, Kostecki, Robert, and Latz, Arnulf. Wed .
"Strategies towards enabling lithium metal in batteries: interphases and electrodes". United Kingdom. https://doi.org/10.1039/D1EE00767J.
@article{osti_1811080,
title = {Strategies towards enabling lithium metal in batteries: interphases and electrodes},
author = {Horstmann, Birger and Shi, Jiayan and Amine, Rachid and Werres, Martin and He, Xin and Jia, Hao and Hausen, Florian and Cekic-Laskovic, Isidora and Wiemers-Meyer, Simon and Lopez, Jeffrey and Galvez-Aranda, Diego and Baakes, Florian and Bresser, Dominic and Su, Chi-Cheung and Xu, Yaobin and Xu, Wu and Jakes, Peter and Eichel, Rüdiger-A. and Figgemeier, Egbert and Krewer, Ulrike and Seminario, Jorge M. and Balbuena, Perla B. and Wang, Chongmin and Passerini, Stefano and Shao-Horn, Yang and Winter, Martin and Amine, Khalil and Kostecki, Robert and Latz, Arnulf},
abstractNote = {Despite the continuous increase in capacity, lithium-ion intercalation batteries are approaching their performance limits. As a result, research is intensifying on next-generation battery technologies. The use of a lithium metal anode promises the highest theoretical energy density and enables use of lithium-free or novel high-energy cathodes. However, the lithium metal anode suffers from poor morphological stability and Coulombic efficiency during cycling, especially in liquid electrolytes. In contrast to solid electrolytes, liquid electrolytes have the advantage of high ionic conductivity and good wetting of the anode, despite the lithium metal volume change during cycling. Rapid capacity fade due to inhomogeneous deposition and dissolution of lithium is the main hindrance to the successful utilization of the lithium metal anode in combination with liquid electrolytes. In this perspective, we discuss how experimental and theoretical insights can provide possible pathways for reversible cycling of two-dimensional lithium metal. Therefore, we discuss improvements in the understanding of lithium metal nucleation, deposition, and stripping on the nanoscale. As the solid–electrolyte interphase (SEI) plays a key role in the lithium morphology, we discuss how the proper SEI design might allow stable cycling. We highlight recent advances in conventional and (localized) highly concentrated electrolytes in view of their respective SEIs. We also discuss artificial interphases and three-dimensional host frameworks, which show prospects of mitigating morphological instabilities and suppressing large shape change on the electrode level.},
doi = {10.1039/D1EE00767J},
journal = {Energy & Environmental Science},
number = 10,
volume = 14,
place = {United Kingdom},
year = {2021},
month = {10}
}
https://doi.org/10.1039/D1EE00767J
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