High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses

Lee, Changmin; Rohwer, Timm; Sie, Edbert J.; Zong, Alfred; Baldini, Edoardo; Straquadine, Joshua; Walmsley, Philip; Gardner, Dillon; Lee, Young S.; Fisher, Ian R.; Gedik, Nuh

doi:10.1063/1.5139556

Title: High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses

Abstract

Performing time- and angle-resolved photoemission (tr-ARPES) spectroscopy at high momenta necessitates extreme ultraviolet laser pulses, which are typically produced via high harmonic generation (HHG). Despite current advances, HHG-based setups still require large pulse energies (from hundreds of μJ to mJ) and their energy resolution is limited to tens of meV. Here, we present a novel 11 eV tr-ARPES setup that generates a flux of 5 × 10¹⁰ photons/s and achieves an unprecedented energy resolution of 16 meV. It can be operated at high repetition rates (up to 250 kHz) while using input pulse energies down to 3 µJ. We demonstrate these unique capabilities by simultaneously capturing the energy and momentum resolved dynamics in two well-separated momentum space regions of a charge density wave material ErTe₃. This novel setup provides the opportunity to study the non-equilibrium band structure of solids with exceptional energy and time resolutions at high repetition rates.

Authors:

^[1];

^[2];

^[3];

^[4];

^[5];

^[5]; Gardner, Dillon ^[4]; Lee, Young S. ^[6];

^[5];

^[4]

Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). Center for Free-Electron Laser Science
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)
Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Publication Date:: Thu Apr 09 00:00:00 EDT 2020

Research Org.:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); Gordon and Betty Moore Foundation; Army Research Office (ARO); Swiss National Science Foundation (SNSF)

OSTI Identifier:: 1616758

Alternate Identifier(s):: OSTI ID: 1616480

Grant/Contract Number:: FG02-08ER46521; AC02-76SF00515; GBMF4540; W911NF-15-1-0128

Resource Type:: Accepted Manuscript

Journal Name:: Review of Scientific Instruments

Additional Journal Information:: Journal Volume: 91; Journal Issue: 4; Journal ID: ISSN 0034-6748

Publisher:: American Institute of Physics (AIP)

Country of Publication:: United States

Language:: English

Subject:: 47 OTHER INSTRUMENTATION

Citation Formats


                    Lee, Changmin, Rohwer, Timm, Sie, Edbert J., Zong, Alfred, Baldini, Edoardo, Straquadine, Joshua, Walmsley, Philip, Gardner, Dillon, Lee, Young S., Fisher, Ian R., and Gedik, Nuh. High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses.  United States: N. p., 2020. 
Web.  doi:10.1063/1.5139556.

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                    Lee, Changmin, Rohwer, Timm, Sie, Edbert J., Zong, Alfred, Baldini, Edoardo, Straquadine, Joshua, Walmsley, Philip, Gardner, Dillon, Lee, Young S., Fisher, Ian R., & Gedik, Nuh. High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses.  United States.  https://doi.org/10.1063/1.5139556

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                    Lee, Changmin, Rohwer, Timm, Sie, Edbert J., Zong, Alfred, Baldini, Edoardo, Straquadine, Joshua, Walmsley, Philip, Gardner, Dillon, Lee, Young S., Fisher, Ian R., and Gedik, Nuh. Thu .  
"High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses".  United States.  https://doi.org/10.1063/1.5139556.  https://www.osti.gov/servlets/purl/1616758.

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@article{osti_1616758,

  title        = {High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses},

  author       = {Lee, Changmin and Rohwer, Timm and Sie, Edbert J. and Zong, Alfred and Baldini, Edoardo and Straquadine, Joshua and Walmsley, Philip and Gardner, Dillon and Lee, Young S. and Fisher, Ian R. and Gedik, Nuh},

  abstractNote = {Performing time- and angle-resolved photoemission (tr-ARPES) spectroscopy at high momenta necessitates extreme ultraviolet laser pulses, which are typically produced via high harmonic generation (HHG). Despite current advances, HHG-based setups still require large pulse energies (from hundreds of μJ to mJ) and their energy resolution is limited to tens of meV. Here, we present a novel 11 eV tr-ARPES setup that generates a flux of 5 × 1010 photons/s and achieves an unprecedented energy resolution of 16 meV. It can be operated at high repetition rates (up to 250 kHz) while using input pulse energies down to 3 µJ. We demonstrate these unique capabilities by simultaneously capturing the energy and momentum resolved dynamics in two well-separated momentum space regions of a charge density wave material ErTe3. This novel setup provides the opportunity to study the non-equilibrium band structure of solids with exceptional energy and time resolutions at high repetition rates.},

  doi          = {10.1063/1.5139556},

  journal      = {Review of Scientific Instruments},

  number       = 4,

  volume       = 91,

  place        = {United States},

  year         = {Thu Apr 09 00:00:00 EDT 2020},

  month        = {Thu Apr 09 00:00:00 EDT 2020}

}

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Title: High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses

Abstract

Citation Formats

A high-order harmonic generation apparatus for time- and angle-resolved photoelectron spectroscopy journal, July 2013

Coherent narrowband light source for ultrafast photoelectron spectroscopy in the 17–31 eV photon energy range journal, January 2020

Ultrafast extreme ultraviolet photoemission without space charge journal, September 2018

Full characterization and optimization of a femtosecond ultraviolet laser source for time and angle-resolved photoemission on solid surfaces journal, April 2012

Time-resolved photoemission apparatus achieving sub-20-meV energy resolution and high stability journal, December 2014

A versatile system for ultrahigh resolution, low temperature, and polarization dependent Laser-angle-resolved photoemission spectroscopy journal, January 2008

Collapse of long-range charge order tracked by time-resolved photoemission at high momenta journal, March 2011

Evidence for topological defects in a photoinduced phase transition journal, October 2018

Bright high-repetition-rate source of narrowband extreme-ultraviolet harmonics beyond 22 eV journal, June 2015

Sixth Harmonic of A Nd:YVO 4 Laser Generation In KBBF for ARPES journal, March 2008

Observation of Floquet-Bloch States on the Surface of a Topological Insulator journal, October 2013

Tracking Cooper Pairs in a Cuprate Superconductor by Ultrafast Angle-Resolved Photoemission journal, May 2012

Selective scattering between Floquet–Bloch and Volkov states in a topological insulator journal, January 2016

Time-resolved ARPES with sub-15 fs temporal and near Fourier-limited spectral resolution journal, October 2016

Cavity-enhanced high harmonic generation for extreme ultraviolet time- and angle-resolved photoemission spectroscopy journal, August 2019

Extreme ultraviolet time- and angle-resolved photoemission setup with 21.5 meV resolution using high-order harmonic generation from a turn-key Yb:KGW amplifier journal, January 2020

Persistent order due to transiently enhanced nesting in an electronically excited charge density wave journal, January 2016

Femtosecond core-level photoemision spectroscopy on 1 T -TaS 2 using a 60-eV laser source journal, February 2011

Recent advances in deep and vacuum-UV harmonic generation with KBBF crystal journal, September 2004

Clocking the Melting Transition of Charge and Lattice Order in 1 T − TaS 2 with Ultrafast Extreme-Ultraviolet Angle-Resolved Photoemission Spectroscopy journal, October 2011

Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution journal, August 2019

The development of new borate-based UV nonlinear optical crystals journal, January 2005

Time- and angle-resolved photoemission spectroscopy with optimized high-harmonic pulses using frequency-doubled Ti:Sapphire lasers journal, August 2014

Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate journal, February 2019

Transient Electronic Structure and Melting of a Charge Density Wave in TbTe3 journal, September 2008

Can silver nanoparticles be useful as potential biological labels? journal, May 2008

Advancing non-equilibrium ARPES experiments by a 9.3eV coherent ultrafast photon source journal, February 2016

X-ray monochromator designs based on extreme off-plane grating mountings journal, January 1981

A setup for extreme-ultraviolet ultrafast angle-resolved photoelectron spectroscopy at 50-kHz repetition rate journal, February 2019

Time- and angle-resolved photoemission spectroscopy with optimized high-harmonic pulses using frequency-doubled Ti:Sapphire lasers journal, August 2014

Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate text, January 2018

A high-order harmonic generation apparatus for time- and angle-resolved photoelectron spectroscopy
journal, July 2013

Coherent narrowband light source for ultrafast photoelectron spectroscopy in the 17–31 eV photon energy range
journal, January 2020

Ultrafast extreme ultraviolet photoemission without space charge
journal, September 2018

Full characterization and optimization of a femtosecond ultraviolet laser source for time and angle-resolved photoemission on solid surfaces
journal, April 2012

Time-resolved photoemission apparatus achieving sub-20-meV energy resolution and high stability
journal, December 2014

A versatile system for ultrahigh resolution, low temperature, and polarization dependent Laser-angle-resolved photoemission spectroscopy
journal, January 2008

Collapse of long-range charge order tracked by time-resolved photoemission at high momenta
journal, March 2011

Evidence for topological defects in a photoinduced phase transition
journal, October 2018

Bright high-repetition-rate source of narrowband extreme-ultraviolet harmonics beyond 22 eV
journal, June 2015

Sixth Harmonic of A Nd:YVO ₄ Laser Generation In KBBF for ARPES
journal, March 2008

Observation of Floquet-Bloch States on the Surface of a Topological Insulator
journal, October 2013

Tracking Cooper Pairs in a Cuprate Superconductor by Ultrafast Angle-Resolved Photoemission
journal, May 2012

Selective scattering between Floquet–Bloch and Volkov states in a topological insulator
journal, January 2016

Time-resolved ARPES with sub-15 fs temporal and near Fourier-limited spectral resolution
journal, October 2016

Cavity-enhanced high harmonic generation for extreme ultraviolet time- and angle-resolved photoemission spectroscopy
journal, August 2019

Extreme ultraviolet time- and angle-resolved photoemission setup with 21.5 meV resolution using high-order harmonic generation from a turn-key Yb:KGW amplifier
journal, January 2020

Persistent order due to transiently enhanced nesting in an electronically excited charge density wave
journal, January 2016

Femtosecond core-level photoemision spectroscopy on $1 T$ -TaS $_{2}$ using a 60-eV laser source
journal, February 2011

Recent advances in deep and vacuum-UV harmonic generation with KBBF crystal
journal, September 2004

Clocking the Melting Transition of Charge and Lattice Order in $1 T − {TaS}_{2}$ with Ultrafast Extreme-Ultraviolet Angle-Resolved Photoemission Spectroscopy
journal, October 2011

Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution
journal, August 2019

The development of new borate-based UV nonlinear optical crystals
journal, January 2005

Time- and angle-resolved photoemission spectroscopy with optimized high-harmonic pulses using frequency-doubled Ti:Sapphire lasers
journal, August 2014

Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate
journal, February 2019

Transient Electronic Structure and Melting of a Charge Density Wave in TbTe3
journal, September 2008

Can silver nanoparticles be useful as potential biological labels?
journal, May 2008

Advancing non-equilibrium ARPES experiments by a 9.3eV coherent ultrafast photon source
journal, February 2016

X-ray monochromator designs based on extreme off-plane grating mountings
journal, January 1981

A setup for extreme-ultraviolet ultrafast angle-resolved photoelectron spectroscopy at 50-kHz repetition rate
journal, February 2019

Time- and angle-resolved photoemission spectroscopy with optimized high-harmonic pulses using frequency-doubled Ti:Sapphire lasers
journal, August 2014

Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate
text, January 2018