Regional Similarities and NOx-Related Increases in Biogenic Secondary Organic Aerosol in Summertime Southeastern United States
Abstract
Abstract During the 2013 Southern Oxidant and Aerosol Study, Fourier transform infrared spectroscopy (FTIR) and aerosol mass spectrometer (AMS) measurements of submicron mass were collected at Look Rock (LRK), Tennessee, and Centreville (CTR), Alabama. Carbon monoxide and submicron sulfate and organic mass concentrations were 15–60% higher at CTR than at LRK, but their time series had moderate correlations ( r ~ 0.5). However, NO x had no correlation ( r = 0.08) between the two sites with nighttime‐to‐early‐morning peaks 3–10 times higher at CTR than at LRK. Organic mass (OM) sources identified by FTIR Positive Matrix Factorization (PMF) had three very similar factors at both sites: fossil fuel combustion‐related organic aerosols, mixed organic aerosols, and biogenic organic aerosols (BOA). The BOA spectrum from FTIR is similar (cosine similarity > 0.6) to that of lab‐generated particle mass from the photochemical oxidation of both isoprene and monoterpenes under high NO x conditions from chamber experiments. The BOA mass fraction was highest during the night at CTR but in the afternoon at LRK. AMS PMF resulted in two similar pairs of factors at both sites and a third nighttime NO x ‐related factor (33% of OM) at CTR but a daytime nitrate‐related factor (28% of OM) atmore »
- Authors:
-
[1];
[1];
[2];
[3];
[4];
[6];
[7];
[9];
[10]
- Univ. of California, San Diego, CA (United States). Scripps Inst. of Oceanography
- Federal Inst. of Technology, Lausanne (Switzerland)
- Univ. of Colorado, Boulder, CO (United States)
- U.S. Environmental Protection Agency, Research Triangle Park, NC (United States). National Exposure Research Laboratory
- California Inst. of Technology (CalTech), Pasadena, CA (United States)
- Georgia Inst. of Technology, Atlanta, GA (United States)
- Harvard Univ., Cambridge, MA (United States)
- Nanyang Technological Univ. (Singapore)
- Univ. of Wisconsin, Madison, WI (United States)
- Univ. of North Carolina, Chapel Hill, NC (United States)
- Publication Date:
- Research Org.:
- Univ. of California, San Diego, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1539758
- Alternate Identifier(s):
- OSTI ID: 1472149
- Grant/Contract Number:
- SC0006431; DE‐SC0006431
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Additional Journal Information:
- Journal Volume: 123; Journal Issue: 18; Journal ID: ISSN 2169-897X
- Publisher:
- American Geophysical Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES; Meteorology & Atmospheric Sciences
Citation Formats
Liu, Jun, Russell, Lynn M., Ruggeri, Giulia, Takahama, Satoshi, Claflin, Megan S., Ziemann, Paul J., Pye, Havala O. T., Murphy, Benjamin N., Xu, Lu, Ng, Nga L., McKinney, Karena A., Budisulistiorini, Sri Hapsari, Bertram, Timothy H., Nenes, Athanasios, and Surratt, Jason D. Regional Similarities and NOx-Related Increases in Biogenic Secondary Organic Aerosol in Summertime Southeastern United States. United States: N. p., 2018.
Web. doi:10.1029/2018jd028491.
Liu, Jun, Russell, Lynn M., Ruggeri, Giulia, Takahama, Satoshi, Claflin, Megan S., Ziemann, Paul J., Pye, Havala O. T., Murphy, Benjamin N., Xu, Lu, Ng, Nga L., McKinney, Karena A., Budisulistiorini, Sri Hapsari, Bertram, Timothy H., Nenes, Athanasios, & Surratt, Jason D. Regional Similarities and NOx-Related Increases in Biogenic Secondary Organic Aerosol in Summertime Southeastern United States. United States. https://doi.org/10.1029/2018jd028491
Liu, Jun, Russell, Lynn M., Ruggeri, Giulia, Takahama, Satoshi, Claflin, Megan S., Ziemann, Paul J., Pye, Havala O. T., Murphy, Benjamin N., Xu, Lu, Ng, Nga L., McKinney, Karena A., Budisulistiorini, Sri Hapsari, Bertram, Timothy H., Nenes, Athanasios, and Surratt, Jason D. Sat .
"Regional Similarities and NOx-Related Increases in Biogenic Secondary Organic Aerosol in Summertime Southeastern United States". United States. https://doi.org/10.1029/2018jd028491. https://www.osti.gov/servlets/purl/1539758.
@article{osti_1539758,
title = {Regional Similarities and NOx-Related Increases in Biogenic Secondary Organic Aerosol in Summertime Southeastern United States},
author = {Liu, Jun and Russell, Lynn M. and Ruggeri, Giulia and Takahama, Satoshi and Claflin, Megan S. and Ziemann, Paul J. and Pye, Havala O. T. and Murphy, Benjamin N. and Xu, Lu and Ng, Nga L. and McKinney, Karena A. and Budisulistiorini, Sri Hapsari and Bertram, Timothy H. and Nenes, Athanasios and Surratt, Jason D.},
abstractNote = {Abstract During the 2013 Southern Oxidant and Aerosol Study, Fourier transform infrared spectroscopy (FTIR) and aerosol mass spectrometer (AMS) measurements of submicron mass were collected at Look Rock (LRK), Tennessee, and Centreville (CTR), Alabama. Carbon monoxide and submicron sulfate and organic mass concentrations were 15–60% higher at CTR than at LRK, but their time series had moderate correlations ( r ~ 0.5). However, NO x had no correlation ( r = 0.08) between the two sites with nighttime‐to‐early‐morning peaks 3–10 times higher at CTR than at LRK. Organic mass (OM) sources identified by FTIR Positive Matrix Factorization (PMF) had three very similar factors at both sites: fossil fuel combustion‐related organic aerosols, mixed organic aerosols, and biogenic organic aerosols (BOA). The BOA spectrum from FTIR is similar (cosine similarity > 0.6) to that of lab‐generated particle mass from the photochemical oxidation of both isoprene and monoterpenes under high NO x conditions from chamber experiments. The BOA mass fraction was highest during the night at CTR but in the afternoon at LRK. AMS PMF resulted in two similar pairs of factors at both sites and a third nighttime NO x ‐related factor (33% of OM) at CTR but a daytime nitrate‐related factor (28% of OM) at LRK. NO x was correlated with BOA and LO‐OOA for NO x concentrations higher than 1 ppb at both sites, producing 0.5 ± 0.1 μ g/m 3 for CTR‐LO‐OOA and 1.0 ± 0.3 μ g/m 3 for CTR‐BOA additional biogenic OM for each 1 ppb increase of NO x .},
doi = {10.1029/2018jd028491},
journal = {Journal of Geophysical Research: Atmospheres},
number = 18,
volume = 123,
place = {United States},
year = {Sat Aug 04 00:00:00 EDT 2018},
month = {Sat Aug 04 00:00:00 EDT 2018}
}
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Works referencing / citing this record:
Quantifying organic matter and functional groups in particulate matter filter samples from the southeastern United States – Part 1: Methods
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