Anisotropic susceptibilities in the honeycomb Kitaev system
Abstract
The magnetic insulator is a promising candidate to realize Kitaev interactions on a quasi-two-dimensional honeycomb lattice. We perform extensive susceptibility measurements on single crystals of , including angle dependence of the in-plane longitudinal and transverse susceptibilities, which reveal a unidirectional anisotropy within the honeycomb plane. By comparing the experimental results to a high-temperature expansion of a Kitaev-Heisenberg-$$\textbf{Γ}$$ spin Hamiltonian with bond anisotropy, we find excellent agreement with the observed phase shift and periodicity of the angle-resolved susceptibilities. Within this model, we show that the pronounced difference between in-plane and out-of-plane susceptibilities as well as the finite transverse susceptibility are rooted in strong symmetric off-diagonal $$\textbf{Γ}$$ spin exchange. The $$\textbf{Γ}$$ couplings and relationships between other terms in the model Hamiltonian are quantified by extracting relevant Curie-Weiss intercepts from the experimental data.
- Authors:
-
- Univ. of Tennessee, Knoxville, TN (United States). Dept. of Materials Science and Engineering; Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division
- Univ. of Melbourne (Australia). School of Physics; Technical Univ. of Dresden (Germany). Inst. of Theoretical Physics
- Freie Univ., Berlin (Germany). Dahlem Center for Complex Quantum Systems and Dept. of Physics; Helmholtz-Zentrum Berlin (HZB), (Germany). German Research Centre for Materials and Energy
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Division
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Chemical Sciences Division
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; Gordon and Betty Moore Foundation; German Research Foundation (DFG)
- OSTI Identifier:
- 1474459
- Alternate Identifier(s):
- OSTI ID: 1469737
- Grant/Contract Number:
- AC05-00OR22725; GBMF4416; SFB 1143
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 98; Journal Issue: 10; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; magnetic anisotropy; quantum spin liquid; DC susceptibility measurements; Kitaev-Heisenberg model
Citation Formats
Lampen-Kelley, Paula J., Rachel, S., Reuther, J., Yan, Jiaqiang -Q., Banerjee, Arnab, Bridges, Craig A., Cao, Huibo B., Nagler, Stephen E., and Mandrus, D. Anisotropic susceptibilities in the honeycomb Kitaev system α-RuCl3. United States: N. p., 2018.
Web. doi:10.1103/PhysRevB.98.100403.
Lampen-Kelley, Paula J., Rachel, S., Reuther, J., Yan, Jiaqiang -Q., Banerjee, Arnab, Bridges, Craig A., Cao, Huibo B., Nagler, Stephen E., & Mandrus, D. Anisotropic susceptibilities in the honeycomb Kitaev system α-RuCl3. United States. https://doi.org/10.1103/PhysRevB.98.100403
Lampen-Kelley, Paula J., Rachel, S., Reuther, J., Yan, Jiaqiang -Q., Banerjee, Arnab, Bridges, Craig A., Cao, Huibo B., Nagler, Stephen E., and Mandrus, D. Wed .
"Anisotropic susceptibilities in the honeycomb Kitaev system α-RuCl3". United States. https://doi.org/10.1103/PhysRevB.98.100403. https://www.osti.gov/servlets/purl/1474459.
@article{osti_1474459,
title = {Anisotropic susceptibilities in the honeycomb Kitaev system α-RuCl3},
author = {Lampen-Kelley, Paula J. and Rachel, S. and Reuther, J. and Yan, Jiaqiang -Q. and Banerjee, Arnab and Bridges, Craig A. and Cao, Huibo B. and Nagler, Stephen E. and Mandrus, D.},
abstractNote = {The magnetic insulator α-RuCl3 is a promising candidate to realize Kitaev interactions on a quasi-two-dimensional honeycomb lattice. We perform extensive susceptibility measurements on single crystals of α-RuCl3, including angle dependence of the in-plane longitudinal and transverse susceptibilities, which reveal a unidirectional anisotropy within the honeycomb plane. By comparing the experimental results to a high-temperature expansion of a Kitaev-Heisenberg-$\textbf{Γ}$ spin Hamiltonian with bond anisotropy, we find excellent agreement with the observed phase shift and periodicity of the angle-resolved susceptibilities. Within this model, we show that the pronounced difference between in-plane and out-of-plane susceptibilities as well as the finite transverse susceptibility are rooted in strong symmetric off-diagonal $\textbf{Γ}$ spin exchange. The $\textbf{Γ}$ couplings and relationships between other terms in the model Hamiltonian are quantified by extracting relevant Curie-Weiss intercepts from the experimental data.},
doi = {10.1103/PhysRevB.98.100403},
journal = {Physical Review B},
number = 10,
volume = 98,
place = {United States},
year = {Wed Sep 12 00:00:00 EDT 2018},
month = {Wed Sep 12 00:00:00 EDT 2018}
}
Web of Science
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Works referencing / citing this record:
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