Space- and time-resolved small angle X-ray scattering to probe assembly of silver nanocrystal superlattices

Yu, Yixuan; Yu, Dian; Sadigh, Babak; Orme, Christine A.

doi:10.1038/s41467-018-06734-9

Title: Space- and time-resolved small angle X-ray scattering to probe assembly of silver nanocrystal superlattices

Journal Article · 11 October 2018 · Nature Communications

DOI: https://doi.org/10.1038/s41467-018-06734-9 · OSTI ID:1619802

; Yu, Dian; Sadigh, Babak;

Abstract The structure of nanocrystal superlattices has been extensively studied and well documented, however, their assembly process is poorly understood. In this work, we demonstrate an in situ space- and time-resolved small angle X-ray scattering measurement that we use to probe the assembly of silver nanocrystal superlattices driven by electric fields. The electric field creates a nanocrystal flux to the surface, providing a systematic means to vary the nanocrystal concentration near the electrode and thereby to initiate nucleation and growth of superlattices in several minutes. Using this approach, we measure the space- and time-resolved concentration and polydispersity gradients during deposition and show how they affect the superlattice constant and degree of order. We find that the field induces a size-selection effect that can reduce the polydispersity near the substrate by 21% leading to better quality crystals and resulting in field strength-dependent superlattice lattice constants.

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Sponsoring Organization:: USDOE

OSTI ID:: 1619802

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 9; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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