Design of 3D Oxide–Metal Hybrid Metamaterial for Tailorable Light–Matter Interactions in Visible and Near-Infrared Region
Abstract
Abstract Dielectric–metallic hybrid metamaterials exhibit extraordinary optical properties due to the light–matter interactions at the dielectric–metallic interfaces. The ability in precision control of the light–matter interactions in nanoscale is key to tailor the optical properties of hybrid metamaterials. In this work, a complex 3D framework of multilayered self‐assembled BaTiO 3 (BTO)‐Au hybrid thin films is demonstrated with such precision control of the light–matter interaction in nanoscale. Unique “bamboo‐like” Au nanostructures are formed via the bilayer and trilayer stacking of BTO‐Au hybrid layers with interlayers of SrTiO 3 , CeO 2 , or MgO. Different film strain states introduced by the three interlayers result in variable diameter and density of Au nanopillars. Both simulated and experimental optical data demonstrate the localized surface plasmon resonance change and hyperbolic dispersion wavelength shift in visible to near‐infrared because of the effective tuning of the Au nanopillar aspect ratio and free electron density. The highly tunable optical properties along with the ferroelectric behavior and thermal robustness of the 3D hybrid film enable it to be a great candidate for multifunctional applications. This study demonstrates a unique 3D approach for precision optical property tuning and combined functionalities in oxide–metal metamaterial systems toward future integrated photonic andmore »
- Authors:
-
[1]
- Purdue Univ., West Lafayette, IN (United States)
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Publication Date:
- Research Org.:
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA); US Department of the Navy, Office of Naval Research (ONR)
- OSTI Identifier:
- 1738926
- Alternate Identifier(s):
- OSTI ID: 1785770
- Report Number(s):
- SAND-2020-13468J
Journal ID: ISSN 2195-1071; 692709
- Grant/Contract Number:
- AC04-94AL85000; SC0020077; NA0003525; N00014-17-1-2087; N00014-20-1-2043
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Optical Materials
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2195-1071
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; Hybrid metamaterials; Multilayer; Localized surface plasmon resonance; Hyperbolic dispersion; Tunability
Citation Formats
Zhang, Di, Lu, Ping, Misra, Shikhar, Wissel, Ashley, He, Zihao, Qi, Zhimin, Gao, Xingyao, Sun, Xing, Liu, Juncheng, Lu, Juanjuan, Zhang, Xinghang, and Wang, Haiyan. Design of 3D Oxide–Metal Hybrid Metamaterial for Tailorable Light–Matter Interactions in Visible and Near-Infrared Region. United States: N. p., 2020.
Web. doi:10.1002/adom.202001154.
Zhang, Di, Lu, Ping, Misra, Shikhar, Wissel, Ashley, He, Zihao, Qi, Zhimin, Gao, Xingyao, Sun, Xing, Liu, Juncheng, Lu, Juanjuan, Zhang, Xinghang, & Wang, Haiyan. Design of 3D Oxide–Metal Hybrid Metamaterial for Tailorable Light–Matter Interactions in Visible and Near-Infrared Region. United States. https://doi.org/10.1002/adom.202001154
Zhang, Di, Lu, Ping, Misra, Shikhar, Wissel, Ashley, He, Zihao, Qi, Zhimin, Gao, Xingyao, Sun, Xing, Liu, Juncheng, Lu, Juanjuan, Zhang, Xinghang, and Wang, Haiyan. Sun .
"Design of 3D Oxide–Metal Hybrid Metamaterial for Tailorable Light–Matter Interactions in Visible and Near-Infrared Region". United States. https://doi.org/10.1002/adom.202001154. https://www.osti.gov/servlets/purl/1738926.
@article{osti_1738926,
title = {Design of 3D Oxide–Metal Hybrid Metamaterial for Tailorable Light–Matter Interactions in Visible and Near-Infrared Region},
author = {Zhang, Di and Lu, Ping and Misra, Shikhar and Wissel, Ashley and He, Zihao and Qi, Zhimin and Gao, Xingyao and Sun, Xing and Liu, Juncheng and Lu, Juanjuan and Zhang, Xinghang and Wang, Haiyan},
abstractNote = {Abstract Dielectric–metallic hybrid metamaterials exhibit extraordinary optical properties due to the light–matter interactions at the dielectric–metallic interfaces. The ability in precision control of the light–matter interactions in nanoscale is key to tailor the optical properties of hybrid metamaterials. In this work, a complex 3D framework of multilayered self‐assembled BaTiO 3 (BTO)‐Au hybrid thin films is demonstrated with such precision control of the light–matter interaction in nanoscale. Unique “bamboo‐like” Au nanostructures are formed via the bilayer and trilayer stacking of BTO‐Au hybrid layers with interlayers of SrTiO 3 , CeO 2 , or MgO. Different film strain states introduced by the three interlayers result in variable diameter and density of Au nanopillars. Both simulated and experimental optical data demonstrate the localized surface plasmon resonance change and hyperbolic dispersion wavelength shift in visible to near‐infrared because of the effective tuning of the Au nanopillar aspect ratio and free electron density. The highly tunable optical properties along with the ferroelectric behavior and thermal robustness of the 3D hybrid film enable it to be a great candidate for multifunctional applications. This study demonstrates a unique 3D approach for precision optical property tuning and combined functionalities in oxide–metal metamaterial systems toward future integrated photonic and electronic devices.},
doi = {10.1002/adom.202001154},
journal = {Advanced Optical Materials},
number = 1,
volume = 9,
place = {United States},
year = {Sun Nov 08 00:00:00 EST 2020},
month = {Sun Nov 08 00:00:00 EST 2020}
}
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