Charge Condensation and Lattice Coupling Drives Stripe Formation in Nickelates

Shen, Yao; Fabbris, G.; Miao, H.; Cao, Y.; Meyers, D.; Mazzone, D. G.; Assefa, T. A.; Chen, X. M.; Kisslinger, K.; Prabhakaran, D.; Boothroyd, A. T.; Tranquada, J. M.; Hu, Wen; Barbour, A. M.; Wilkins, S. B.; Mazzoli, C.; Robinson, I. K.; Dean, Mark P. M.

doi:10.1103/physrevlett.126.177601

Title: Charge Condensation and Lattice Coupling Drives Stripe Formation in Nickelates

Abstract

Revealing the predominant driving force behind symmetry breaking in correlated materials is sometimes a formidable task due to the intertwined nature of different degrees of freedom. This is the case for La_2–xSr_xNiO_4+δ, in which coupled incommensurate charge and spin stripes form at low temperatures. Here, we use resonant x-ray photon correlation spectroscopy to study the temporal stability and domain memory of the charge and spin stripes in La_2–xSr_xNiO_4+δ. Although spin stripes are more spatially correlated, charge stripes maintain a better temporal stability against temperature change. More intriguingly, charge order shows robust domain memory with thermal cycling up to 250 K, far above the ordering temperature. Furthermore, these results demonstrate the pinning of charge stripes to the lattice and that charge condensation is the predominant factor in the formation of stripe orders in nickelates.

Authors:

^[1];

^[2];

^[3]; Cao, Y. ^[2]; Meyers, D. ^[4];

^[5];

^[1]; Chen, X. M. ^[1]; Kisslinger, K. ^[1]; Prabhakaran, D. ^[6]; Boothroyd, A. T. ^[6];

^[1]; Hu, Wen ^[1]; Barbour, A. M. ^[1]; Wilkins, S. B. ^[1]; Mazzoli, C. ^[1]; Robinson, I. K. ^[1];

^[1]

Brookhaven National Lab. (BNL), Upton, NY (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Argonne National Lab. (ANL), Lemont, IL (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Oklahoma State Univ., Stillwater, OK (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Paul Scherrer Inst. (PSI), Villigen (Switzerland)
Univ. of Oxford (United Kingdom)

Publication Date:: Fri Apr 30 00:00:00 EDT 2021

Research Org.:: Brookhaven National Lab. (BNL), Upton, NY (United States); Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1782544

Alternate Identifier(s):: OSTI ID: 1797793; OSTI ID: 1823619

Report Number(s):: BNL-221368-2021-JAAM; BNL-222088-2021-JAAM
Journal ID: ISSN 0031-9007; TRN: US2210014

Grant/Contract Number:: SC0012704; AC0206CH11357; AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Letters

Additional Journal Information:: Journal Volume: 126; Journal Issue: 17; Journal ID: ISSN 0031-9007

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Charge order; Magnetic order; Complex oxides; Coherent X-ray scattering

Citation Formats


                    Shen, Yao, Fabbris, G., Miao, H., Cao, Y., Meyers, D., Mazzone, D. G., Assefa, T. A., Chen, X. M., Kisslinger, K., Prabhakaran, D., Boothroyd, A. T., Tranquada, J. M., Hu, Wen, Barbour, A. M., Wilkins, S. B., Mazzoli, C., Robinson, I. K., and Dean, Mark P. M. Charge Condensation and Lattice Coupling Drives Stripe Formation in Nickelates.  United States: N. p., 2021. 
Web.  doi:10.1103/physrevlett.126.177601.

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                    Shen, Yao, Fabbris, G., Miao, H., Cao, Y., Meyers, D., Mazzone, D. G., Assefa, T. A., Chen, X. M., Kisslinger, K., Prabhakaran, D., Boothroyd, A. T., Tranquada, J. M., Hu, Wen, Barbour, A. M., Wilkins, S. B., Mazzoli, C., Robinson, I. K., & Dean, Mark P. M. Charge Condensation and Lattice Coupling Drives Stripe Formation in Nickelates.  United States.  https://doi.org/10.1103/physrevlett.126.177601

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                    Shen, Yao, Fabbris, G., Miao, H., Cao, Y., Meyers, D., Mazzone, D. G., Assefa, T. A., Chen, X. M., Kisslinger, K., Prabhakaran, D., Boothroyd, A. T., Tranquada, J. M., Hu, Wen, Barbour, A. M., Wilkins, S. B., Mazzoli, C., Robinson, I. K., and Dean, Mark P. M. Fri .  
"Charge Condensation and Lattice Coupling Drives Stripe Formation in Nickelates".  United States.  https://doi.org/10.1103/physrevlett.126.177601.  https://www.osti.gov/servlets/purl/1782544.

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@article{osti_1782544,

  title        = {Charge Condensation and Lattice Coupling Drives Stripe Formation in Nickelates},

  author       = {Shen, Yao and Fabbris, G. and Miao, H. and Cao, Y. and Meyers, D. and Mazzone, D. G. and Assefa, T. A. and Chen, X. M. and Kisslinger, K. and Prabhakaran, D. and Boothroyd, A. T. and Tranquada, J. M. and Hu, Wen and Barbour, A. M. and Wilkins, S. B. and Mazzoli, C. and Robinson, I. K. and Dean, Mark P. M.},

  abstractNote = {Revealing the predominant driving force behind symmetry breaking in correlated materials is sometimes a formidable task due to the intertwined nature of different degrees of freedom. This is the case for La2–xSrxNiO4+δ, in which coupled incommensurate charge and spin stripes form at low temperatures. Here, we use resonant x-ray photon correlation spectroscopy to study the temporal stability and domain memory of the charge and spin stripes in La2–xSrxNiO4+δ. Although spin stripes are more spatially correlated, charge stripes maintain a better temporal stability against temperature change. More intriguingly, charge order shows robust domain memory with thermal cycling up to 250 K, far above the ordering temperature. Furthermore, these results demonstrate the pinning of charge stripes to the lattice and that charge condensation is the predominant factor in the formation of stripe orders in nickelates.},

  doi          = {10.1103/physrevlett.126.177601},

  journal      = {Physical Review Letters},

  number       = 17,

  volume       = 126,

  place        = {United States},

  year         = {Fri Apr 30 00:00:00 EDT 2021},

  month        = {Fri Apr 30 00:00:00 EDT 2021}

}

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Title: Charge Condensation and Lattice Coupling Drives Stripe Formation in Nickelates

Abstract

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Static charge-density-wave order in the superconducting state of La 2 − x Ba x CuO 4 journal, June 2017

Superconductivity in an infinite-layer nickelate journal, August 2019

Stripe Conductivity in La 1.775 Sr 0.225 NiO 4 journal, April 2000

Spectroscopy of Stripe Order in La 1.8 Sr 0.2 NiO 4 Using Resonant Soft X-Ray Diffraction journal, October 2005

The Physics of Pair-Density Waves: Cuprate Superconductors and Beyond journal, March 2020

Incommensurate charge stripe ordering in La 2 − x Sr x Ni O 4 for x = ( 0.33 , 0.30 , 0.275 ) journal, October 2004

Stripe order at low temperatures in La 2 − x Sr x NiO 4 with 0.289 ≲ x ≲ 0.5 journal, January 2000

Evidence for Short-Range-Ordered Charge Stripes Far above the Charge-Ordering Transition in La 1.67 Sr 0.33 NiO 4 journal, August 2013

Charge and canted spin order in La 2 − x Sr x NiO 4 ( x = 0.275 and 1 3 ) journal, January 2001

Charge and spin ordering in La 2 − x Sr x NiO 4.00 with x =0.135 and 0.20 journal, May 1995

Melting of Quasi-Two-Dimensional Charge Stripes in La 5 / 3 Sr 1 / 3 NiO 4 journal, September 1997

Stripe order and magnetic transitions in La 2 − x Sr x NiO 4 journal, July 2004

X-ray scattering studies of charge stripes in La2−xSrxNiO4 (x=0.20−0.33) journal, June 2002

Charge-ordered states in (La,Sr ) 2 NiO 4 for hole concentrations n h =1/3 and 1/2 journal, March 1994

Doping a Mott insulator: Physics of high-temperature superconductivity journal, January 2006

Growth of large La2–xSrxNiO4+δ single crystals by the floating-zone technique journal, April 2002

Orbital Domain Dynamics in Magnetite below the Verwey Transition
journal, October 2018

Pairing of charge-ordered stripes in (La,Ca)MnO3
journal, April 1998

One-dimensional nature of the magnetic fluctuations in YBa2Cu 3O6.6
journal, April 2000

Spin Stripe Order in a Square Planar Trilayer Nickelate
journal, June 2019

Neutron scattering studies on stripe phases in non-cuprate materials
journal, November 2012

Commensurate-Incommensurate Crossover of Charge Stripe in ${La}_{2 - x} {Sr}_{x} {NiO}_{4}$ ( $x \sim 1 / 3$ )
journal, May 2004

Incommensurate stripe order in ${La}_{2 - x}$ ${Sr}_{x}$ ${NiO}_{4}$ with x =0.225
journal, November 1996

Landau theory of stripe phases in cuprates and nickelates
journal, January 1998

A Four Unit Cell Periodic Pattern of Quasi-Particle States Surrounding Vortex Cores in Bi2Sr2CaCu2O8+delta
journal, January 2002

Strong Superexchange in a $d^{9 - δ}$ Nickelate Revealed by Resonant Inelastic X-Ray Scattering
journal, February 2021

Spin-gap proximity effect mechanism of high-temperature superconductivity
journal, September 1997

Giant electron–phonon coupling of the breathing plane oxygen phonons in the dynamic stripe phase of $$\hbox {La}_{1.67}\hbox {Sr}_{0.33}\hbox {NiO}_4$$
journal, July 2020

Electronic liquid-crystal phases of a doped Mott insulator
journal, June 1998

Resonant elastic soft x-ray scattering
journal, April 2013

Stacked charge stripes in the quasi-2D trilayer nickelate La ₄ Ni ₃ O ₈
journal, July 2016

Charge modulations in ${La}_{2 - x}$ ${Sr}_{x}$ ${NiO}_{4 + y}$ : Ordering of polarons
journal, October 1993

Orbital Ordering, New Phases, and Stripe Formation in Doped Layered Nickelates
journal, June 2004

Oxygen and strontium codoping of ${La}_{2} Ni O_{4}$ : Room-temperature phase diagrams
journal, August 2004

Formation of Incommensurate Charge Density Waves in Cuprates
journal, September 2019

Magnon spintronics
journal, June 2015

Simultaneous Ordering of Holes and Spins in ${La}_{2}$ Ni $O_{4.125}$
journal, August 1994

Microscopic origin of diagonal stripe phases in doped nickelates
journal, March 2006

Evidence for stripe correlations of spins and holes in copper oxide superconductors
journal, June 1995

Bond-Stretching-Phonon Anomalies in Stripe-Ordered ${La}_{1.69} {Sr}_{0.31} {NiO}_{4}$
journal, January 2002

Freezing electronic correlations by polaronic instabilities in doped ${La}_{2}$ ${NiO}_{4}$
journal, September 1994

X-Ray Intensity Fluctuation Spectroscopy Observations of Critical Dynamics in Fe3Al
journal, March 1995

Colloquium : Theory of intertwined orders in high temperature superconductors
journal, May 2015

Remarkable Stability of Charge Density Wave Order in ${La}_{1.875} {Ba}_{0.125} {CuO}_{4}$
journal, October 2016

Evidence for a Nematic Phase in ${La}_{1.75} {Sr}_{0.25} {NiO}_{4}$
journal, April 2017

Hole concentration dependence of the ordering process of the stripe order in La2-xSrxNiO4
journal, September 2001

Large orbital polarization in a metallic square-planar nickelate
journal, June 2017

Resonant X-Ray Scattering Studies of Charge Order in Cuprates
journal, March 2016

Charge density wave memory in a cuprate superconductor
journal, March 2019

Magnetization of ${La}_{2 - x} {Sr}_{x} Ni O_{4 + δ}$ $(0 ⩽ x ⩽ 0.5)$ : Spin-glass and memory effects
journal, January 2006

Static charge-density-wave order in the superconducting state of ${La}_{2 - x} {Ba}_{x} {CuO}_{4}$
journal, June 2017

Superconductivity in an infinite-layer nickelate
journal, August 2019

Stripe Conductivity in ${La}_{1.775} {Sr}_{0.225} {NiO}_{4}$
journal, April 2000

Spectroscopy of Stripe Order in ${La}_{1.8} {Sr}_{0.2} {NiO}_{4}$ Using Resonant Soft X-Ray Diffraction
journal, October 2005

The Physics of Pair-Density Waves: Cuprate Superconductors and Beyond
journal, March 2020

Incommensurate charge stripe ordering in ${La}_{2 - x} {Sr}_{x} Ni O_{4}$ for $x = (0.33, 0.30, 0.275)$
journal, October 2004

Stripe order at low temperatures in ${La}_{2 - x} {Sr}_{x} {NiO}_{4}$ with $0.289 ≲ x ≲ 0.5$
journal, January 2000

Evidence for Short-Range-Ordered Charge Stripes Far above the Charge-Ordering Transition in ${La}_{1.67} {Sr}_{0.33} {NiO}_{4}$
journal, August 2013

Charge and canted spin order in ${La}_{2 - x} {Sr}_{x} {NiO}_{4}$ $(x = 0.275$ and $\frac{1}{3})$
journal, January 2001

Charge and spin ordering in ${La}_{2 - x}$ ${Sr}_{x}$ ${NiO}_{4.00}$ with x =0.135 and 0.20
journal, May 1995

Melting of Quasi-Two-Dimensional Charge Stripes in ${La}_{5 / 3} {Sr}_{1 / 3} {NiO}_{4}$
journal, September 1997

Stripe order and magnetic transitions in ${La}_{2 - x} {Sr}_{x} {NiO}_{4}$
journal, July 2004

X-ray scattering studies of charge stripes in La2−xSrxNiO4 (x=0.20−0.33)
journal, June 2002

Charge-ordered states in (La,Sr $)_{2}$ ${NiO}_{4}$ for hole concentrations $n_{h}$ =1/3 and 1/2
journal, March 1994

Doping a Mott insulator: Physics of high-temperature superconductivity
journal, January 2006

Growth of large La2–xSrxNiO4+δ single crystals by the floating-zone technique
journal, April 2002