Dynamic and programmable morphology and size evolution via a living hierarchical self-assembly strategy
Abstract
Recent advances in the preparation of shape-shifting and size-growing nanostructures are hot topics in development of nanoscience, because many intelligent functions are always relied on their shape and dimension. Here we report a tunable manipulation of sequential self-assembled transformation in situ via a hierarchical assembly strategy based on a living thiol–disulfide exchange reaction. By tailoring the external stimuli, the reactive points can be generated at the ends of initially unimolecular micelles, which subsequently drive the pre-assemblies to periodically proceed into the hierarchically micellar connection, axial growth, bending, and cyclization processes from nanoscopic assemblies to macroscopic particles. Of particular interest would be systems that acquired the shape control and size adjustment of self-assemblies after termination or reactivation of disulfide reshuffling reaction by regulating external stimuli whenever needed. Such a hierarchical strategy for self-assembled evolution is universally applicable not only for other disulfide-linked dendritic polymers but also for exploitation of biological applications.
- Authors:
-
- Chinese Academy of Sciences (CAS), Beijing (China)
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Chinese Academy of Sciences (CAS), Beijing (China); Zhengzhou Univ., Henan (China)
- Chinese Academy of Sciences (CAS), Beijing (China); Univ. of Chinese Academy of Sciences, Beijing (China)
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1531348
- Report Number(s):
- PNNL-SA-136487
Journal ID: ISSN 2041-1723
- Grant/Contract Number:
- AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY
Citation Formats
Wang, Xing, Gao, Peiyuan, Yang, Yanyu, Guo, Hongxia, and Wu, Decheng. Dynamic and programmable morphology and size evolution via a living hierarchical self-assembly strategy. United States: N. p., 2018.
Web. doi:10.1038/s41467-018-05142-3.
Wang, Xing, Gao, Peiyuan, Yang, Yanyu, Guo, Hongxia, & Wu, Decheng. Dynamic and programmable morphology and size evolution via a living hierarchical self-assembly strategy. United States. https://doi.org/10.1038/s41467-018-05142-3
Wang, Xing, Gao, Peiyuan, Yang, Yanyu, Guo, Hongxia, and Wu, Decheng. Tue .
"Dynamic and programmable morphology and size evolution via a living hierarchical self-assembly strategy". United States. https://doi.org/10.1038/s41467-018-05142-3. https://www.osti.gov/servlets/purl/1531348.
@article{osti_1531348,
title = {Dynamic and programmable morphology and size evolution via a living hierarchical self-assembly strategy},
author = {Wang, Xing and Gao, Peiyuan and Yang, Yanyu and Guo, Hongxia and Wu, Decheng},
abstractNote = {Recent advances in the preparation of shape-shifting and size-growing nanostructures are hot topics in development of nanoscience, because many intelligent functions are always relied on their shape and dimension. Here we report a tunable manipulation of sequential self-assembled transformation in situ via a hierarchical assembly strategy based on a living thiol–disulfide exchange reaction. By tailoring the external stimuli, the reactive points can be generated at the ends of initially unimolecular micelles, which subsequently drive the pre-assemblies to periodically proceed into the hierarchically micellar connection, axial growth, bending, and cyclization processes from nanoscopic assemblies to macroscopic particles. Of particular interest would be systems that acquired the shape control and size adjustment of self-assemblies after termination or reactivation of disulfide reshuffling reaction by regulating external stimuli whenever needed. Such a hierarchical strategy for self-assembled evolution is universally applicable not only for other disulfide-linked dendritic polymers but also for exploitation of biological applications.},
doi = {10.1038/s41467-018-05142-3},
journal = {Nature Communications},
number = 1,
volume = 9,
place = {United States},
year = {Tue Jul 17 00:00:00 EDT 2018},
month = {Tue Jul 17 00:00:00 EDT 2018}
}
Web of Science
Works referenced in this record:
Atomically Precise Prediction of 2D Self-Assembly of Weakly Bonded Nanostructures: STM Insight into Concentration-Dependent Architectures
journal, November 2015
- El Garah, Mohamed; Dianat, Arezoo; Cadeddu, Andrea
- Small, Vol. 12, Issue 3
Bioinspired polymer vesicles and membranes for biological and medical applications
journal, January 2016
- Palivan, Cornelia G.; Goers, Roland; Najer, Adrian
- Chemical Society Reviews, Vol. 45, Issue 2
Hierarchical Self-Assembly for Nanomedicine
journal, January 2016
- Bishop, Kyle J. M.
- Angewandte Chemie International Edition, Vol. 55, Issue 5
Polymeric Nanoparticles Amenable to Simultaneous Installation of Exterior Targeting and Interior Therapeutic Proteins
journal, February 2016
- Zhu, Xi; Wu, Jun; Shan, Wei
- Angewandte Chemie International Edition, Vol. 55, Issue 10
Self-assembly of block copolymers
journal, January 2012
- Mai, Yiyong; Eisenberg, Adi
- Chemical Society Reviews, Vol. 41, Issue 18
Hydrogel Formation upon Photoinduced Covalent Capture of Macrocycle Stacks from Dynamic Combinatorial Libraries
journal, July 2011
- Li, Jianwei; Carnall, Jacqui M. A.; Stuart, Marc C. A.
- Angewandte Chemie International Edition, Vol. 50, Issue 36
Antimicrobial Metallopolymers and Their Bioconjugates with Conventional Antibiotics against Multidrug-Resistant Bacteria
journal, March 2014
- Zhang, Jiuyang; Chen, Yung Pin; Miller, Kristen P.
- Journal of the American Chemical Society, Vol. 136, Issue 13
Controlling the Structure and Length of Self-Synthesizing Supramolecular Polymers through Nucleated Growth and Disassembly
journal, May 2015
- Pal, Asish; Malakoutikhah, Morteza; Leonetti, Giulia
- Angewandte Chemie International Edition, Vol. 54, Issue 27
Dynamic Combinatorial Chemistry
journal, September 2006
- Corbett, Peter T.; Leclaire, Julien; Vial, Laurent
- Chemical Reviews, Vol. 106, Issue 9
Synthetic Self-Assembled Materials in Biological Environments
journal, April 2016
- Versluis, Frank; van Esch, Jan H.; Eelkema, Rienk
- Advanced Materials, Vol. 28, Issue 23
Fabrication of pH-Responsive Nanoparticles with an AIE Feature for Imaging Intracellular Drug Delivery
journal, August 2016
- Wang, Xing; Yang, Yanyu; Zhuang, Yaping
- Biomacromolecules, Vol. 17, Issue 9
Dual Redox Responsive Assemblies Formed from Diselenide Block Copolymers
journal, January 2010
- Ma, Ning; Li, Ying; Xu, Huaping
- Journal of the American Chemical Society, Vol. 132, Issue 2
Self-Assembly of a Functional Oligo(Aniline)-Based Amphiphile into Helical Conductive Nanowires
journal, November 2015
- Bell, O. Alexander; Wu, Guanglu; Haataja, Johannes S.
- Journal of the American Chemical Society, Vol. 137, Issue 45
Dynamic Cylindrical Assembly of Triblock Copolymers by a Hierarchical Process of Covalent and Supramolecular Interactions
journal, February 2011
- Li, Zhou; Ma, Jun; Lee, Nam S.
- Journal of the American Chemical Society, Vol. 133, Issue 5
Molecular Biodynamers: Dynamic Covalent Analogues of Biopolymers
journal, January 2017
- Liu, Yun; Lehn, Jean-Marie; Hirsch, Anna K. H.
- Accounts of Chemical Research, Vol. 50, Issue 2
Transient laser heating induced hierarchical porous structures from block copolymer–directed self-assembly
journal, July 2015
- Tan, Kwan Wee; Jung, Byungki; Werner, Jörg G.
- Science, Vol. 349, Issue 6243
Tuning the Amphiphilicity of Building Blocks: Controlled Self-Assembly and Disassembly for Functional Supramolecular Materials
journal, July 2009
- Wang, Yapei; Xu, Huaping; Zhang, Xi
- Advanced Materials, Vol. 21, Issue 28
Hierarchically structured transparent hybrid membranes by in situ growth of mesostructured organosilica in host polymer
journal, January 2006
- Vallé, Karine; Belleville, Philippe; Pereira, Franck
- Nature Materials, Vol. 5, Issue 2
Kinetically Controlled Sequential Growth of Surface-Grafted Chiral Supramolecular Copolymers
journal, March 2016
- Frisch, Hendrik; Fritz, Eva-Corinna; Stricker, Friedrich
- Angewandte Chemie International Edition, Vol. 55, Issue 25
Photoresponsive Supramolecular Amphiphiles for Controlled Self-Assembly of Nanofibers and Vesicles
journal, May 2010
- Wang, Chao; Chen, Qishui; Xu, Huaping
- Advanced Materials, Vol. 22, Issue 23
Synthesis of Nonequilibrium Supramolecular Peptide Polymers on a Microfluidic Platform
journal, July 2016
- Mason, Thomas O.; Michaels, Thomas C. T.; Levin, Aviad
- Journal of the American Chemical Society, Vol. 138, Issue 30
Controlled Self-Assembly Manipulated by Charge-Transfer Interactions: From Tubes to Vesicles
journal, November 2008
- Wang, Chao; Yin, Shouchun; Chen, Senlin
- Angewandte Chemie International Edition, Vol. 47, Issue 47
Nanoscale Control of Polymer Assembly on a Synthetic Catalyst–Bilayer System
journal, July 2016
- Gorgoll, Ricardo M.; Harano, Koji; Nakamura, Eiichi
- Journal of the American Chemical Society, Vol. 138, Issue 30
Programming Self-Assembly of DNA Origami Honeycomb Two-Dimensional Lattices and Plasmonic Metamaterials
journal, June 2016
- Wang, Pengfei; Gaitanaros, Stavros; Lee, Seungwoo
- Journal of the American Chemical Society, Vol. 138, Issue 24
Synthesis and self-assembly behavior of POSS-embedded hyperbranched polymers
journal, January 2015
- Li, Dawei; Niu, Yuguang; Yang, Yanyu
- Chemical Communications, Vol. 51, Issue 39
Self-assembly of noble metal monolayers on transition metal carbide nanoparticle catalysts
journal, May 2016
- Hunt, S. T.; Milina, M.; Alba-Rubio, A. C.
- Science, Vol. 352, Issue 6288
Selective assemblies of giant tetrahedra via precisely controlled positional interactions
journal, April 2015
- Huang, M.; Hsu, C. -H.; Wang, J.
- Science, Vol. 348, Issue 6233
Guided hierarchical co-assembly of soft patchy nanoparticles
journal, November 2013
- Gröschel, André H.; Walther, Andreas; Löbling, Tina I.
- Nature, Vol. 503, Issue 7475
Supramolecular Coordination: Self-Assembly of Finite Two- and Three-Dimensional Ensembles
journal, November 2011
- Chakrabarty, Rajesh; Mukherjee, Partha Sarathi; Stang, Peter J.
- Chemical Reviews, Vol. 111, Issue 11, p. 6810-6918
Applications of Orthogonal “Click” Chemistries in the Synthesis of Functional Soft Materials
journal, November 2009
- Iha, Rhiannon K.; Wooley, Karen L.; Nyström, Andreas M.
- Chemical Reviews, Vol. 109, Issue 11
The Convergence of Synthetic Organic and Polymer Chemistries
journal, August 2005
- Hawker, C. J.
- Science, Vol. 309, Issue 5738
Design of polymeric nanoparticles for biomedical delivery applications
journal, January 2012
- Elsabahy, Mahmoud; Wooley, Karen L.
- Chemical Society Reviews, Vol. 41, Issue 7
Reversible Supramolecular Surface Attachment of Enzyme-Polymer Conjugates for the Design of Biocatalytic Filtration Membranes
journal, October 2015
- Moridi, Negar; Corvini, Philippe F. -X.; Shahgaldian, Patrick
- Angewandte Chemie International Edition, Vol. 54, Issue 49
Simultaneous In-Situ Synthesis and Characterization of Co@Cu Core-Shell Nanoparticle Arrays
journal, December 2014
- McKeown, Joseph T.; Wu, Yueying; Fowlkes, Jason D.
- Advanced Materials, Vol. 27, Issue 6
A Dual-Thermoresponsive Gemini-Type Supra-amphiphilic Macromolecular [3]Pseudorotaxane Based on Pillar[10]arene/Paraquat Cooperative Complexation
journal, February 2016
- Chi, Xiaodong; Yu, Guocan; Shao, Li
- Journal of the American Chemical Society, Vol. 138, Issue 9
Shape-shifting colloids via stimulated dewetting
journal, July 2016
- Youssef, Mena; Hueckel, Theodore; Yi, Gi-Ra
- Nature Communications, Vol. 7, Issue 1
Block Copolymer Assembly via Kinetic Control
journal, August 2007
- Cui, H.; Chen, Z.; Zhong, S.
- Science, Vol. 317, Issue 5838
Reversibly Shape-Shifting Organic Optical Waveguides: Formation of Organic Nanorings, Nanotubes, and Nanosheets
journal, January 2012
- Chandrasekhar, Naisa; Chandrasekar, Rajadurai
- Angewandte Chemie International Edition, Vol. 51, Issue 15
Simulation-Assisted Self-Assembly of Multicomponent Polymers into Hierarchical Assemblies with Varied Morphologies
journal, June 2013
- Cai, Chunhua; Li, Yongliang; Lin, Jiaping
- Angewandte Chemie International Edition, Vol. 52, Issue 30
Cover Picture: Structurally Defined Molecular Hypervalent Iodine Catalysts for Intermolecular Enantioselective Reactions (Angew. Chem. Int. Ed. 1/2016)
journal, December 2015
- Haubenreisser, Stefan; Wöste, Thorsten H.; Martínez, Claudio
- Angewandte Chemie International Edition, Vol. 55, Issue 1
An Intriguing Morphology Evolution of Polyoxometalate-Polystyrene Hybrid Amphiphiles from Vesicles to Tubular Aggregates
journal, November 2010
- Han, Yao-Kun; Zhang, Zi-Jian; Wang, Yong-Liang
- Macromolecular Chemistry and Physics, Vol. 212, Issue 1
A Filled-Honeycomb-Structured Crystal Formed by Self-Assembly of a Janus Polyoxometalate-Silsesquioxane (POM-POSS) Co-Cluster
journal, November 2015
- Ma, Chi; Wu, Han; Huang, Zi-Han
- Angewandte Chemie International Edition, Vol. 54, Issue 52
‘Living’ Controlled in Situ Gelling Systems: Thiol−Disulfide Exchange Method toward Tailor-Made Biodegradable Hydrogels
journal, November 2010
- Wu, De-Cheng; Loh, Xian Jun; Wu, Yun-Long
- Journal of the American Chemical Society, Vol. 132, Issue 43
Controlled cross-linking strategy: from hybrid hydrogels to nanoparticle macroscopic aggregates
journal, January 2013
- Wang, Xing; Li, Dan; Yang, Fei
- Polymer Chemistry, Vol. 4, Issue 17
A Giant Surfactant of Polystyrene−(Carboxylic Acid-Functionalized Polyhedral Oligomeric Silsesquioxane) Amphiphile with Highly Stretched Polystyrene Tails in Micellar Assemblies
journal, December 2010
- Yu, Xinfei; Zhong, Sheng; Li, Xiaopeng
- Journal of the American Chemical Society, Vol. 132, Issue 47
Breaking Symmetry toward Nonspherical Janus Particles Based on Polyhedral Oligomeric Silsesquioxanes: Molecular Design, “Click” Synthesis, and Hierarchical Structure
journal, July 2011
- Li, Yiwen; Zhang, Wen-Bin; Hsieh, I-Fan
- Journal of the American Chemical Society, Vol. 133, Issue 28
Pathway toward Large Two-Dimensional Hexagonally Patterned Colloidal Nanosheets in Solution
journal, January 2015
- Ni, Bo; Huang, Mingjun; Chen, Ziran
- Journal of the American Chemical Society, Vol. 137, Issue 4
Facile creation of FRET systems from a pH-responsive AIE fluorescent vesicle
journal, January 2016
- Wang, Xing; Yang, Yanyu; Zuo, Yunfei
- Chemical Communications, Vol. 52, Issue 30
Synthesis, Self-Assembly, and Photoresponsive Behavior of Tadpole-Shaped Azobenzene Polymers
journal, November 2015
- Wang, Xing; Yang, Yanyu; Gao, Peiyuan
- ACS Macro Letters, Vol. 4, Issue 12
POSS dendrimers constructed from a 1 → 7 branching monomer
journal, January 2014
- Wang, Xing; Yang, Yanyu; Gao, Peiyuan
- Chemical Communications, Vol. 50, Issue 46
Molecular-Curvature-Induced Spontaneous Formation of Curved and Concentric Lamellae through Nucleation
journal, January 2016
- Dong, Xue-Hui; Ni, Bo; Huang, Mingjun
- Angewandte Chemie International Edition, Vol. 55, Issue 7
Asymmetric Giant “Bolaform-like” Surfactants: Precise Synthesis, Phase Diagram, and Crystallization-Induced Phase Separation
journal, July 2014
- Wu, Kan; Huang, Mingjun; Yue, Kan
- Macromolecules, Vol. 47, Issue 14
Manipulation of Self-Assembled Nanostructure Dimensions in Molecular Janus Particles
journal, June 2016
- Liu, Hao; Luo, Jiancheng; Shan, Wenpeng
- ACS Nano, Vol. 10, Issue 7
Architecture, self-assembly and properties of well-defined hybrid polymers based on polyhedral oligomeric silsequioxane (POSS)
journal, August 2013
- Zhang, Weian; Müller, Axel H. E.
- Progress in Polymer Science, Vol. 38, Issue 8
Self-Assembly of Polymer Tethered Molecular Nanoparticle Shape Amphiphiles in Selective Solvents
journal, April 2015
- Ma, Shiying; Hu, Yi; Wang, Rong
- Macromolecules, Vol. 48, Issue 9
Simulating Microscopic Hydrodynamic Phenomena with Dissipative Particle Dynamics
journal, June 1992
- Hoogerbrugge, P. J.; Koelman, J. M. V. A.
- Europhysics Letters (EPL), Vol. 19, Issue 3
Dynamic Simulations of Hard-Sphere Suspensions Under Steady Shear
journal, January 1993
- Koelman, J. M. V. A.; Hoogerbrugge, P. J.
- Europhysics Letters (EPL), Vol. 21, Issue 3
A Supramolecular Janus Hyperbranched Polymer and Its Photoresponsive Self-Assembly of Vesicles with Narrow Size Distribution
journal, March 2013
- Liu, Yong; Yu, Chunyang; Jin, Haibao
- Journal of the American Chemical Society, Vol. 135, Issue 12
A Coarse-Grained Model for Polyethylene Oxide and Polyethylene Glycol: Conformation and Hydrodynamics
journal, October 2009
- Lee, Hwankyu; de Vries, Alex H.; Marrink, Siewert-Jan
- The Journal of Physical Chemistry B, Vol. 113, Issue 40
Controlled Self-Assembly Manipulated by Charge-Transfer Interactions: From Tubes to Vesicles
journal, November 2008
- Wang, Chao; Yin, Shouchun; Chen, Senlin
- Angewandte Chemie, Vol. 120, Issue 47
Hydrogel Formation upon Photoinduced Covalent Capture of Macrocycle Stacks from Dynamic Combinatorial Libraries
journal, July 2011
- Li, Jianwei; Carnall, Jacqui M. A.; Stuart, Marc C. A.
- Angewandte Chemie, Vol. 123, Issue 36
A Filled-Honeycomb-Structured Crystal Formed by Self-Assembly of a Janus Polyoxometalate-Silsesquioxane (POM-POSS) Co-Cluster
journal, November 2015
- Ma, Chi; Wu, Han; Huang, Zi-Han
- Angewandte Chemie, Vol. 127, Issue 52
Size evolution of highly amphiphilic macromolecular solution assemblies via a distinct bimodal pathway
journal, April 2014
- Kelley, Elizabeth G.; Murphy, Ryan P.; Seppala, Jonathan E.
- Nature Communications, Vol. 5, Issue 1
Reversibly Shape-Shifting Organic Optical Waveguides: Formation of Organic Nanorings, Nanotubes, and Nanosheets
journal, January 2012
- Chandrasekhar, Naisa; Chandrasekar, Rajadurai
- Angewandte Chemie, Vol. 124, Issue 15
Simulation-Assisted Self-Assembly of Multicomponent Polymers into Hierarchical Assemblies with Varied Morphologies
journal, June 2013
- Cai, Chunhua; Li, Yongliang; Lin, Jiaping
- Angewandte Chemie, Vol. 125, Issue 30
Controlling the Structure and Length of Self-Synthesizing Supramolecular Polymers through Nucleated Growth and Disassembly
journal, May 2015
- Pal, Asish; Malakoutikhah, Morteza; Leonetti, Giulia
- Angewandte Chemie, Vol. 127, Issue 27
Reversible Supramolecular Surface Attachment of Enzyme–Polymer Conjugates for the Design of Biocatalytic Filtration Membranes
journal, October 2015
- Moridi, Negar; Corvini, Philippe F. ‐X.; Shahgaldian, Patrick
- Angewandte Chemie, Vol. 127, Issue 49
Polymeric Nanoparticles Amenable to Simultaneous Installation of Exterior Targeting and Interior Therapeutic Proteins
journal, February 2016
- Zhu, Xi; Wu, Jun; Shan, Wei
- Angewandte Chemie, Vol. 128, Issue 10
Self-assembly of block copolymers
journal, August 1998
- Noolandi, Jaan; Shi, An-Chang
- Current Opinion in Colloid & Interface Science, Vol. 3, Issue 4
Molecular Biodynamers: Dynamic Covalent Analogues of Biopolymers
collection, January 2017
- Liu, Yun; Lehn, Jean-Marie; Hirsch, Anna
- Universität des Saarlandes
Bioinspired polymer vesicles and membranes for biological and medical applications
text, January 2016
- Palivan, Cornelia G.; Goers, Roland; Najer, Adrian
- Royal Society of Chemistry
Dynamic Combinatorial Chemistry
journal, November 2006
- Corbett, Peter T.; Leclaire, Julien; Vial, Laurent
- ChemInform, Vol. 37, Issue 48
Tuning the Amphiphilicity of Building Blocks: Controlled Self-Assembly and Disassembly for Functional Supramolecular Materials
journal, July 2009
- Wang, Yapei; Xu, Huaping; Zhang, Xi
- Advanced Materials, Vol. 21, Issue 28
Synthetic Self-Assembled Materials in Biological Environments
journal, April 2016
- Versluis, Frank; van Esch, Jan H.; Eelkema, Rienk
- Advanced Materials, Vol. 28, Issue 23
Hydrogel Formation upon Photoinduced Covalent Capture of Macrocycle Stacks from Dynamic Combinatorial Libraries
journal, July 2011
- Li, Jianwei; Carnall, Jacqui M. A.; Stuart, Marc C. A.
- Angewandte Chemie, Vol. 123, Issue 36
Reversibly Shape-Shifting Organic Optical Waveguides: Formation of Organic Nanorings, Nanotubes, and Nanosheets
journal, January 2012
- Chandrasekhar, Naisa; Chandrasekar, Rajadurai
- Angewandte Chemie, Vol. 124, Issue 15
Controlling the Structure and Length of Self-Synthesizing Supramolecular Polymers through Nucleated Growth and Disassembly
journal, May 2015
- Pal, Asish; Malakoutikhah, Morteza; Leonetti, Giulia
- Angewandte Chemie, Vol. 127, Issue 27
Reversible Supramolecular Surface Attachment of Enzyme–Polymer Conjugates for the Design of Biocatalytic Filtration Membranes
journal, October 2015
- Moridi, Negar; Corvini, Philippe F. ‐X.; Shahgaldian, Patrick
- Angewandte Chemie, Vol. 127, Issue 49
A Filled-Honeycomb-Structured Crystal Formed by Self-Assembly of a Janus Polyoxometalate-Silsesquioxane (POM-POSS) Co-Cluster
journal, November 2015
- Ma, Chi; Wu, Han; Huang, Zi-Han
- Angewandte Chemie, Vol. 127, Issue 52
Polymeric Nanoparticles Amenable to Simultaneous Installation of Exterior Targeting and Interior Therapeutic Proteins
journal, February 2016
- Zhu, Xi; Wu, Jun; Shan, Wei
- Angewandte Chemie International Edition, Vol. 55, Issue 10
Molecular-Curvature-Induced Spontaneous Formation of Curved and Concentric Lamellae through Nucleation
journal, January 2016
- Dong, Xue-Hui; Ni, Bo; Huang, Mingjun
- Angewandte Chemie International Edition, Vol. 55, Issue 7
Hierarchical Self-Assembly for Nanomedicine
journal, January 2016
- Bishop, Kyle J. M.
- Angewandte Chemie International Edition, Vol. 55, Issue 5
Cover Picture: Structurally Defined Molecular Hypervalent Iodine Catalysts for Intermolecular Enantioselective Reactions (Angew. Chem. Int. Ed. 1/2016)
journal, December 2015
- Haubenreisser, Stefan; Wöste, Thorsten H.; Martínez, Claudio
- Angewandte Chemie International Edition, Vol. 55, Issue 1
Kinetically Controlled Sequential Growth of Surface-Grafted Chiral Supramolecular Copolymers
journal, March 2016
- Frisch, Hendrik; Fritz, Eva-Corinna; Stricker, Friedrich
- Angewandte Chemie International Edition, Vol. 55, Issue 25
Atomically Precise Prediction of 2D Self-Assembly of Weakly Bonded Nanostructures: STM Insight into Concentration-Dependent Architectures
journal, November 2015
- El Garah, Mohamed; Dianat, Arezoo; Cadeddu, Andrea
- Small, Vol. 12, Issue 3
Architecture, self-assembly and properties of well-defined hybrid polymers based on polyhedral oligomeric silsequioxane (POSS)
journal, August 2013
- Zhang, Weian; Müller, Axel H. E.
- Progress in Polymer Science, Vol. 38, Issue 8
Molecular Biodynamers: Dynamic Covalent Analogues of Biopolymers
journal, January 2017
- Liu, Yun; Lehn, Jean-Marie; Hirsch, Anna K. H.
- Accounts of Chemical Research, Vol. 50, Issue 2
Fabrication of pH-Responsive Nanoparticles with an AIE Feature for Imaging Intracellular Drug Delivery
journal, August 2016
- Wang, Xing; Yang, Yanyu; Zhuang, Yaping
- Biomacromolecules, Vol. 17, Issue 9
Synthesis, Self-Assembly, and Photoresponsive Behavior of Tadpole-Shaped Azobenzene Polymers
journal, November 2015
- Wang, Xing; Yang, Yanyu; Gao, Peiyuan
- ACS Macro Letters, Vol. 4, Issue 12
Manipulation of Self-Assembled Nanostructure Dimensions in Molecular Janus Particles
journal, June 2016
- Liu, Hao; Luo, Jiancheng; Shan, Wenpeng
- ACS Nano, Vol. 10, Issue 7
Dynamic Combinatorial Chemistry
journal, September 2006
- Corbett, Peter T.; Leclaire, Julien; Vial, Laurent
- Chemical Reviews, Vol. 106, Issue 9
Supramolecular Coordination: Self-Assembly of Finite Two- and Three-Dimensional Ensembles
journal, November 2011
- Chakrabarty, Rajesh; Mukherjee, Partha Sarathi; Stang, Peter J.
- Chemical Reviews, Vol. 111, Issue 11, p. 6810-6918
Applications of Orthogonal “Click” Chemistries in the Synthesis of Functional Soft Materials
journal, November 2009
- Iha, Rhiannon K.; Wooley, Karen L.; Nyström, Andreas M.
- Chemical Reviews, Vol. 109, Issue 11
‘Living’ Controlled in Situ Gelling Systems: Thiol−Disulfide Exchange Method toward Tailor-Made Biodegradable Hydrogels
journal, November 2010
- Wu, De-Cheng; Loh, Xian Jun; Wu, Yun-Long
- Journal of the American Chemical Society, Vol. 132, Issue 43
A Giant Surfactant of Polystyrene−(Carboxylic Acid-Functionalized Polyhedral Oligomeric Silsesquioxane) Amphiphile with Highly Stretched Polystyrene Tails in Micellar Assemblies
journal, December 2010
- Yu, Xinfei; Zhong, Sheng; Li, Xiaopeng
- Journal of the American Chemical Society, Vol. 132, Issue 47
Dynamic Cylindrical Assembly of Triblock Copolymers by a Hierarchical Process of Covalent and Supramolecular Interactions
journal, February 2011
- Li, Zhou; Ma, Jun; Lee, Nam S.
- Journal of the American Chemical Society, Vol. 133, Issue 5
A Supramolecular Janus Hyperbranched Polymer and Its Photoresponsive Self-Assembly of Vesicles with Narrow Size Distribution
journal, March 2013
- Liu, Yong; Yu, Chunyang; Jin, Haibao
- Journal of the American Chemical Society, Vol. 135, Issue 12
Pathway toward Large Two-Dimensional Hexagonally Patterned Colloidal Nanosheets in Solution
journal, January 2015
- Ni, Bo; Huang, Mingjun; Chen, Ziran
- Journal of the American Chemical Society, Vol. 137, Issue 4
A Dual-Thermoresponsive Gemini-Type Supra-amphiphilic Macromolecular [3]Pseudorotaxane Based on Pillar[10]arene/Paraquat Cooperative Complexation
journal, February 2016
- Chi, Xiaodong; Yu, Guocan; Shao, Li
- Journal of the American Chemical Society, Vol. 138, Issue 9
Programming Self-Assembly of DNA Origami Honeycomb Two-Dimensional Lattices and Plasmonic Metamaterials
journal, June 2016
- Wang, Pengfei; Gaitanaros, Stavros; Lee, Seungwoo
- Journal of the American Chemical Society, Vol. 138, Issue 24
Synthesis of Nonequilibrium Supramolecular Peptide Polymers on a Microfluidic Platform
journal, July 2016
- Mason, Thomas O.; Michaels, Thomas C. T.; Levin, Aviad
- Journal of the American Chemical Society, Vol. 138, Issue 30
Nanoscale Control of Polymer Assembly on a Synthetic Catalyst–Bilayer System
journal, July 2016
- Gorgoll, Ricardo M.; Harano, Koji; Nakamura, Eiichi
- Journal of the American Chemical Society, Vol. 138, Issue 30
A Coarse-Grained Model for Polyethylene Oxide and Polyethylene Glycol: Conformation and Hydrodynamics
journal, October 2009
- Lee, Hwankyu; de Vries, Alex H.; Marrink, Siewert-Jan
- The Journal of Physical Chemistry B, Vol. 113, Issue 40
Self-Assembly of Polymer Tethered Molecular Nanoparticle Shape Amphiphiles in Selective Solvents
journal, April 2015
- Ma, Shiying; Hu, Yi; Wang, Rong
- Macromolecules, Vol. 48, Issue 9
Guided hierarchical co-assembly of soft patchy nanoparticles
journal, November 2013
- Gröschel, André H.; Walther, Andreas; Löbling, Tina I.
- Nature, Vol. 503, Issue 7475
Shape-shifting colloids via stimulated dewetting
journal, July 2016
- Youssef, Mena; Hueckel, Theodore; Yi, Gi-Ra
- Nature Communications, Vol. 7, Issue 1
Hierarchically structured transparent hybrid membranes by in situ growth of mesostructured organosilica in host polymer
journal, January 2006
- Vallé, Karine; Belleville, Philippe; Pereira, Franck
- Nature Materials, Vol. 5, Issue 2
Design of polymeric nanoparticles for biomedical delivery applications
journal, January 2012
- Elsabahy, Mahmoud; Wooley, Karen L.
- Chemical Society Reviews, Vol. 41, Issue 7
Self-assembly of block copolymers
journal, January 2012
- Mai, Yiyong; Eisenberg, Adi
- Chemical Society Reviews, Vol. 41, Issue 18
Controlled cross-linking strategy: from hybrid hydrogels to nanoparticle macroscopic aggregates
journal, January 2013
- Wang, Xing; Li, Dan; Yang, Fei
- Polymer Chemistry, Vol. 4, Issue 17
Block copolymer self-assembly for nanophotonics
journal, January 2015
- Stefik, Morgan; Guldin, Stefan; Vignolini, Silvia
- Chemical Society Reviews, Vol. 44, Issue 15
The influence of the dianhydride precursor in hyper-cross-linked hybrid polyPOSS-imide networks
journal, January 2016
- Neyertz, Sylvie; Brown, David; Raaijmakers, Michiel J. T.
- Physical Chemistry Chemical Physics, Vol. 18, Issue 41
Controlling amphiphilic copolymer self-assembly morphologies based on macrocycle/anion recognition and nucleotide-induced payload release
journal, January 2016
- Ji, Xiaofan; Wang, Hu; Li, Yang
- Chemical Science, Vol. 7, Issue 9
The Convergence of Synthetic Organic and Polymer Chemistries
journal, August 2005
- Hawker, C. J.
- Science, Vol. 309, Issue 5738
Block Copolymer Assembly via Kinetic Control
journal, August 2007
- Cui, H.; Chen, Z.; Zhong, S.
- Science, Vol. 317, Issue 5838
Transient laser heating induced hierarchical porous structures from block copolymer–directed self-assembly
journal, July 2015
- Tan, Kwan Wee; Jung, Byungki; Werner, Jörg G.
- Science, Vol. 349, Issue 6243
Simulating Microscopic Hydrodynamic Phenomena with Dissipative Particle Dynamics
journal, June 1992
- Hoogerbrugge, P. J.; Koelman, J. M. V. A.
- Europhysics Letters (EPL), Vol. 19, Issue 3
Dynamic Simulations of Hard-Sphere Suspensions Under Steady Shear
journal, January 1993
- Koelman, J. M. V. A.; Hoogerbrugge, P. J.
- Europhysics Letters (EPL), Vol. 21, Issue 3
Works referencing / citing this record:
Controllable hierarchical self-assembly of porphyrin-derived supra-amphiphiles
journal, March 2019
- Wang, Shu-Ping; Lin, Wei; Wang, Xiaolin
- Nature Communications, Vol. 10, Issue 1
Fabrication of POSS-embedded supramolecular hyperbranched polymers with multi-responsive morphology transitions
journal, January 2018
- Tang, Guoke; Wang, Xing; Li, Dawei
- Polymer Chemistry, Vol. 9, Issue 44
POSS-based supramolecular amphiphilic zwitterionic complexes for drug delivery
journal, January 2019
- Fan, Linfeng; Wang, Xing; Cao, Qingchen
- Biomaterials Science, Vol. 7, Issue 5
In situ bone regeneration enabled by a biodegradable hybrid double-network hydrogel
journal, January 2019
- Zhang, Yuanhao; Chen, Mingjiao; Tian, Jia
- Biomaterials Science, Vol. 7, Issue 8
Fabrication of zwitterionic and pH-responsive polyacetal dendrimers for anticancer drug delivery
journal, January 2019
- Wang, Yaqiang; Huang, Da; Wang, Xing
- Biomaterials Science, Vol. 7, Issue 8
Self-Assembly and Applications of Amphiphilic Hybrid POSS Copolymers
journal, September 2018
- Chi, Hong; Wang, Mingyue; Xiao, Yiting
- Molecules, Vol. 23, Issue 10
Controllable hierarchical self-assembly of porphyrin-derived supra-amphiphiles
journal, March 2019
- Wang, Shu-Ping; Lin, Wei; Wang, Xiaolin
- Nature Communications, Vol. 10, Issue 1
Fabrication of Customized Nanogel Carriers From a UV-Triggered Dynamic Self-Assembly Strategy
journal, November 2019
- Bao, Wuren; Lyu, Jieran; Li, Chunlin
- Frontiers in Chemistry, Vol. 7
Progressive 3D Printing Technology and Its Application in Medical Materials
journal, March 2020
- Fan, Daoyang; Li, Yan; Wang, Xing
- Frontiers in Pharmacology, Vol. 11
Self-Assembly and Applications of Amphiphilic Hybrid POSS Copolymers
journal, September 2018
- Chi, Hong; Wang, Mingyue; Xiao, Yiting
- Molecules, Vol. 23, Issue 10