Ultrafast optical switching and power limiting in intersubband polaritonic metasurfaces
Abstract
Highly nonlinear optical materials with fast third-order nonlinear optical response are crucial for the operation of all-optical photonic devices, such as switches for signal processing and computation, power limiters, and saturable absorbers. The nonlinear response of traditional optical materials is weak, thus requiring large light intensities to induce significant changes in their properties. Here we show that optical control of the coupling rate in subwavelength patch antennas coupled to intersubband transitions in multi-quantum-well semiconductor heterostructures can provide a giant third-order nonlinear response, on the order of , with a response time . We utilize this effect to realize intersubband polaritonic metasurfaces and demonstrate their operation as highly nonlinear saturable and reverse saturable absorbers, enabling optical power limiters and other elements for all-optical modulation and control. Our approach enables a plethora of compact, low-power, highly nonlinear devices with spectral, temporal, and structured wavefront responses tailored by design.
- Authors:
- Publication Date:
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1779953
- Grant/Contract Number:
- NA0003525
- Resource Type:
- Published Article
- Journal Name:
- Optica
- Additional Journal Information:
- Journal Name: Optica Journal Volume: 8 Journal Issue: 5; Journal ID: ISSN 2334-2536
- Publisher:
- Optical Society of America
- Country of Publication:
- United States
- Language:
- English
Citation Formats
Mann, Sander A., Nookala, Nishant, Johnson, Samuel C., Cotrufo, Michele, Mekawy, Ahmed, Klem, John F., Brener, Igal, Raschke, Markus B., Alù, Andrea, and Belkin, Mikhail A. Ultrafast optical switching and power limiting in intersubband polaritonic metasurfaces. United States: N. p., 2021.
Web. doi:10.1364/OPTICA.415581.
Mann, Sander A., Nookala, Nishant, Johnson, Samuel C., Cotrufo, Michele, Mekawy, Ahmed, Klem, John F., Brener, Igal, Raschke, Markus B., Alù, Andrea, & Belkin, Mikhail A. Ultrafast optical switching and power limiting in intersubband polaritonic metasurfaces. United States. https://doi.org/10.1364/OPTICA.415581
Mann, Sander A., Nookala, Nishant, Johnson, Samuel C., Cotrufo, Michele, Mekawy, Ahmed, Klem, John F., Brener, Igal, Raschke, Markus B., Alù, Andrea, and Belkin, Mikhail A. Thu .
"Ultrafast optical switching and power limiting in intersubband polaritonic metasurfaces". United States. https://doi.org/10.1364/OPTICA.415581.
@article{osti_1779953,
title = {Ultrafast optical switching and power limiting in intersubband polaritonic metasurfaces},
author = {Mann, Sander A. and Nookala, Nishant and Johnson, Samuel C. and Cotrufo, Michele and Mekawy, Ahmed and Klem, John F. and Brener, Igal and Raschke, Markus B. and Alù, Andrea and Belkin, Mikhail A.},
abstractNote = {Highly nonlinear optical materials with fast third-order nonlinear optical response are crucial for the operation of all-optical photonic devices, such as switches for signal processing and computation, power limiters, and saturable absorbers. The nonlinear response of traditional optical materials is weak, thus requiring large light intensities to induce significant changes in their properties. Here we show that optical control of the coupling rate in subwavelength patch antennas coupled to intersubband transitions in multi-quantum-well semiconductor heterostructures can provide a giant third-order nonlinear response, on the order of 3.4 × <#comment/> 10 − <#comment/> 13 m 2 / V 2 , with a response time < <#comment/> 2 p s . We utilize this effect to realize intersubband polaritonic metasurfaces and demonstrate their operation as highly nonlinear saturable and reverse saturable absorbers, enabling optical power limiters and other elements for all-optical modulation and control. Our approach enables a plethora of compact, low-power, highly nonlinear devices with spectral, temporal, and structured wavefront responses tailored by design.},
doi = {10.1364/OPTICA.415581},
journal = {Optica},
number = 5,
volume = 8,
place = {United States},
year = {Thu Apr 29 00:00:00 EDT 2021},
month = {Thu Apr 29 00:00:00 EDT 2021}
}
https://doi.org/10.1364/OPTICA.415581
Works referenced in this record:
Gradient Nonlinear Pancharatnam-Berry Metasurfaces
journal, November 2015
- Tymchenko, Mykhailo; Gomez-Diaz, J. Sebastian; Lee, Jongwon
- Physical Review Letters, Vol. 115, Issue 20
Ultrastrong Light-Matter Coupling Regime with Polariton Dots
journal, November 2010
- Todorov, Y.; Andrews, A. M.; Colombelli, R.
- Physical Review Letters, Vol. 105, Issue 19
Coupled quantum well semiconductors with giant electric field tunable nonlinear optical properties in the infrared
journal, May 1994
- Capasso, F.; Sirtori, C.; Cho, A. Y.
- IEEE Journal of Quantum Electronics, Vol. 30, Issue 5
Resonantly Enhanced Second-Harmonic Generation Using III–V Semiconductor All-Dielectric Metasurfaces
journal, August 2016
- Liu, Sheng; Sinclair, Michael B.; Saravi, Sina
- Nano Letters, Vol. 16, Issue 9, p. 5426-5432
Nonlinear plasmonics
journal, November 2012
- Kauranen, Martti; Zayats, Anatoly V.
- Nature Photonics, Vol. 6, Issue 11
Saturation and bistability of defect-mode intersubband polaritons
journal, February 2015
- Zanotto, Simone; Bianco, Federica; Sorba, Lucia
- Physical Review B, Vol. 91, Issue 8
Femtosecond optical polarization switching using a cadmium oxide-based perfect absorber
journal, May 2017
- Yang, Yuanmu; Kelley, Kyle; Sachet, Edward
- Nature Photonics, Vol. 11, Issue 6
Ultrafast All-Optical Switching with Magnetic Resonances in Nonlinear Dielectric Nanostructures
journal, September 2015
- Shcherbakov, Maxim R.; Vabishchevich, Polina P.; Shorokhov, Alexander S.
- Nano Letters, Vol. 15, Issue 10
Thin Perfect Absorbers for Electromagnetic Waves: Theory, Design, and Realizations
journal, March 2015
- Ra’di, Y.; Simovski, C. R.; Tretyakov, S. A.
- Physical Review Applied, Vol. 3, Issue 3
Ultra-subwavelength resonators for high temperature high performance quantum detectors
journal, November 2016
- Palaferri, Daniele; Todorov, Yanko; Mottaghizadeh, Alireza
- New Journal of Physics, Vol. 18, Issue 11
Low-Power Absorption Saturation in Semiconductor Metasurfaces
journal, September 2019
- Zubyuk, Varvara V.; Vabishchevich, Polina P.; Shcherbakov, Maxim R.
- ACS Photonics, Vol. 6, Issue 11
Enhanced Nonlinear Refractive Index in -Near-Zero Materials
journal, June 2016
- Caspani, L.; Kaipurath, R. P. M.; Clerici, M.
- Physical Review Letters, Vol. 116, Issue 23
Large optical nonlinearity of indium tin oxide in its epsilon-near-zero region
journal, April 2016
- Alam, M. Z.; De Leon, I.; Boyd, R. W.
- Science, Vol. 352, Issue 6287
Theory of optical maser amplifiers
journal, July 1965
- Arecchi, F.; Bonifacio, R.
- IEEE Journal of Quantum Electronics, Vol. 1, Issue 4
Quantum Engineering of Optical Nonlinearities
journal, January 1996
- Rosencher, E.; Fiore, A.; Vinter, B.
- Science, Vol. 271, Issue 5246
Third order optical nonlinearity of graphene
journal, May 2014
- Cheng, J. L.; Vermeulen, N.; Sipe, J. E.
- New Journal of Physics, Vol. 16, Issue 5
Strong Light-Matter Coupling in Subwavelength Metal-Dielectric Microcavities at Terahertz Frequencies
journal, May 2009
- Todorov, Y.; Andrews, A. M.; Sagnes, I.
- Physical Review Letters, Vol. 102, Issue 18
Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions
journal, July 2014
- Lee, Jongwon; Tymchenko, Mykhailo; Argyropoulos, Christos
- Nature, Vol. 511, Issue 7507
Ultrafast Manipulation of Strong Coupling in Metal−Molecular Aggregate Hybrid Nanostructures
journal, November 2010
- Vasa, P.; Pomraenke, R.; Cirmi, G.
- ACS Nano, Vol. 4, Issue 12
Tuning optical properties of metasurface via piezoelectric effect
journal, June 2019
- Mekawy, Ahmed; Khalifa, Mohammad; Ali, Tamer A.
- IET Optoelectronics, Vol. 13, Issue 3
Enhanced optical nonlinearities in the near-infrared using III-nitride heterostructures coupled to metamaterials
journal, October 2015
- Wolf, Omri; Allerman, Andrew A.; Ma, Xuedan
- Applied Physics Letters, Vol. 107, Issue 15, Article No. 151108
Light Propagation with Phase Discontinuities: Generalized Laws of Reflection and Refraction
journal, September 2011
- Yu, N.; Genevet, P.; Kats, M. A.
- Science, Vol. 334, Issue 6054
Ultrafast optical bleaching of intersubband cavity polaritons
journal, November 2012
- Zanotto, Simone; Degl'Innocenti, Riccardo; Xu, Ji-Hua
- Physical Review B, Vol. 86, Issue 20
Resonant Nanophotonic Spectrum Splitting for Ultrathin Multijunction Solar Cells
journal, July 2015
- Mann, Sander A.; Garnett, Erik C.
- ACS Photonics, Vol. 2, Issue 7
Thermalization and Cooling of Plasmon-Exciton Polaritons: Towards Quantum Condensation
journal, October 2013
- Rodriguez, S. R. K.; Feist, J.; Verschuuren, M. A.
- Physical Review Letters, Vol. 111, Issue 16
Nonlinear epsilon-near-zero materials explained: opinion
journal, January 2019
- Kinsey, N.; Khurgin, J.
- Optical Materials Express, Vol. 9, Issue 7
Observation of large second order susceptibility via intersubband transitions at λ∼10 μm in asymmetric coupled AlInAs/GaInAs quantum wells
journal, October 1991
- Sirtori, Carlo; Capasso, Federico; Sivco, Deborah L.
- Applied Physics Letters, Vol. 59, Issue 18
Emerging Low-Dimensional Materials for Nonlinear Optics and Ultrafast Photonics
journal, February 2017
- Liu, Xiaofeng; Guo, Qiangbing; Qiu, Jianrong
- Advanced Materials, Vol. 29, Issue 14
Transition from strong to ultrastrong coupling regime in mid-infrared metal-dielectric-metal cavities
journal, June 2011
- Jouy, P.; Vasanelli, A.; Todorov, Y.
- Applied Physics Letters, Vol. 98, Issue 23
Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in metal nanostructures with J-aggregates
journal, January 2013
- Vasa, Parinda; Wang, Wei; Pomraenke, Robert
- Nature Photonics, Vol. 7, Issue 2
Nonlinear processes in multi-quantum-well plasmonic metasurfaces: Electromagnetic response, saturation effects, limits, and potentials
journal, September 2015
- Gomez-Diaz, J. S.; Tymchenko, M.; Lee, J.
- Physical Review B, Vol. 92, Issue 12
Self-Induced Transparency by Pulsed Coherent Light
journal, May 1967
- McCall, S. L.; Hahn, E. L.
- Physical Review Letters, Vol. 18, Issue 21
Quantum Plexcitonics: Strongly Interacting Plasmons and Excitons
journal, May 2011
- Manjavacas, A.; García de Abajo, F. J.; Nordlander, P.
- Nano Letters, Vol. 11, Issue 6
Semiconductor saturable absorber mirrors (SESAM's) for femtosecond to nanosecond pulse generation in solid-state lasers
journal, January 1996
- Keller, U.; Weingarten, K. J.; Kartner, F. X.
- IEEE Journal of Selected Topics in Quantum Electronics, Vol. 2, Issue 3
Theory of patch-antenna metamaterial perfect absorbers
journal, June 2016
- Bowen, Patrick T.; Baron, Alexandre; Smith, David R.
- Physical Review A, Vol. 93, Issue 6
Plexciton Dynamics: Exciton−Plasmon Coupling in a J-Aggregate−Au Nanoshell Complex Provides a Mechanism for Nonlinearity
journal, April 2011
- Fofang, Nche T.; Grady, Nathaniel K.; Fan, Zhiyuan
- Nano Letters, Vol. 11, Issue 4
Nonlinear Fano-Resonant Dielectric Metasurfaces
journal, October 2015
- Yang, Yuanmu; Wang, Wenyi; Boulesbaa, Abdelaziz
- Nano Letters, Vol. 15, Issue 11, p. 7388-7393
Ultrathin gradient nonlinear metasurface with a giant nonlinear response
journal, January 2016
- Nookala, Nishant; Lee, Jongwon; Tymchenko, Mykhailo
- Optica, Vol. 3, Issue 3
Nanostructured Plasmonic Medium for Terahertz Bandwidth All-Optical Switching
journal, October 2011
- Ren, Mengxin; Jia, Baohua; Ou, Jun-Yu
- Advanced Materials, Vol. 23, Issue 46
Ultrastrong coupling between light and matter
journal, January 2019
- Frisk Kockum, Anton; Miranowicz, Adam; De Liberato, Simone
- Nature Reviews Physics, Vol. 1, Issue 1
Microcavity Polariton Splitting of Intersubband Transitions
journal, March 2003
- Dini, Dimitri; Köhler, Rüdeger; Tredicucci, Alessandro
- Physical Review Letters, Vol. 90, Issue 11
Sub-cycle switch-on of ultrastrong light–matter interaction
journal, March 2009
- Günter, G.; Anappara, A. A.; Hees, J.
- Nature, Vol. 458, Issue 7235
Non-linear population processes of Er3+ laser levels in chromium-doped garnet crystals
journal, July 1990
- Noginov, M. A.; Smirnov, V. A.; Shcherbakov, I. A.
- Optical and Quantum Electronics, Vol. 22, Issue S1
Second-order nonlinear effects in asymmetric quantum-well structures
journal, August 1988
- Khurgin, J.
- Physical Review B, Vol. 38, Issue 6
Ultrafast Nonlinear Optical Response of a Single Gold Nanorod near Its Surface Plasmon Resonance
journal, July 2011
- Baida, H.; Mongin, D.; Christofilos, D.
- Physical Review Letters, Vol. 107, Issue 5
Large optical nonlinearity of nanoantennas coupled to an epsilon-near-zero material
journal, January 2018
- Alam, M. Zahirul; Schulz, Sebastian A.; Upham, Jeremy
- Nature Photonics, Vol. 12, Issue 2
Ultrathin Second‐Harmonic Metasurfaces with Record‐High Nonlinear Optical Response
journal, February 2016
- Lee, Jongwon; Nookala, Nishant; Gomez‐Diaz, J. Sebastian
- Advanced Optical Materials, Vol. 4, Issue 5
Transition from strong to weak coupling and the onset of lasing in semiconductor microcavities
journal, April 2002
- Butté, R.; Delalleau, G.; Tartakovskii, A. I.
- Physical Review B, Vol. 65, Issue 20
Subwavelength optical absorber with an integrated photon sorter
journal, March 2012
- Le Perchec, J.; Desieres, Y.; Rochat, N.
- Applied Physics Letters, Vol. 100, Issue 11
Strong coupling in the sub-wavelength limit using metamaterial nanocavities
journal, November 2013
- Benz, A.; Campione, S.; Liu, S.
- Nature Communications, Vol. 4, Article No. 2882
High-harmonic generation from an epsilon-near-zero material
journal, July 2019
- Yang, Yuanmu; Lu, Jian; Manjavacas, Alejandro
- Nature Physics, Vol. 15, Issue 10
Difference-Frequency Generation in Polaritonic Intersubband Nonlinear Metasurfaces
journal, August 2018
- Liu, Yingnan; Lee, Jongwon; March, Stephen
- Advanced Optical Materials, Vol. 6, Issue 20
Wide-angle perfect absorber/thermal emitter in the terahertz regime
journal, January 2009
- Diem, Marcus; Koschny, Thomas; Soukoulis, C. M.
- Physical Review B, Vol. 79, Issue 3