Neutron scattering study of spin ordering and stripe pinning in superconducting La1.93Sr0.07CuO4

Jacobsen, H.; Zaliznyak, I. A.; Savici, A. T.; Winn, B. L.; Chang, S.; Hücker, M.; Gu, G. D.; Tranquada, J. M.

doi:10.1103/PhysRevB.92.174525

Title: Neutron scattering study of spin ordering and stripe pinning in superconducting ${La}_{1.93} {Sr}_{0.07} {CuO}_{4}$

Journal Article · 19 November 2015 · Physical Review. B, Condensed Matter and Materials Physics

DOI: https://doi.org/10.1103/PhysRevB.92.174525 · OSTI ID:1240590

Jacobsen, H. ^[1]; Zaliznyak, I. A. ^[1]; Savici, A. T. ^[2]; Winn, B. L. ^[2]; Chang, S. ^[3]; Hücker, M. ^[1]; Gu, G. D. ^[1]; Tranquada, J. M. ^[1]

Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)

The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in ${La}_{1.93} {Sr}_{0.07} {CuO}_{4}$ a superconductor with a transition temperature of T_c = 20 K. At T<< T_c, we find incommensurate spin fluctuations with a quasielastic energy spectrum and no sign of a gap within the energy range from 0.2 to 15 meV. A weak elastic magnetic component grows below ~ 10 K, consistent with results from local probes. Regarding the atomic lattice, we have discovered unexpectedly strong fluctuations of the CuO₆octahedra about Cu-O bonds, which are associated with inequivalent O sites within the CuO₂ planes. Moreover, we observed a weak elastic (3 ^⁻30) superlattice peak that implies a reduced lattice symmetry. The presence of inequivalent O sites rationalizes various pieces of evidence for charge stripe order in underdoped La_2-xSr_xCuO₄. The coexistence of superconductivity with quasi-static spin-stripe order suggests the presence of intertwined orders; however, the rotation of the stripe orientation away from the Cu-O bonds might be connected with evidence for a finite gap at the nodal points of the superconducting gap function.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). High Flux Isotope Reactor (HFIR); Spallation Neutron Source

Sponsoring Organization:: USDOE Office of Science (SC); USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1240590

Report Number(s):: BNL-111750-2016-JA; KC0201060

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Journal Name: Physical Review. B, Condensed Matter and Materials Physics Journal Issue: 17 Vol. 92; ISSN 1098-0121; ISSN PRBMDO

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Colloquium : Theory of intertwined orders in high temperature superconductors Fradkin, Eduardo; Kivelson, Steven A.; Tranquada, John M. Reviews of Modern Physics, Vol. 87, Issue 2 https://doi.org/10.1103/RevModPhys.87.457	journal	May 2015
Structural and superconducting properties of La 2 − x Sr x CuO 4 as a function of Sr content Radaelli, P. G.; Hinks, D. G.; Mitchell, A. W. Physical Review B, Vol. 49, Issue 6 https://doi.org/10.1103/physrevb.49.4163	journal	February 1994
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Low-temperature structural transitions and T c suppression in La 2 − x M x CuO 4 ( M =Ba, Sr) Koyama, Y.; Wakabayashi, Y.; Ito, K. Physical Review B, Vol. 51, Issue 14 https://doi.org/10.1103/physrevb.51.9045	journal	April 1995
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High-resolution x-ray diffraction study of La 1.88 − y Sr 0.12 Nd y CuO 4 Moodenbaugh, A. R.; Wu, Lijun; Zhu, Yimei Physical Review B, Vol. 58, Issue 14 https://doi.org/10.1103/physrevb.58.9549	journal	October 1998
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Reconciliation of local and long-range tilt correlations in underdoped La 2 − x Ba x CuO 4 ( 0 ≤ x ≤ 0.155 ) Bozin, Emil S.; Zhong, Ruidan; Knox, Kevin R. Physical Review B, Vol. 91, Issue 5 https://doi.org/10.1103/physrevb.91.054521	journal	February 2015
Quasi-two-dimensional spin and phonon excitations in La 1.965 Ba 0.035 CuO 4 Wagman, J. J.; Parshall, D.; Stone, M. B. Physical Review B, Vol. 91, Issue 22 https://doi.org/10.1103/physrevb.91.224404	journal	June 2015
Towards a Two-Dimensional Superconducting State of La 2 − x Sr x CuO 4 in a Moderate External Magnetic Field Schafgans, A. A.; LaForge, A. D.; Dordevic, S. V. Physical Review Letters, Vol. 104, Issue 15 https://doi.org/10.1103/physrevlett.104.157002	journal	April 2010
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Stripe States with Spatially Oscillating d -Wave Superconductivity in the Two-Dimensional t − t ′ − J Model Himeda, A.; Kato, T.; Ogata, M. Physical Review Letters, Vol. 88, Issue 11 https://doi.org/10.1103/physrevlett.88.117001	journal	February 2002
Magnetic-Field-Induced Localization of Quasiparticles in Underdoped L a 2 − x S r x C u O 4 Single Crystals Sun, X. F.; Komiya, Seiki; Takeya, J. Physical Review Letters, Vol. 90, Issue 11 https://doi.org/10.1103/physrevlett.90.117004	journal	March 2003
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Dimensional Crossover and Charge Order in Half-Doped Manganites and Cobaltites Zachar, Oron; Zaliznyak, Igor Physical Review Letters, Vol. 91, Issue 3 https://doi.org/10.1103/physrevlett.91.036401	journal	July 2003
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Dispersive Excitations in the High-Temperature Superconductor L a 2 − x S r x C u O 4 Christensen, N. B.; McMorrow, D. F.; Rønnow, H. M. Physical Review Letters, Vol. 93, Issue 14 https://doi.org/10.1103/physrevlett.93.147002	journal	September 2004
Theory of Incommensurate Magnetic Correlations Across the Insulator-Superconductor Transition of Underdoped La 2 − x Sr x CuO 4 Sushkov, Oleg P.; Kotov, Valeri N. Physical Review Letters, Vol. 94, Issue 9 https://doi.org/10.1103/physrevlett.94.097005	journal	March 2005
Magic Doping Fractions for High-Temperature Superconductors Komiya, Seiki; Chen, Han-Dong; Zhang, Shou-Cheng Physical Review Letters, Vol. 94, Issue 20 https://doi.org/10.1103/physrevlett.94.207004	journal	May 2005
Magnetic-Field-Induced Spin Excitations and Renormalized Spin Gap of the Underdoped La 1.895 Sr 0.105 CuO 4 Superconductor Chang, J.; Schnyder, A. P.; Gilardi, R. Physical Review Letters, Vol. 98, Issue 7 https://doi.org/10.1103/physrevlett.98.077004	journal	February 2007
Two-Dimensional Superconducting Fluctuations in Stripe-Ordered La 1.875 Ba 0.125 CuO 4 Li, Q.; Hücker, M.; Gu, G. D. Physical Review Letters, Vol. 99, Issue 6 https://doi.org/10.1103/physrevlett.99.067001	journal	August 2007
Dynamical Layer Decoupling in a Stripe-Ordered High- T c Superconductor Berg, E.; Fradkin, E.; Kim, E. -A. Physical Review Letters, Vol. 99, Issue 12 https://doi.org/10.1103/physrevlett.99.127003	journal	September 2007
Spin- and Pair-Density-Wave Glasses Mross, David F.; Senthil, T. Physical Review X, Vol. 5, Issue 3 https://doi.org/10.1103/physrevx.5.031008	journal	July 2015
Magnetic, transport, and optical properties of monolayer copper oxides Kastner, M. A.; Birgeneau, R. J.; Shirane, G. Reviews of Modern Physics, Vol. 70, Issue 3 https://doi.org/10.1103/revmodphys.70.897	journal	July 1998
Pairing symmetry in cuprate superconductors Tsuei, C. C.; Kirtley, J. R. Reviews of Modern Physics, Vol. 72, Issue 4, p. 969-1016 https://doi.org/10.1103/revmodphys.72.969	journal	October 2000
A common thread: The pairing interaction for unconventional superconductors Scalapino, D. J. Reviews of Modern Physics, Vol. 84, Issue 4 https://doi.org/10.1103/revmodphys.84.1383	journal	October 2012
Colloquium : Theory of intertwined orders in high temperature superconductors Fradkin, Eduardo; Kivelson, Steven A.; Tranquada, John M. Reviews of Modern Physics, Vol. 87, Issue 2 https://doi.org/10.1103/revmodphys.87.457	journal	May 2015
Quantum Impurities in the Two-Dimensional Spin One-Half Heisenberg Antiferromagnet Vajk, O. P. Science, Vol. 295, Issue 5560 https://doi.org/10.1126/science.1067110	journal	March 2002
The Ground State of the Pseudogap in Cuprate Superconductors Valla, T.; Fedorov, A. V.; Lee, Jinho Science, Vol. 314, Issue 5807 https://doi.org/10.1126/science.1134742	journal	November 2006
Thermal conductivity and competing orders in d-wave superconductors Gusynin, V. P.; Miransky, V. A. The European Physical Journal B - Condensed Matter, Vol. 37, Issue 3 https://doi.org/10.1140/epjb/e2004-00067-3	journal	February 2003
Energy Spectrum of Spin Fluctuations in Superconducting La _{2 - x} Sr _x CuO ₄ ( 0.10 ≤ x ≤ 0.25 ) Lee, Chul-Ho; Yamada, Kazuyoshi; Endoh, Yasuo Journal of the Physical Society of Japan, Vol. 69, Issue 4 https://doi.org/10.1143/JPSJ.69.1170	journal	April 2000
Structural Instability Associated with the Tilting of CuO ₆ Octahedra in La _{2 - x} Sr _x CuO ₄ Kimura, Hiroyuki; Hirota, Kazuma; Lee, Chul-Ho Journal of the Physical Society of Japan, Vol. 69, Issue 3 https://doi.org/10.1143/JPSJ.69.851	journal	March 2000
Spin Fluctuations in the Underdoped High- T _c Cuprate La _1.93 Sr _0.07 CuO ₄ Hiraka, Haruhiro; Endoh, Yasuo; Fujita, Masaki Journal of the Physical Society of Japan, Vol. 70, Issue 3 https://doi.org/10.1143/JPSJ.70.853	journal	March 2001
Quasiparticle Heat Transport in Mixed State of High- T _c Superconductors Takigawa, Mitsuaki; Ichioka, Masanori; Machida, Kazushige Journal of the Physical Society of Japan, Vol. 73, Issue 8 https://doi.org/10.1143/JPSJ.73.2049	journal	August 2004
Neutron Scattering Study of Soft Phonons and Diffuse Scattering in Insulating La _1.95 Sr _0.05 CuO ₄ Wakimoto, Shuichi; Lee, Seunghun; M. Gehring, Peter Journal of the Physical Society of Japan, Vol. 73, Issue 12 https://doi.org/10.1143/JPSJ.73.3413	journal	December 2004
Energy Spectrum of Spin Fluctuations in Superconducting La _{2 - x} Sr _x CuO ₄ ( 0.10 ≤ x ≤ 0.25 ) Lee, Chul-Ho; Yamada, Kazuyoshi; Endoh, Yasuo Journal of the Physical Society of Japan, Vol. 69, Issue 4 https://doi.org/10.1143/jpsj.69.1170	journal	April 2000
Quasiparticle Heat Transport in Mixed State of High- T _c Superconductors Takigawa, Mitsuaki; Ichioka, Masanori; Machida, Kazushige Journal of the Physical Society of Japan, Vol. 73, Issue 8 https://doi.org/10.1143/jpsj.73.2049	journal	August 2004
Neutron Scattering Study of Soft Phonons and Diffuse Scattering in Insulating La _1.95 Sr _0.05 CuO ₄ Wakimoto, Shuichi; Lee, Seunghun; M. Gehring, Peter Journal of the Physical Society of Japan, Vol. 73, Issue 12 https://doi.org/10.1143/jpsj.73.3413	journal	December 2004
“Nodal Gap” Induced by the Incommensurate Diagonal Spin Density Modulation in Underdoped High- T c Superconductors Zhou, Tao; Gao, Yi; Zhu, Jian-Xin Advances in Condensed Matter Physics, Vol. 2015 https://doi.org/10.1155/2015/652424	journal	January 2015
Unusual Magnetic Susceptibility Anisotropy in Untwinned La2xSrxCuO4 Single Crystals in the Lightly Doped Region Ando, Yoichi; Komiya, Seiki; Lavrov, A. N. The American Physical Society https://doi.org/10.17877/de290r-6417	text	January 2001
NMR study on the local structure in La-based high-Tc cuprates Goto, T.; Tonishi, J.; Suzuki, T. arXiv https://doi.org/10.48550/arxiv.0802.3240	text	January 2008
Theory of the striped superconductor Berg, Erez; Fradkin, Eduardo; Kivelson, Steven A. arXiv https://doi.org/10.48550/arxiv.0810.1564	text	January 2008
Energy gaps in the failed high-Tc superconductor La1.875Ba0.125CuO4 He, Rui-Hua; Tanaka, Kiyohisa; Mo, Sung-Kwan arXiv https://doi.org/10.48550/arxiv.0812.3882	text	January 2008
Charge $4e$ superconductivity from pair density wave order in certain high temperature superconductors Berg, E.; Fradkin, E.; Kivelson, S. A. arXiv https://doi.org/10.48550/arxiv.0904.1230	text	January 2009
Competing states in the t-J model: uniform d-wave state versus stripe state Corboz, Philippe; Rice, T. M.; Troyer, Matthias arXiv https://doi.org/10.48550/arxiv.1402.2859	text	January 2014
The geometric order of stripes and Luttinger liquids Zaanen, J.; Osman, O. Y.; Kruis, H. V. arXiv https://doi.org/10.48550/arxiv.cond-mat/0102103	text	January 2001
Spin Fluctuations in the Underdoped High-Tc Cuprate La1.93Sr0.07CuO4 Hiraka, H.; Endoh, Y.; Fujita, M. arXiv https://doi.org/10.48550/arxiv.cond-mat/0104087	text	January 2001
Dimensional cross-over and charge order in half-doped Manganites and Cobaltites Zachar, Oron; Zaliznyak, Igor arXiv https://doi.org/10.48550/arxiv.cond-mat/0112240	text	January 2001
Quantum Impurities in the Two-Dimensional Spin One-Half Heisenberg Antiferromagnet Vajk, O. P.; Mang, P. K.; Greven, M. arXiv https://doi.org/10.48550/arxiv.cond-mat/0203141	text	January 2002
Thermal Conductivity across the Phase Diagram of Cuprates: Low-Energy Quasiparticles and Doping Dependence of the Superconducting Gap Sutherland, Mike; Hawthorn, D. G.; Hill, R. W. arXiv https://doi.org/10.48550/arxiv.cond-mat/0301105	text	January 2003
Heat transport of La$_{2-y}$Eu$_y$CuO$_4$ and La$_{1.88-y}$Eu$_y$Sr$_{0.12}$CuO$_4$ single crystals Sun, X. F.; Komiya, Seiki; Ando, Yoichi arXiv https://doi.org/10.48550/arxiv.cond-mat/0304126	text	January 2003
Quasiparticle heat transport in the mixed state of high $T_c$ superconductors Takigawa, Mitsuaki; Ichioka, Masanori; Machida, Kazushige arXiv https://doi.org/10.48550/arxiv.cond-mat/0306492	text	January 2003
Neutron scattering study of soft phonons and diffuse scattering in insulating La$_{1.95}$Sr$_{0.05}$CuO$_{4}$ Wakimoto, Shuichi; Lee, Seunghun; Gehring, Peter M. arXiv https://doi.org/10.48550/arxiv.cond-mat/0408519	text	January 2004
The effect of collective spin-1 excitations on electronic spectra in high-Tc superconductors Eschrig, Matthias arXiv https://doi.org/10.48550/arxiv.cond-mat/0510286	text	January 2005
Distinguishing Patterns of Charge Order: Stripes or Checkerboards Robertson, John A.; Kivelson, Steven A.; Fradkin, Eduardo arXiv https://doi.org/10.48550/arxiv.cond-mat/0602675	text	January 2006
The Ground State of the Pseudogap in Cuprate Superconductors Valla, T.; Fedorov, A. V.; Lee, Jinho arXiv https://doi.org/10.48550/arxiv.cond-mat/0612672	text	January 2006
Direct Observation of a One Dimensional Static Spin Modulation in Insulating La1.95Sr0.05CuO4 Wakimoto, S.; Birgeneau, R. J.; Kastner, M. A. arXiv https://doi.org/10.48550/arxiv.cond-mat/9908115	text	January 1999
Impurity-Induced Quasiparticle Transport and Universal Limit Wiedemann-Franz Violation in d-Wave Superconductors Durst, A. C.; Lee, P. A. arXiv https://doi.org/10.48550/arxiv.cond-mat/9908182	text	January 1999

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Pairing Symmetry, Nodal and Antinodal Superconducting Gap in $$\text {La}_{2-x}\text {Sr}_x\text {CuO}_{4}$$: A Doping Scenario Verma, Sanjeev K.; Gupta, Anushri; Kumari, Anita Journal of Low Temperature Physics, Vol. 196, Issue 5-6 https://doi.org/10.1007/s10909-019-02199-2	journal	May 2019
Charge-screening role of c -axis atomic displacements in YBa 2 Cu 3 O 6 + x and related superconductors Božin, E. S.; Huq, A.; Shen, Bing Physical Review B, Vol. 93, Issue 5 https://doi.org/10.1103/physrevb.93.054523	journal	February 2016
Staging superstructures in high- T c Sr/O codoped La 2 − x Sr x CuO 4 + y Ray, P. J.; Andersen, N. H.; Jensen, T. B. S. Physical Review B, Vol. 96, Issue 17 https://doi.org/10.1103/physrevb.96.174106	journal	November 2017
Pair density waves in superconducting vortex halos Wang, Yuxuan; Edkins, Stephen D.; Hamidian, Mohammad H. Physical Review B, Vol. 97, Issue 17 https://doi.org/10.1103/physrevb.97.174510	journal	May 2018
Low-energy antiferromagnetic spin fluctuations limit the coherent superconducting gap in cuprates Li, Yangmu; Zhong, Ruidan; Stone, M. B. Physical Review B, Vol. 98, Issue 22 https://doi.org/10.1103/physrevb.98.224508	journal	December 2018
Remarkable Stability of Charge Density Wave Order in La 1.875 Ba 0.125 CuO 4 Chen, X. M.; Thampy, V.; Mazzoli, C. Physical Review Letters, Vol. 117, Issue 16 https://doi.org/10.1103/physrevlett.117.167001	journal	October 2016
Distinct Nature of Static and Dynamic Magnetic Stripes in Cuprate Superconductors Jacobsen, H.; Holm, S. L.; Lăcătuşu, M. -E. Physical Review Letters, Vol. 120, Issue 3 https://doi.org/10.1103/physrevlett.120.037003	journal	January 2018
Pair Density Waves in Superconducting Vortex Halos Wang, Yuxuan; Edkins, Stephen D.; Hamidian, Mohammad H. arXiv https://doi.org/10.48550/arxiv.1802.01582	text	January 2018
Low-energy antiferromagnetic spin fluctuations limit the coherent superconducting gap in cuprates Li, Yangmu; Zhong, Ruidan; Stone, M. B. arXiv https://doi.org/10.48550/arxiv.1806.10633	text	January 2018

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Title: Neutron scattering study of spin ordering and stripe pinning in superconducting ${La}_{1.93} {Sr}_{0.07} {CuO}_{4}$