Selective Oxidative Cracking of n‐ Butane to Light Olefins over Hexagonal Boron Nitride with Limited Formation of CO x

doi:10.1002/cssc.201901663

Title: Selective Oxidative Cracking of n‐ Butane to Light Olefins over Hexagonal Boron Nitride with Limited Formation of CO _x

Authors:

^[1];

^[2];

^[3]

Department of ChemistryUniversity of Wisconsin-Madison 1101 University Avenue Madison WI 53706 USA
Department of Chemical and Biological EngineeringUniversity of Wisconsin-Madison 1415 Engineering Drive Madison WI 53706 USA
Department of ChemistryUniversity of Wisconsin-Madison 1101 University Avenue Madison WI 53706 USA, Department of Chemical and Biological EngineeringUniversity of Wisconsin-Madison 1415 Engineering Drive Madison WI 53706 USA

Publication Date:: 2019-10-11

Sponsoring Org.:: USDOE

OSTI Identifier:: 1570048

Grant/Contract Number:: SC0017918

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: ChemSusChem

Additional Journal Information:: Journal Name: ChemSusChem Journal Volume: 13 Journal Issue: 1; Journal ID: ISSN 1864-5631

Publisher:: Wiley Blackwell (John Wiley & Sons)

Country of Publication:: Germany

Language:: English

Citation Formats


                    McDermott, William P., Venegas, Juan, and Hermans, Ive. Selective Oxidative Cracking of n‐ Butane to Light Olefins over Hexagonal Boron Nitride with Limited Formation of CO x.  Germany: N. p., 2019. 
        Web.  doi:10.1002/cssc.201901663.

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                    McDermott, William P., Venegas, Juan, & Hermans, Ive. Selective Oxidative Cracking of n‐ Butane to Light Olefins over Hexagonal Boron Nitride with Limited Formation of CO x.  Germany.  doi:10.1002/cssc.201901663.

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                    McDermott, William P., Venegas, Juan, and Hermans, Ive. Fri .  
        "Selective Oxidative Cracking of n‐ Butane to Light Olefins over Hexagonal Boron Nitride with Limited Formation of CO x".  Germany.  doi:10.1002/cssc.201901663.

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@article{osti_1570048,

  title        = {Selective Oxidative Cracking of n‐ Butane to Light Olefins over Hexagonal Boron Nitride with Limited Formation of CO x},

  author       = {McDermott, William P. and Venegas, Juan and Hermans, Ive},

  abstractNote = {},

  doi          = {10.1002/cssc.201901663},

  journal      = {ChemSusChem},

  number       = 1,

  volume       = 13,

  place        = {Germany},

  year         = {2019},

  month        = {10}

}

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DOI: 10.1002/cssc.201901663

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Title: Selective Oxidative Cracking of n‐ Butane to Light Olefins over Hexagonal Boron Nitride with Limited Formation of CO x

Citation Formats

Thermal/catalytic cracking of liquid hydrocarbons for the production of olefins: A state-of-the-art review II: Catalytic cracking review journal, June 2016

Direct Measurements of Rate Constants for the Reactions of CH 3 Radicals with C 2 H 6 , C 2 H 4 , and C 2 H 2 at High Temperatures journal, September 2013

Influence of the Acid-Base Character of Supported Vanadium Catalysts on Their Catalytic Properties for the Oxidative Dehydrogenation of n-Butane journal, December 1995

Enhanced performance of boron nitride catalysts with induction period for the oxidative dehydrogenation of ethane to ethylene journal, September 2018

Oxidative conversion of propane over lithium-promoted magnesia catalyst I. Kinetics and mechanism journal, September 2003

Selective Oxidation of n -Butane and Isobutane Catalyzed by Boron Nitride journal, March 2017

Thermal/catalytic cracking of hydrocarbons for the production of olefins: A state-of-the-art review I: Thermal cracking review journal, January 2015

Synchrotron Photoionization Mass Spectrometry Measurements of Product Formation in Low-Temperature n -Butane Oxidation: Toward a Fundamental Understanding of Autoignition Chemistry and n -C 4 H 9 + O 2 / s -C 4 H 9 + O 2 Reactions journal, November 2013

Partial oxidation of CH4 and C2H6 over noble metalcoated monoliths journal, December 1994

Catalytic oxidation of n-octane over cobalt substituted ceria (Ce0.90Co0.10O2−δ) catalysts journal, December 2012

Selective oxidative dehydrogenation of propane to propene using boron nitride catalysts journal, December 2016

Partial Oxidation of C5and C6Alkanes over Monolith Catalysts at Short Contact Times journal, June 1998

Highly effective oxidative cracking of n-butane in light olefins on a novel cobalt catalyst journal, October 2005

Infrared frequency-modulation probing of product formation in alkyl + O2 reactions. Part IV.For Part III see ref. 12. Reactions of propyl and butyl radicals with O2Electronic Supplementary Information available. See http://www.rsc.org/suppdata/fd/b1/b102237g/ journal, October 2001

The Influence of Reactor Parameters on the Boron Nitride-Catalyzed Oxidative Dehydrogenation of Propane journal, November 2018

Catalytic partial oxidation of alkanes on silver in fluidized bed and monolith reactors journal, June 1996

Selective oxidative dehydrogenation of butane over V$z.sbnd;Mg$z.sbnd;O catalysts journal, June 1987

Gas-Phase Reaction Network of Li/MgO-Catalyzed Oxidative Coupling of Methane and Oxidative Dehydrogenation of Ethane journal, February 2019

Operando Raman spectroscopy study on the deactivation of Pt/Al2O3 and Pt–Sn/Al2O3 propane dehydrogenation catalysts journal, January 2013

Catalytic oxidative cracking of hexane as a route to olefins journal, January 2010

Oxidative catalytic cracking of n-butane to lower alkenes over layered BiOCl catalyst journal, January 2001

Kinetics of 1-butyl and 2-butyl radical reactions with molecular oxygen: Experiment and theory journal, January 2019

Formation of high surface area Li/MgO—Efficient catalyst for the oxidative dehydrogenation/cracking of propane journal, August 2006

Boron and Boron-Containing Catalysts for the Oxidative Dehydrogenation of Propane journal, September 2017

Activation of Alkanes by Gold-Modified Lanthanum Oxide journal, December 2010

Production of Olefins by Oxidative Dehydrogenation of Propane and Butane over Monoliths at Short Contact Times journal, September 1994

Oxidative conversion of propane over lithium-promoted magnesia catalyst II. Active site characterization and hydrocarbon activation journal, September 2003

Probing the Transformation of Boron Nitride Catalysts under Oxidative Dehydrogenation Conditions journal, November 2018

Catalytic Dehydrogenation of Light Alkanes on Metals and Metal Oxides journal, August 2014

Oxidative conversion of light alkanes to olefins over alkali promoted oxide catalysts journal, March 2002

Selective oxidative dehydrogenation of ethane to ethylene over a hydroxylated boron nitride catalyst journal, February 2017

Direct Insight into Ethane Oxidative Dehydrogenation over Boron Nitrides journal, July 2017

Edge-hydroxylated Boron Nitride for Oxidative Dehydrogenation of Propane to Propylene journal, May 2017

Evaluated Kinetics of the Reactions of H and CH 3 with n -Alkanes: Experiments with n -Butane and a Combustion Model Reaction Network Analysis journal, February 2015

Catalytic Oxidative Cracking of Propane Over Nanosized Gold Supported Ce0.5Zr0.5O2 Catalysts journal, July 2013

Olefins by Catalytic Oxidation of Alkanes in Fluidized-Bed Reactors journal, September 1995

Catalytic oxidative cracking of n-propane over nanosized gold supported La2O3 catalysts journal, December 2018

Novel nitrogen containing heterogeneous catalysts for oxidative dehydrogenation of light paraffins journal, August 2002

Title: Selective Oxidative Cracking of n‐ Butane to Light Olefins over Hexagonal Boron Nitride with Limited Formation of CO _x

Thermal/catalytic cracking of liquid hydrocarbons for the production of olefins: A state-of-the-art review II: Catalytic cracking review
journal, June 2016

Direct Measurements of Rate Constants for the Reactions of CH ₃ Radicals with C ₂ H ₆ , C ₂ H ₄ , and C ₂ H ₂ at High Temperatures
journal, September 2013

Influence of the Acid-Base Character of Supported Vanadium Catalysts on Their Catalytic Properties for the Oxidative Dehydrogenation of n-Butane
journal, December 1995

Enhanced performance of boron nitride catalysts with induction period for the oxidative dehydrogenation of ethane to ethylene
journal, September 2018

Oxidative conversion of propane over lithium-promoted magnesia catalyst I. Kinetics and mechanism
journal, September 2003

Selective Oxidation of n -Butane and Isobutane Catalyzed by Boron Nitride
journal, March 2017

Thermal/catalytic cracking of hydrocarbons for the production of olefins: A state-of-the-art review I: Thermal cracking review
journal, January 2015

Synchrotron Photoionization Mass Spectrometry Measurements of Product Formation in Low-Temperature n -Butane Oxidation: Toward a Fundamental Understanding of Autoignition Chemistry and n -C ₄ H ₉ + O ₂ / s -C ₄ H ₉ + O ₂ Reactions
journal, November 2013

Partial oxidation of CH4 and C2H6 over noble metalcoated monoliths
journal, December 1994

Catalytic oxidation of n-octane over cobalt substituted ceria (Ce0.90Co0.10O2−δ) catalysts
journal, December 2012

Selective oxidative dehydrogenation of propane to propene using boron nitride catalysts
journal, December 2016

Partial Oxidation of C5and C6Alkanes over Monolith Catalysts at Short Contact Times
journal, June 1998

Highly effective oxidative cracking of n-butane in light olefins on a novel cobalt catalyst
journal, October 2005

Infrared frequency-modulation probing of product formation in alkyl + O2 reactions. Part IV.For Part III see ref. 12. Reactions of propyl and butyl radicals with O2Electronic Supplementary Information available. See http://www.rsc.org/suppdata/fd/b1/b102237g/
journal, October 2001

The Influence of Reactor Parameters on the Boron Nitride-Catalyzed Oxidative Dehydrogenation of Propane
journal, November 2018

Catalytic partial oxidation of alkanes on silver in fluidized bed and monolith reactors
journal, June 1996

Selective oxidative dehydrogenation of butane over V$z.sbnd;Mg$z.sbnd;O catalysts
journal, June 1987

Gas-Phase Reaction Network of Li/MgO-Catalyzed Oxidative Coupling of Methane and Oxidative Dehydrogenation of Ethane
journal, February 2019

Operando Raman spectroscopy study on the deactivation of Pt/Al2O3 and Pt–Sn/Al2O3 propane dehydrogenation catalysts
journal, January 2013

Catalytic oxidative cracking of hexane as a route to olefins
journal, January 2010

Oxidative catalytic cracking of n-butane to lower alkenes over layered BiOCl catalyst
journal, January 2001

Kinetics of 1-butyl and 2-butyl radical reactions with molecular oxygen: Experiment and theory
journal, January 2019

Formation of high surface area Li/MgO—Efficient catalyst for the oxidative dehydrogenation/cracking of propane
journal, August 2006

Boron and Boron-Containing Catalysts for the Oxidative Dehydrogenation of Propane
journal, September 2017

Activation of Alkanes by Gold-Modified Lanthanum Oxide
journal, December 2010

Production of Olefins by Oxidative Dehydrogenation of Propane and Butane over Monoliths at Short Contact Times
journal, September 1994

Oxidative conversion of propane over lithium-promoted magnesia catalyst II. Active site characterization and hydrocarbon activation
journal, September 2003

Probing the Transformation of Boron Nitride Catalysts under Oxidative Dehydrogenation Conditions
journal, November 2018

Catalytic Dehydrogenation of Light Alkanes on Metals and Metal Oxides
journal, August 2014

Oxidative conversion of light alkanes to olefins over alkali promoted oxide catalysts
journal, March 2002

Selective oxidative dehydrogenation of ethane to ethylene over a hydroxylated boron nitride catalyst
journal, February 2017

Direct Insight into Ethane Oxidative Dehydrogenation over Boron Nitrides
journal, July 2017

Edge-hydroxylated Boron Nitride for Oxidative Dehydrogenation of Propane to Propylene
journal, May 2017

Evaluated Kinetics of the Reactions of H and CH ₃ with n -Alkanes: Experiments with n -Butane and a Combustion Model Reaction Network Analysis
journal, February 2015

Catalytic Oxidative Cracking of Propane Over Nanosized Gold Supported Ce0.5Zr0.5O2 Catalysts
journal, July 2013

Olefins by Catalytic Oxidation of Alkanes in Fluidized-Bed Reactors
journal, September 1995

Catalytic oxidative cracking of n-propane over nanosized gold supported La2O3 catalysts
journal, December 2018

Novel nitrogen containing heterogeneous catalysts for oxidative dehydrogenation of light paraffins
journal, August 2002