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Title: Precision heterodyne oxygen-corrected spectrometry: vertical profiling of water and carbon dioxide in the troposphere and lower stratosphere

Abstract

We describe the development of a near-infrared laser heterodyne radiometer: the precision heterodyne oxygen-corrected spectrometer (PHOCS). The prototype instrument is equipped with two heterodyne receivers for oxygen and water (measured near 1278 nanometers) and carbon dioxide (near 1572 nanometers) concentration profiles, respectively. The latter may be substituted by a heterodyne receiver module equipped with a laser to monitor atmospheric methane near 1651 nanometers. Oxygen measurements are intended to provide dry gas corrections and—more importantly—determine accurate temperature and pressure profiles that, in turn, improve the precision of the C O 2 and H 2 O column retrievals. Vertical profiling is made feasible by interrogating the very low-noise absorption lines shapes collected at ≈ <#comment/> 0.0067 c m − <#comment/> 1 resolution. PHOCS complements the results from the Orbiting Carbon Observatory (OCO-2), Active Sensing of C O 2 Emissions over Nights, Days, and Seasons (ASCENDS), and ground-based Fourier transform spectrometers. In this paper, we describe the development of the instrument by Mesa Photonics and present the results of initial tests in the vicinity of  Washington, DC.

Authors:
ORCiD logo [1];  [1];  [2];  [2]
  1. Mesa Photonics, Santa Fe, NM (United States)
  2. George Washington Univ., Washington, DC (United States)
Publication Date:
Research Org.:
Mesa Photonics LLC, Santa Fe, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC); National Aeronautics and Space Administration (NASA)
OSTI Identifier:
1582595
Alternate Identifier(s):
OSTI ID: 1598744
Grant/Contract Number:  
SC0019543
Resource Type:
Accepted Manuscript
Journal Name:
Applied Optics
Additional Journal Information:
Journal Volume: 59; Journal Issue: 7; Journal ID: ISSN 1559-128X
Publisher:
Optical Society of America
Country of Publication:
United States
Language:
English
Subject:
54 ENVIRONMENTAL SCIENCES; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; heterodyne; water vapor; oxygen; atmosphere; profile

Citation Formats

Bomse, David, Tso, Jared, Flores, Monia M., and Miller, John Houston. Precision heterodyne oxygen-corrected spectrometry: vertical profiling of water and carbon dioxide in the troposphere and lower stratosphere. United States: N. p., 2019. Web. doi:10.1364/AO.379684.
Bomse, David, Tso, Jared, Flores, Monia M., & Miller, John Houston. Precision heterodyne oxygen-corrected spectrometry: vertical profiling of water and carbon dioxide in the troposphere and lower stratosphere. United States. https://doi.org/10.1364/AO.379684
Bomse, David, Tso, Jared, Flores, Monia M., and Miller, John Houston. Wed . "Precision heterodyne oxygen-corrected spectrometry: vertical profiling of water and carbon dioxide in the troposphere and lower stratosphere". United States. https://doi.org/10.1364/AO.379684. https://www.osti.gov/servlets/purl/1582595.
@article{osti_1582595,
title = {Precision heterodyne oxygen-corrected spectrometry: vertical profiling of water and carbon dioxide in the troposphere and lower stratosphere},
author = {Bomse, David and Tso, Jared and Flores, Monia M. and Miller, John Houston},
abstractNote = {We describe the development of a near-infrared laser heterodyne radiometer: the precision heterodyne oxygen-corrected spectrometer (PHOCS). The prototype instrument is equipped with two heterodyne receivers for oxygen and water (measured near 1278 nanometers) and carbon dioxide (near 1572 nanometers) concentration profiles, respectively. The latter may be substituted by a heterodyne receiver module equipped with a laser to monitor atmospheric methane near 1651 nanometers. Oxygen measurements are intended to provide dry gas corrections and—more importantly—determine accurate temperature and pressure profiles that, in turn, improve the precision of the C O 2 and H 2 O column retrievals. Vertical profiling is made feasible by interrogating the very low-noise absorption lines shapes collected at ≈ <#comment/> 0.0067 c m − <#comment/> 1 resolution. PHOCS complements the results from the Orbiting Carbon Observatory (OCO-2), Active Sensing of C O 2 Emissions over Nights, Days, and Seasons (ASCENDS), and ground-based Fourier transform spectrometers. In this paper, we describe the development of the instrument by Mesa Photonics and present the results of initial tests in the vicinity of  Washington, DC.},
doi = {10.1364/AO.379684},
journal = {Applied Optics},
number = 7,
volume = 59,
place = {United States},
year = {Wed Dec 18 00:00:00 EST 2019},
month = {Wed Dec 18 00:00:00 EST 2019}
}

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