Chemical looping beyond combustion – a perspective

Zhu, Xing; Imtiaz, Qasim; Donat, Felix; Müller, Christoph R.; Li, Fanxing

doi:10.1039/c9ee03793d

Title: Chemical looping beyond combustion – a perspective

Journal Article · 13 January 2020 · Energy & Environmental Science

DOI: https://doi.org/10.1039/c9ee03793d · OSTI ID:1596169

Zhu, Xing ^[1]; Imtiaz, Qasim ^[2];

^[3];

^[4]

North Carolina State Univ., Raleigh, NC (United States). Dept. of Chemical and Biomolecular Engineering; Kunming Univ. of Science and Technology (China). State Key Lab. of Complex Nonferrous Metal Resources Clean Utilization. Faculty of Metallurgical and Energy Engineering
ETH Zurich (Switzerland). Dept. of Mechanical and Process Engineering. Lab. of Energy Science and Engineering; Lahore Univ. of Management Sciences (Pakistan). Dept. of Chemistry and Chemical Engineering
ETH Zurich (Switzerland). Dept. of Mechanical and Process Engineering. Lab. of Energy Science and Engineering
North Carolina State Univ., Raleigh, NC (United States). Dept. of Chemical and Biomolecular Engineering

As a promising approach for carbon dioxide capture, chemical looping combustion has been extensively investigated for more than two decades. However, the chemical looping strategy can be and has been extended well beyond carbon capture. In fact, significant impacts on emission reduction, energy conservation, and value-creation can be anticipated from chemical looping beyond combustion (CLBC). This article aims to demonstrate the versatility and transformational benefits of CLBC. Specifically, we focus on the use of oxygen carriers or redox catalysts for chemical production – a $4 trillion industry that consumes 40.9 quadrillion BTU of energy. Compared to state-of-the-art chemical production technologies, we illustrate that chemical looping offers significant opportunities for process intensification and exergy loss minimization. In many cases, an order of magnitude reduction in energy consumption and CO₂ emission can be realized without the needs for carbon dioxide capture. In addition to providing various CLBC examples, this article elaborates on generalized design principles for CLBC, potential benefits and pitfalls, as well as redox catalyst selection, design, optimization, and redox reaction mechanism.

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Research Organization:: North Carolina State University, Raleigh, NC (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Energy Efficiency Office. Advanced Manufacturing Office; USDOE Office of Fossil Energy (FE)

Grant/Contract Number:: EE0007888; FE0031521; EE0007888-05-6

OSTI ID:: 1596169

Alternate ID(s):: OSTI ID: 1799401

Journal Information:: Energy & Environmental Science, Vol. 13, Issue 3; ISSN 1754-5692

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 263 works

Citation information provided by
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