Chemical looping beyond combustion – a perspective

Zhu, Xing; Imtiaz, Qasim; Donat, Felix; Müller, Christoph R.; Li, Fanxing

doi:10.1039/C9EE03793D

Title: Chemical looping beyond combustion – a perspective

Abstract

As a promising approach for carbon dioxide capture, chemical looping combustion has been extensively investigated for more than two decades. However, the chemical looping strategy can be and has been extended well beyond carbon capture. In fact, significant impacts on emission reduction, energy conservation, and value-creation can be anticipated from chemical looping beyond combustion (CLBC). This article aims to demonstrate the versatility and transformational benefits of CLBC. Specifically, we focus on the use of oxygen carriers or redox catalysts for chemical production – a $4 trillion industry that consumes 40.9 quadrillion BTU of energy. Compared to state-of-the-art chemical production technologies, we illustrate that chemical looping offers significant opportunities for process intensification and exergy loss minimization. In many cases, an order of magnitude reduction in energy consumption and CO₂ emission can be realized without the needs for carbon dioxide capture. In addition to providing various CLBC examples, this article elaborates on generalized design principles for CLBC, potential benefits and pitfalls, as well as redox catalyst selection, design, optimization, and redox reaction mechanism.

Authors:

Zhu, Xing ^[1]; Imtiaz, Qasim ^[2];

^[2];

^[3]

Department of Chemical and Biomolecular Engineering, North Carolina State University, Raleigh, USA, State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization
Department of Mechanical and Process Engineering, Laboratory of Energy Science and Engineering, ETH Zurich, Zurich, Switzerland
Department of Chemical and Biomolecular Engineering, North Carolina State University, Raleigh, USA

Publication Date:: Wed Mar 18 00:00:00 EDT 2020

Research Org.:: North Carolina State University, Raleigh, NC (United States)

Sponsoring Org.:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Energy Efficiency Office. Advanced Manufacturing Office; USDOE Office of Fossil Energy (FE)

OSTI Identifier:: 1596169

Alternate Identifier(s):: OSTI ID: 1799401

Grant/Contract Number:: EE0007888-05-6; FE0031521; EE0007888

Resource Type:: Published Article

Journal Name:: Energy & Environmental Science

Additional Journal Information:: Journal Name: Energy & Environmental Science Journal Volume: 13 Journal Issue: 3; Journal ID: ISSN 1754-5692

Publisher:: Royal Society of Chemistry (RSC)

Country of Publication:: United Kingdom

Language:: English

Subject:: 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats


                    Zhu, Xing, Imtiaz, Qasim, Donat, Felix, Müller, Christoph R., and Li, Fanxing. Chemical looping beyond combustion – a perspective.  United Kingdom: N. p., 2020. 
Web.  doi:10.1039/C9EE03793D.

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                    Zhu, Xing, Imtiaz, Qasim, Donat, Felix, Müller, Christoph R., & Li, Fanxing. Chemical looping beyond combustion – a perspective.  United Kingdom.  https://doi.org/10.1039/C9EE03793D

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                    Zhu, Xing, Imtiaz, Qasim, Donat, Felix, Müller, Christoph R., and Li, Fanxing. Wed .  
"Chemical looping beyond combustion – a perspective".  United Kingdom.  https://doi.org/10.1039/C9EE03793D.

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@article{osti_1596169,

  title        = {Chemical looping beyond combustion – a perspective},

  author       = {Zhu, Xing and Imtiaz, Qasim and Donat, Felix and Müller, Christoph R. and Li, Fanxing},

  abstractNote = {As a promising approach for carbon dioxide capture, chemical looping combustion has been extensively investigated for more than two decades. However, the chemical looping strategy can be and has been extended well beyond carbon capture. In fact, significant impacts on emission reduction, energy conservation, and value-creation can be anticipated from chemical looping beyond combustion (CLBC). This article aims to demonstrate the versatility and transformational benefits of CLBC. Specifically, we focus on the use of oxygen carriers or redox catalysts for chemical production – a $4 trillion industry that consumes 40.9 quadrillion BTU of energy. Compared to state-of-the-art chemical production technologies, we illustrate that chemical looping offers significant opportunities for process intensification and exergy loss minimization. In many cases, an order of magnitude reduction in energy consumption and CO2 emission can be realized without the needs for carbon dioxide capture. In addition to providing various CLBC examples, this article elaborates on generalized design principles for CLBC, potential benefits and pitfalls, as well as redox catalyst selection, design, optimization, and redox reaction mechanism.},

  doi          = {10.1039/C9EE03793D},

  journal      = {Energy & Environmental Science},

  number       = 3,

  volume       = 13,

  place        = {United Kingdom},

  year         = {Wed Mar 18 00:00:00 EDT 2020},

  month        = {Wed Mar 18 00:00:00 EDT 2020}

}

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Predicting the solar thermochemical water splitting ability and reaction mechanism of metal oxides: a case study of the hercynite family of water splitting cycles journal, January 2015

Ionic diffusion in the oxidation of iron—effect of support and its implications to chemical looping applications journal, January 2011

Methane partial oxidation using FeO x @La 0.8 Sr 0.2 FeO 3−δ core–shell catalyst – transient pulse studies journal, January 2015

Chemical Looping Combustion with Different Types of Liquid Fuels journal, February 2011

Oxidative dehydrogenation of ethane using MoO3/Fe2O3 catalysts in a cyclic redox mode journal, November 2018

CaCO3 calcination by the simultaneous reduction of CuO in a Ca/Cu chemical looping process journal, December 2015

Bifunctional core-shell architecture allows stable H2 production utilizing CH4 and CO2 in a catalytic chemical looping process journal, December 2019

Fe 2 O 3 , a cost effective and environmentally friendly catalyst for the generation of NH 3 – a future fuel – using a new Al 2 O 3 -looping based technology journal, January 2017

In situ encapsulation of iron(0) for solar thermochemical syngas production over iron-based perovskite material journal, September 2018

Recent Advances in Intensified Ethylene Production—A Review journal, August 2019

Upper bound on the yield for oxidative coupling of methane
journal, September 2003

The production of methyl formate by the vapor-phase oxidation of methanol
journal, September 1982

The effect of copper on the redox behaviour of iron oxide for chemical-looping hydrogen production probed by in situ X-ray absorption spectroscopy
journal, January 2018

Multimetallic catalysts of RuO 2 –CuO–Cs 2 O–TiO 2 /SiO 2 for direct gas-phase epoxidation of propylene to propylene oxide
journal, January 2016

Chemical-looping combustion (CLC) for inherent ${CO}_{2}$ separations—a review
journal, September 2008

Thermodynamic potential of high temperature chemical looping combustion with molten iron oxide as the oxygen carrier
journal, April 2017

Integration of Calcium and Chemical Looping Combustion using Composite CaO/CuO-Based Materials
journal, December 2011

Critical Literature Review of the Kinetics for the Oxidative Dehydrogenation of Propane over Well-Defined Supported Vanadium Oxide Catalysts
journal, September 2014

Diffuse reflectance Fourier-transform IR studies on the role of catalyst support on selectivity in ethene oxidation
journal, April 1991

High-Performance Ni–Fe Redox Catalysts for Selective CH 4 to Syngas Conversion via Chemical Looping
journal, January 2018

Highly Selective Oxidation of Ethyl Lactate to Ethyl Pyruvate Catalyzed by Mesoporous Vanadia–Titania
journal, January 2018

Combined calcium looping and chemical looping combustion cycles with CaO–CuO pellets in a fixed bed reactor
journal, August 2015

Chemical looping reforming of waste cooking oil in packed bed reactor
journal, August 2010

Catalytic behaviour of BIMEVOX powders in the oxidative dehydrodimerisation of propene
journal, July 2004

Supported vanadium oxide-based catalysts for the oxidehydrogenation of propane under cyclic conditions
journal, July 2004

CO production from CO 2 via reverse water–gas shift reaction performed in a chemical looping mode: Kinetics on modified iron oxide
journal, January 2017

Chemical Looping Co-splitting of H 2 O–CO 2 for Efficient Generation of Syngas
journal, August 2019

Oxygen and hydrogen productivities and repeatable reactivity of 30-mol%-Fe-, Co-, Ni-, Mn-doped CeO2−δ for thermochemical two-step water-splitting cycle
journal, October 2015

The use of La1−xSrxFeO3 perovskite-type oxides as oxygen carriers in chemical-looping reforming of methane
journal, June 2013

A Critical Assessment of Li/MgO-Based Catalysts for the Oxidative Coupling of Methane
journal, October 2011

Comparative study on the influence of second metals on Ag-loaded mesoporous SrTiO3 catalysts for ethylene oxide evolution
journal, June 2013

Ethylene Epoxidation Activity Over Ag-Based Catalysts on Different Nanocrystalline Perovskite Titanate Supports
journal, June 2012

Pd–Co based spinel oxides derived from pd nanoparticles immobilized on layered double hydroxides for toluene combustion
journal, February 2016

Oxidative dehydrogenation of ethane to ethylene in a system with circulating microspherical metal oxide oxygen carrier: 2. Ethylene production in a pilot unit with a riser reactor
journal, August 2016

Reactivity study on a novel hydrogen fueled chemical-looping combustion
journal, August 2001

N-desorption or NH3 generation of TiO2-loaded Al-based nitrogen carrier during chemical looping ammonia generation technology
journal, August 2018

Process design of a hydrogen production plant from natural gas with CO2 capture based on a novel Ca/Cu chemical loop
journal, February 2014

Dissociation of methane on different transition metals
journal, December 1998

Response to Comment on “Selective anaerobic oxidation of methane enables direct synthesis of methanol”
journal, October 2017

Deactivation kinetics of Ag/Al2O3 catalyst for ethylene epoxidation
journal, September 2004

Oxidative dehydrogenation of ethane: A study over the structure and robustness of Ni–W–O catalysts
journal, March 2014

Study of the calcination of CaCO3 by means of a Cu/CuO chemical loop using methane as fuel gas
journal, August 2019

Selectivity Patterns in Alkane Oxidation over Mg3(VO4)2-MgO, Mg2V2O7, and (VO)2P2O7
journal, March 1993

Enhanced sintering resistance of Fe2O3/CeO2 oxygen carrier for chemical looping hydrogen generation using core-shell structure
journal, March 2019

Dehydrogenation of Ethane via the Mars–van Krevelen Mechanism over La 0.8 Ba 0.2 MnO 3−δ Perovskites under Anaerobic Conditions
journal, October 2019

Manganese-containing redox catalysts for selective hydrogen combustion under a cyclic redox scheme
journal, April 2018

Oxidation of methanol to methyl formate over V-Ti oxide catalysts
journal, January 1987

Application of Fe2O3/Al2O3 Composite Particles as Oxygen Carrier of Chemical Looping Combustion
journal, June 2007

A hybrid solar-redox scheme for liquid fuel and hydrogen coproduction
journal, January 2014

Perovskite-type oxides LaFe1−Co O3 for chemical looping steam methane reforming to syngas and hydrogen co-production
journal, April 2016

Improving Syngas Selectivity of Fe 2 O 3 /Al 2 O 3 with Yttrium Modification in Chemical Looping Methane Conversion
journal, August 2019

Biomass direct chemical looping process: Process simulation
journal, December 2010

Selective Hydrodeoxygenation of Lignin-Derived Phenolic Monomers and Dimers to Cycloalkanes on Pd/C and HZSM-5 Catalysts
journal, November 2011

Methanol Selective Oxidation to Formaldehyde over Iron‐Molybdate Catalysts
journal, February 2005

Nano-sized silver crystals and their dispersion over α-alumina for ethylene epoxidation
journal, September 2009

Synergy of the catalytic activation on Ni and the CeO ₂ –TiO ₂ /Ce ₂ Ti ₂ O ₇ stoichiometric redox cycle for dramatically enhanced solar fuel production
journal, January 2019

Chemical looping partial oxidation of methane with CO2 utilization on the ceria-enhanced mesoporous Fe2O3 oxygen carrier
journal, March 2018

Recent advancements in chemical looping water splitting for the production of hydrogen
journal, January 2016

Chromium oxide supported on Zr modified alumina for stable and selective propane dehydrogenation in oxygen free moving bed process
journal, July 2017

Oxydehydrogenation of propane catalyzed by VSiO cogels: enhancement of the selectivity to propylene by operation under cyclic conditions
journal, January 2003

The relative performance of alternative oxygen carriers for liquid chemical looping combustion and gasification
journal, June 2017

Intensification of Ethylene Production from Naphtha via a Redox Oxy-Cracking Scheme: Process Simulations and Analysis
journal, October 2018

Dynamic Isotope Tracing: Role of Subsurface Oxygen in Ethylene Epoxidation on Silver
journal, May 1999

Progress in Chemical-Looping Combustion and Reforming technologies
journal, April 2012

A green chemistry approach to styrene from ethylbenzene and air on Mn x Ti 1−x O 2 catalyst
journal, January 2014

CaO-Based Pellets with Oxygen Carriers and Catalysts
journal, October 2011

Crystal structure of a bacterial non-haem iron hydroxylase that catalyses the biological oxidation of methane
journal, December 1993

From post-combustion carbon capture to sorption-enhanced hydrogen production: A state-of-the-art review of carbonate looping process feasibility
journal, December 2018

Chemical looping as reactor concept for the oxidative coupling of methane over a Na 2 WO 4 /Mn/SiO 2 catalyst
journal, December 2016

Super-dry reforming of methane intensifies CO2 utilization via Le Chateliers principle
journal, October 2016

Modulating Lattice Oxygen in Dual-Functional Mo–V–O Mixed Oxides for Chemical Looping Oxidative Dehydrogenation
journal, November 2019

Redox mechanism for selective oxidation of ethanol over monolayer V2O5/TiO2 catalysts
journal, June 2016

Dupont's CFB technology for maleic anhydride
journal, November 1999

Alkali Metal-Promoted La _x Sr _{2– x} FeO _4−δ Redox Catalysts for Chemical Looping Oxidative Dehydrogenation of Ethane
journal, January 2018

Chemical looping reforming of methane using magnetite as oxygen carrier: Structure evolution and reduction kinetics
journal, February 2018

Reliable oxygen transfer in MgAl2O4 spinel through the reversible formation of oxygen vacancies by Cu2+/Fe3+ anchoring
journal, June 2018

Enhanced hydrogen production performance through controllable redox exsolution within CoFeAlO x spinel oxygen carrier materials
journal, January 2018

Predicting the solar thermochemical water splitting ability and reaction mechanism of metal oxides: a case study of the hercynite family of water splitting cycles
journal, January 2015

Ionic diffusion in the oxidation of iron—effect of support and its implications to chemical looping applications
journal, January 2011

Methane partial oxidation using FeO _x @La _0.8 Sr _0.2 FeO _3−δ core–shell catalyst – transient pulse studies
journal, January 2015

Chemical Looping Combustion with Different Types of Liquid Fuels
journal, February 2011

Oxidative dehydrogenation of ethane using MoO3/Fe2O3 catalysts in a cyclic redox mode
journal, November 2018

CaCO3 calcination by the simultaneous reduction of CuO in a Ca/Cu chemical looping process
journal, December 2015

Bifunctional core-shell architecture allows stable H2 production utilizing CH4 and CO2 in a catalytic chemical looping process
journal, December 2019

Fe 2 O 3 , a cost effective and environmentally friendly catalyst for the generation of NH 3 – a future fuel – using a new Al 2 O 3 -looping based technology
journal, January 2017

In situ encapsulation of iron(0) for solar thermochemical syngas production over iron-based perovskite material
journal, September 2018

Recent Advances in Intensified Ethylene Production—A Review
journal, August 2019

Oxidative dehydrogenation of ethane to ethylene: A promising CeO2-ZrO2-modified NiO-Al2O3/Ni-foam catalyst
journal, January 2018

11,000 h of chemical-looping combustion operation—Where are we and where do we want to go?
journal, September 2019

Modeling Thermochemical Solar-to-Fuel Conversion: CALPHAD for Thermodynamic Assessment Studies of Perovskites, Exemplified for (La,Sr)MnO ₃
journal, September 2016