Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution
Abstract
Abstract High harmonic generation of ultrafast laser pulses can be used to perform angle-resolved photoemission spectroscopy (ARPES) to map the electronic band structure of materials with femtosecond time resolution. However, currently it is difficult to reach high momenta with narrow energy resolution. Here, we combine a gas phase extreme ultraviolet (XUV) femtosecond light source, an XUV monochromator, and a time-of-flight electron analyzer to develop XUV-based time-resolved ARPES. Our technique can produce tunable photon energy between 24–33 eV with an unprecedented energy resolution of 30 meV and time resolution of 200 fs. This technique enables time-, energy- and momentum-resolved investigation of the nonequilibrium dynamics of electrons in materials with a full access to their first Brillouin zone. We evaluate the performance of this setup through exemplary measurements on various quantum materials, including WTe 2 , WSe 2 , TiSe 2 , and Bi 2 Sr 2 CaCu 2 O 8+δ .
- Publication Date:
- Research Org.:
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
- Sponsoring Org.:
- USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; US Army Research Office (ARO); Gordon and Betty Moore Foundation (GBMF)
- OSTI Identifier:
- 1619647
- Alternate Identifier(s):
- OSTI ID: 1624182
- Grant/Contract Number:
- GBMF4540
- Resource Type:
- Published Article
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Name: Nature Communications Journal Volume: 10 Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- 47 OTHER INSTRUMENTATION; science & technology
Citation Formats
Sie, Edbert J., Rohwer, Timm, Lee, Changmin, and Gedik, Nuh. Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution. United Kingdom: N. p., 2019.
Web. doi:10.1038/s41467-019-11492-3.
Sie, Edbert J., Rohwer, Timm, Lee, Changmin, & Gedik, Nuh. Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution. United Kingdom. https://doi.org/10.1038/s41467-019-11492-3
Sie, Edbert J., Rohwer, Timm, Lee, Changmin, and Gedik, Nuh. Tue .
"Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution". United Kingdom. https://doi.org/10.1038/s41467-019-11492-3.
@article{osti_1619647,
title = {Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution},
author = {Sie, Edbert J. and Rohwer, Timm and Lee, Changmin and Gedik, Nuh},
abstractNote = {Abstract High harmonic generation of ultrafast laser pulses can be used to perform angle-resolved photoemission spectroscopy (ARPES) to map the electronic band structure of materials with femtosecond time resolution. However, currently it is difficult to reach high momenta with narrow energy resolution. Here, we combine a gas phase extreme ultraviolet (XUV) femtosecond light source, an XUV monochromator, and a time-of-flight electron analyzer to develop XUV-based time-resolved ARPES. Our technique can produce tunable photon energy between 24–33 eV with an unprecedented energy resolution of 30 meV and time resolution of 200 fs. This technique enables time-, energy- and momentum-resolved investigation of the nonequilibrium dynamics of electrons in materials with a full access to their first Brillouin zone. We evaluate the performance of this setup through exemplary measurements on various quantum materials, including WTe 2 , WSe 2 , TiSe 2 , and Bi 2 Sr 2 CaCu 2 O 8+δ .},
doi = {10.1038/s41467-019-11492-3},
journal = {Nature Communications},
number = 1,
volume = 10,
place = {United Kingdom},
year = {2019},
month = {8}
}
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https://doi.org/10.1038/s41467-019-11492-3
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Cited by: 45 works
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Figures / Tables:
Fig. 1: XUV-based time-resolved ARPES setup overview. Inset (top-right) shows the experimental layout for high harmonic generation (HHG) of a near infrared (NIR) light through a hollow fiber filled with krypton gas to generate extreme ultraviolet (XUV) light
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