DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Attosecond Coherence Time Characterization in Hard X-Ray Free-Electron Laser

Abstract

One of the key challenges in scientific researches based on free-electron lasers (FELs) is the characterization of the coherence time of the ultra-fast hard x-ray pulse, which fundamentally influences the interaction process between x-rays and materials. Conventional optical methods, based on autocorrelation, are very difficult to realize due to the lack of mirrors. Here, we experimentally demonstrate a novel method which yields a coherence time of 174.7 attoseconds for the 6.92 keV FEL pulses at the Linac Coherent Light Source. In our experiment, a phase shifter is adopted to control the cross-correlation between x-ray and microbunched electrons. This approach provides critical diagnostics for the temporal coherence of x-ray FELs and is universal for general machine parameters; applicable for wide range of photon energy, radiation brightness, repetition rate and FEL pulse duration.

Authors:
; ; ; ; ORCiD logo; ORCiD logo; ORCiD logo; ; ; ; ; ; ; ; ORCiD logo
Publication Date:
Research Org.:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1619824
Alternate Identifier(s):
OSTI ID: 1623285
Grant/Contract Number:  
AC02-76SF00515; FWP-2013-SLAC-100164
Resource Type:
Published Article
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Name: Scientific Reports Journal Volume: 10 Journal Issue: 1; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United Kingdom
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS

Citation Formats

Zhou, Guanqun, Decker, Franz-Josef, Ding, Yuantao, Jiao, Yi, Lutman, Alberto A., Maxwell, Timothy J., Raubenheimer, Tor O., Wang, Jiuqing, Holman, Aaron J., Tsai, Cheng-Ying, Wu, Jerome Y., Wu, Weiwei, Yang, Chuan, Yoon, Moohyun, and Wu, Juhao. Attosecond Coherence Time Characterization in Hard X-Ray Free-Electron Laser. United Kingdom: N. p., 2020. Web. doi:10.1038/s41598-020-60328-4.
Zhou, Guanqun, Decker, Franz-Josef, Ding, Yuantao, Jiao, Yi, Lutman, Alberto A., Maxwell, Timothy J., Raubenheimer, Tor O., Wang, Jiuqing, Holman, Aaron J., Tsai, Cheng-Ying, Wu, Jerome Y., Wu, Weiwei, Yang, Chuan, Yoon, Moohyun, & Wu, Juhao. Attosecond Coherence Time Characterization in Hard X-Ray Free-Electron Laser. United Kingdom. https://doi.org/10.1038/s41598-020-60328-4
Zhou, Guanqun, Decker, Franz-Josef, Ding, Yuantao, Jiao, Yi, Lutman, Alberto A., Maxwell, Timothy J., Raubenheimer, Tor O., Wang, Jiuqing, Holman, Aaron J., Tsai, Cheng-Ying, Wu, Jerome Y., Wu, Weiwei, Yang, Chuan, Yoon, Moohyun, and Wu, Juhao. Mon . "Attosecond Coherence Time Characterization in Hard X-Ray Free-Electron Laser". United Kingdom. https://doi.org/10.1038/s41598-020-60328-4.
@article{osti_1619824,
title = {Attosecond Coherence Time Characterization in Hard X-Ray Free-Electron Laser},
author = {Zhou, Guanqun and Decker, Franz-Josef and Ding, Yuantao and Jiao, Yi and Lutman, Alberto A. and Maxwell, Timothy J. and Raubenheimer, Tor O. and Wang, Jiuqing and Holman, Aaron J. and Tsai, Cheng-Ying and Wu, Jerome Y. and Wu, Weiwei and Yang, Chuan and Yoon, Moohyun and Wu, Juhao},
abstractNote = {One of the key challenges in scientific researches based on free-electron lasers (FELs) is the characterization of the coherence time of the ultra-fast hard x-ray pulse, which fundamentally influences the interaction process between x-rays and materials. Conventional optical methods, based on autocorrelation, are very difficult to realize due to the lack of mirrors. Here, we experimentally demonstrate a novel method which yields a coherence time of 174.7 attoseconds for the 6.92 keV FEL pulses at the Linac Coherent Light Source. In our experiment, a phase shifter is adopted to control the cross-correlation between x-ray and microbunched electrons. This approach provides critical diagnostics for the temporal coherence of x-ray FELs and is universal for general machine parameters; applicable for wide range of photon energy, radiation brightness, repetition rate and FEL pulse duration.},
doi = {10.1038/s41598-020-60328-4},
journal = {Scientific Reports},
number = 1,
volume = 10,
place = {United Kingdom},
year = {Mon Apr 06 00:00:00 EDT 2020},
month = {Mon Apr 06 00:00:00 EDT 2020}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1038/s41598-020-60328-4

Figures / Tables:

Figure 1 Figure 1: Schematic description of hard x-ray SASE FEL coherence time measurement based on crosscorrelation between microbunched electrons and x-ray pulse. Hard x-ray SASE FEL is generated in the beforedelay undulators, then a phase shifter is employed to generate a relative delay between the electrons and the x-ray and themore » final undulator converts the correlation to x-ray pulse energy. (a) Visualizing the radiation wave and the microbunched electrons at the beginning of the phase shifter. (b) Illustrating the case that the phase shifter induced delay is small. (c) Showing that when the delay is quite large, the microbunched electrons would work with x-rays in other coherence spikes.« less

Save / Share:

Works referenced in this record:

Single mimivirus particles intercepted and imaged with an X-ray laser
journal, February 2011

  • Seibert, M. Marvin; Ekeberg, Tomas; Maia, Filipe R. N. C.
  • Nature, Vol. 470, Issue 7332
  • DOI: 10.1038/nature09748

Spatio-temporal coherence of free electron laser pulses in the soft x-ray regime
journal, January 2008


Linac Coherent Light Source: The first five years
journal, March 2016


The European X-ray free-electron laser facility in Hamburg
journal, December 2011

  • Altarelli, M.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 269, Issue 24
  • DOI: 10.1016/j.nimb.2011.04.034

A compact X-ray free-electron laser emitting in the sub-ångström region
journal, June 2012


First Observation of Self-Amplified Spontaneous Emission in a Free-Electron Laser at 109 nm Wavelength
journal, October 2000


First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010


Free-Electron Laser Design for Four-Wave Mixing Experiments with Soft-X-Ray Pulses
journal, July 2014


A single-shot intensity-position monitor for hard x-ray FEL sources
conference, September 2011

  • Feng, Yiping; Feldkamp, Jan M.; Fritz, David M.
  • SPIE Optical Engineering + Applications, SPIE Proceedings
  • DOI: 10.1117/12.893740

Spectrum, temporal structure, and fluctuations in a high-gain free-electron laser starting from noise
journal, July 1994


GENESIS 1.3: a fully 3D time-dependent FEL simulation code
journal, June 1999

  • Reiche, S.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 429, Issue 1-3
  • DOI: 10.1016/S0168-9002(99)00114-X

Temporal and spatial coherence properties of free-electron-laser pulses in the extreme ultraviolet regime
journal, August 2011

  • Roling, S.; Siemer, B.; Wöstmann, M.
  • Physical Review Special Topics - Accelerators and Beams, Vol. 14, Issue 8
  • DOI: 10.1103/PhysRevSTAB.14.080701

Tracking excited-state charge and spin dynamics in iron coordination complexes
journal, May 2014

  • Zhang, Wenkai; Alonso-Mori, Roberto; Bergmann, Uwe
  • Nature, Vol. 509, Issue 7500
  • DOI: 10.1038/nature13252

Demonstration of self-seeding in a hard-X-ray free-electron laser
journal, August 2012


Femtosecond electronic response of atoms to ultra-intense X-rays
journal, July 2010


Hard X-ray free-electron laser with femtosecond-scale timing jitter
journal, October 2017


Femtosecond X-Ray Pulse Characterization in Free-Electron Lasers Using a Cross-Correlation Technique
journal, December 2012


Transform-Limited X-Ray Pulse Generation from a High-Brightness Self-Amplified Spontaneous-Emission Free-Electron Laser
journal, March 2013


SwissFEL: The Swiss X-ray Free Electron Laser
journal, July 2017

  • Milne, Christopher; Schietinger, Thomas; Aiba, Masamitsu
  • Applied Sciences, Vol. 7, Issue 7
  • DOI: 10.3390/app7070720

Lensless imaging of magnetic nanostructures by X-ray spectro-holography
journal, December 2004

  • Eisebitt, S.; Lüning, J.; Schlotter, W. F.
  • Nature, Vol. 432, Issue 7019
  • DOI: 10.1038/nature03139

Collective instabilities and high-gain regime in a free electron laser
journal, July 1984


Purified self-amplified spontaneous emission free-electron lasers with slippage-boosted filtering
journal, January 2013

  • Xiang, Dao; Ding, Yuantao; Huang, Zhirong
  • Physical Review Special Topics - Accelerators and Beams, Vol. 16, Issue 1
  • DOI: 10.1103/PhysRevSTAB.16.010703

Femtosecond Visualization of Lattice Dynamics in Shock-Compressed Matter
journal, October 2013


Attosecond time–energy structure of X-ray free-electron laser pulses
journal, March 2018


High-Gain Harmonic-Generation Free-Electron Laser
journal, August 2000


Interplay of the chirps and chirped pulse compression in a high-gain seeded free-electron laser
journal, January 2007

  • Wu, Juhao; Murphy, James B.; Emma, Paul J.
  • Journal of the Optical Society of America B, Vol. 24, Issue 3
  • DOI: 10.1364/JOSAB.24.000484

Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.