Accelerated annealing of colloidal crystal monolayers by means of cyclically applied electric fields
Abstract
Abstract External fields are commonly applied to accelerate colloidal crystallization; however, accelerated self-assembly kinetics can negatively impact the quality of crystal structures. We show that cyclically applied electric fields can produce high quality colloidal crystals by annealing local disorder. We find that the optimal off-duration for maximum annealing is approximately one-half of the characteristic melting half lifetime of the crystalline phase. Local six-fold bond orientational order grows more rapidly than global scattering peaks, indicating that local restructuring leads global annealing. Molecular dynamics simulations of cyclically activated systems show that the ratio of optimal off-duration for maximum annealing and crystal melting time is insensitive to particle interaction details. This research provides a quantitative relationship describing how the cyclic application of fields produces high quality colloidal crystals by cycling at the fundamental time scale for local defect rearrangements; such understanding of dynamics and kinetics can be applied for reconfigurable colloidal assembly.
- Authors:
- Publication Date:
- Research Org.:
- Univ. of Michigan, Ann Arbor, MI (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1784786
- Alternate Identifier(s):
- OSTI ID: 1816717
- Grant/Contract Number:
- SC0013562
- Resource Type:
- Published Article
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Name: Scientific Reports Journal Volume: 11 Journal Issue: 1; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Kao, Peng-Kai, VanSaders, Bryan J., Glotzer, Sharon C., and Solomon, Michael J. Accelerated annealing of colloidal crystal monolayers by means of cyclically applied electric fields. United Kingdom: N. p., 2021.
Web. doi:10.1038/s41598-021-90310-7.
Kao, Peng-Kai, VanSaders, Bryan J., Glotzer, Sharon C., & Solomon, Michael J. Accelerated annealing of colloidal crystal monolayers by means of cyclically applied electric fields. United Kingdom. https://doi.org/10.1038/s41598-021-90310-7
Kao, Peng-Kai, VanSaders, Bryan J., Glotzer, Sharon C., and Solomon, Michael J. Wed .
"Accelerated annealing of colloidal crystal monolayers by means of cyclically applied electric fields". United Kingdom. https://doi.org/10.1038/s41598-021-90310-7.
@article{osti_1784786,
title = {Accelerated annealing of colloidal crystal monolayers by means of cyclically applied electric fields},
author = {Kao, Peng-Kai and VanSaders, Bryan J. and Glotzer, Sharon C. and Solomon, Michael J.},
abstractNote = {Abstract External fields are commonly applied to accelerate colloidal crystallization; however, accelerated self-assembly kinetics can negatively impact the quality of crystal structures. We show that cyclically applied electric fields can produce high quality colloidal crystals by annealing local disorder. We find that the optimal off-duration for maximum annealing is approximately one-half of the characteristic melting half lifetime of the crystalline phase. Local six-fold bond orientational order grows more rapidly than global scattering peaks, indicating that local restructuring leads global annealing. Molecular dynamics simulations of cyclically activated systems show that the ratio of optimal off-duration for maximum annealing and crystal melting time is insensitive to particle interaction details. This research provides a quantitative relationship describing how the cyclic application of fields produces high quality colloidal crystals by cycling at the fundamental time scale for local defect rearrangements; such understanding of dynamics and kinetics can be applied for reconfigurable colloidal assembly.},
doi = {10.1038/s41598-021-90310-7},
journal = {Scientific Reports},
number = 1,
volume = 11,
place = {United Kingdom},
year = {Wed May 26 00:00:00 EDT 2021},
month = {Wed May 26 00:00:00 EDT 2021}
}
https://doi.org/10.1038/s41598-021-90310-7
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