Frustrated magnetic interactions in an bilayer honeycomb lattice compound ( )
Abstract
An inelastic neutron scattering study has been performed in an bilayer honeycomb lattice compound ( ) at ambient and high magnetic fields. Relatively broad and monotonically dispersive magnetic excitations were observed at ambient field, where no long-range magnetic order exists. In the magnetic-field-induced long-range ordered state at 10 T, the magnetic dispersions become slightly more intense, albeit still broad as in the disordered state, and two excitation gaps, probably originating from an easy-plane magnetic anisotropy and intrabilayer interactions, develop. Here, analyzing the magnetic dispersions using the linear spin-wave theory, we estimated the intraplane and intrabilayer magnetic interactions, which are almost consistent with those determined by ab initio density functional theory calculations, except the third and fourth neighbor intrabilayer interactions. Most importantly, as predicted by the theory, there is no significant frustration in the honeycomb plane but frustrating intrabilayer interactions probably give rise to the disordered ground state.
- Authors:
-
[1];
[2];
[1];
[3];
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Duke Univ., Durham, NC (United States)
- National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
- Univ. of Yamanashi, Kofu (Japan)
- Tokyo Inst. of Technology, Yokohama (Japan)
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1571846
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 100; Journal Issue: 13; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Matsuda, Masaaki, Dissanayake, Sachith E., Abernathy, Douglas L., Qiu, Y., Copley, J. R. D., Kumada, N., and Azuma, Masaki. Frustrated magnetic interactions in an S=3/2 bilayer honeycomb lattice compound Bi3Mn4O12 (NO3). United States: N. p., 2019.
Web. doi:10.1103/PhysRevB.100.134430.
Matsuda, Masaaki, Dissanayake, Sachith E., Abernathy, Douglas L., Qiu, Y., Copley, J. R. D., Kumada, N., & Azuma, Masaki. Frustrated magnetic interactions in an S=3/2 bilayer honeycomb lattice compound Bi3Mn4O12 (NO3). United States. https://doi.org/10.1103/PhysRevB.100.134430
Matsuda, Masaaki, Dissanayake, Sachith E., Abernathy, Douglas L., Qiu, Y., Copley, J. R. D., Kumada, N., and Azuma, Masaki. Tue .
"Frustrated magnetic interactions in an S=3/2 bilayer honeycomb lattice compound Bi3Mn4O12 (NO3)". United States. https://doi.org/10.1103/PhysRevB.100.134430. https://www.osti.gov/servlets/purl/1571846.
@article{osti_1571846,
title = {Frustrated magnetic interactions in an S=3/2 bilayer honeycomb lattice compound Bi3Mn4O12 (NO3)},
author = {Matsuda, Masaaki and Dissanayake, Sachith E. and Abernathy, Douglas L. and Qiu, Y. and Copley, J. R. D. and Kumada, N. and Azuma, Masaki},
abstractNote = {An inelastic neutron scattering study has been performed in an S=3/2 bilayer honeycomb lattice compound Bi3Mn4O12 (NO3) at ambient and high magnetic fields. Relatively broad and monotonically dispersive magnetic excitations were observed at ambient field, where no long-range magnetic order exists. In the magnetic-field-induced long-range ordered state at 10 T, the magnetic dispersions become slightly more intense, albeit still broad as in the disordered state, and two excitation gaps, probably originating from an easy-plane magnetic anisotropy and intrabilayer interactions, develop. Here, analyzing the magnetic dispersions using the linear spin-wave theory, we estimated the intraplane and intrabilayer magnetic interactions, which are almost consistent with those determined by ab initio density functional theory calculations, except the third and fourth neighbor intrabilayer interactions. Most importantly, as predicted by the theory, there is no significant frustration in the honeycomb plane but frustrating intrabilayer interactions probably give rise to the disordered ground state.},
doi = {10.1103/PhysRevB.100.134430},
journal = {Physical Review B},
number = 13,
volume = 100,
place = {United States},
year = {2019},
month = {10}
}
Free Publicly Available Full Text
Publisher's Version of Record
Other availability
Search WorldCat to find libraries that may hold this journal
Cited by: 4 works
Citation information provided by
Web of Science
Web of Science
Figures / Tables:
FIG. 1: Schematic structure of the honeycomb bilayer in Bi3Mn4O12(NO3). The open circles represent the Mn4+ moments. Magnetic interactions in a honeycomb plane $J$1 (bold solid line), $J$2(dashed line), and $J$3 (long dashed dotted line) (a) and intrabilayer interactions $J$1c (bold solid line), $J$2c (dashed line), $J$3c (long dashed dottedmore »
All figures and tables
(7 total)
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
Nature of the Spin Liquid State of the Hubbard Model on a Honeycomb Lattice
journal, August 2011
- Clark, B. K.; Abanin, D. A.; Sondhi, S. L.
- Physical Review Letters, Vol. 107, Issue 8
The Disk Chopper Spectrometer at NIST: a new instrument for quasielastic neutron scattering studies
journal, August 2003
- Copley, J. R. D.; Cook, J. C.
- Chemical Physics, Vol. 292, Issue 2-3
Phase diagram of a frustrated quantum antiferromagnet on the honeycomb lattice: Magnetic order versus valence-bond crystal formation
journal, July 2011
- Albuquerque, A. F.; Schwandt, D.; Hetényi, B.
- Physical Review B, Vol. 84, Issue 2
Anyons in an exactly solved model and beyond
journal, January 2006
- Kitaev, Alexei
- Annals of Physics, Vol. 321, Issue 1
DAVE: A Comprehensive Software Suite for the Reduction, Visualization, and Analysis of Low Energy Neutron Spectroscopic Data
journal, November 2009
- Azuah, Richard Tumanjong; Kneller, Larry R.; Qiu, Yiming
- Journal of Research of the National Institute of Standards and Technology, Vol. 114, Issue 6
Spiral order by disorder and lattice nematic order in a frustrated Heisenberg antiferromagnet on the honeycomb lattice
journal, June 2010
- Mulder, A.; Ganesh, R.; Capriotti, L.
- Physical Review B, Vol. 81, Issue 21
Broken discrete symmetries in a frustrated honeycomb antiferromagnet
journal, March 2013
- Rosales, H. D.; Cabra, D. C.; Lamas, C. A.
- Physical Review B, Vol. 87, Issue 10
Ground-state properties, excitation spectra, and phase transitions in the and bilayer Heisenberg models on the honeycomb lattice
journal, January 2012
- Oitmaa, J.; Singh, R. R. P.
- Physical Review B, Vol. 85, Issue 1
spin liquid and chiral antiferromagnetic phase in the Hubbard model on a honeycomb lattice
journal, July 2011
- Lu, Yuan-Ming; Ran, Ying
- Physical Review B, Vol. 84, Issue 2
Synthesis, Crystal Structure, and Magnetic Properties of Bi 3 Mn 4 O 12 (NO 3 ) Oxynitrate Comprising S = 3/2 Honeycomb Lattice
journal, June 2009
- Smirnova, Olga; Azuma, Masaki; Kumada, Nobuhiro
- Journal of the American Chemical Society, Vol. 131, Issue 23
Origin of magnetic frustration in
journal, October 2017
- Alaei, Mojtaba; Mosadeq, Hamid; Sarsari, Ismaeil Abdolhosseini
- Physical Review B, Vol. 96, Issue 14
Dzyaloshinsky-Moriya interaction and field-induced magnetic order in an antiferromagnetic honeycomb lattice compound Bi Mn O (NO ) studied by high-field electron spin resonance
journal, October 2012
- Okubo, Susumu; Ueda, Tomonari; Ohta, Hitoshi
- Physical Review B, Vol. 86, Issue 14
Néel to dimer transition in spin- antiferromagnets: Comparing bond operator theory with quantum Monte Carlo simulations for bilayer Heisenberg models
journal, December 2011
- Ganesh, R.; Isakov, Sergei V.; Paramekanti, Arun
- Physical Review B, Vol. 84, Issue 21
Quantum phases in the frustrated Heisenberg model on the bilayer honeycomb lattice
journal, January 2014
- Zhang, Hao; Arlego, M.; Lamas, C. A.
- Physical Review B, Vol. 89, Issue 2
Quantum paramagnetic ground states on the honeycomb lattice and field-induced Néel order
journal, April 2011
- Ganesh, R.; Sheng, D. N.; Kim, Young-June
- Physical Review B, Vol. 83, Issue 14
Calculation of magnetic exchange couplings in the honeycomb system (Bi Mn O )NO from first principles
journal, April 2011
- Kandpal, Hem C.; van den Brink, Jeroen
- Physical Review B, Vol. 83, Issue 14
Magnetic ground state of the frustrated honeycomb lattice antiferromagnet Bi Mn O (NO )
journal, May 2012
- Onishi, N.; Oka, K.; Azuma, M.
- Physical Review B, Vol. 85, Issue 18
Complete phase diagram of the spin- - - model (with = ) on the honeycomb lattice
journal, April 2012
- Bishop, R. F.; Li, P. H. Y.
- Physical Review B, Vol. 85, Issue 15
Deconfined Criticality in the Frustrated Heisenberg Honeycomb Antiferromagnet
journal, March 2013
- Ganesh, R.; van den Brink, Jeroen; Nishimoto, Satoshi
- Physical Review Letters, Vol. 110, Issue 12
Unexpected -Direction Ising Antiferromagnetic Order in a Frustrated Spin- Model on the Honeycomb Lattice
journal, December 2013
- Zhu, Zhenyue; Huse, David A.; White, Steven R.
- Physical Review Letters, Vol. 111, Issue 25
Weak Plaquette Valence Bond Order in the Honeycomb Heisenberg Model
journal, March 2013
- Zhu, Zhenyue; Huse, David A.; White, Steven R.
- Physical Review Letters, Vol. 110, Issue 12
Design and operation of the wide angular-range chopper spectrometer ARCS at the Spallation Neutron Source
journal, January 2012
- Abernathy, D. L.; Stone, M. B.; Loguillo, M. J.
- Review of Scientific Instruments, Vol. 83, Issue 1
Quantum disordered phase on the frustrated honeycomb lattice
journal, March 2011
- Cabra, D. C.; Lamas, C. A.; Rosales, H. D.
- Physical Review B, Vol. 83, Issue 9
Short and Long Range Magnetic Ordering in β-MnO 2 –A Temperature Study–
journal, December 2004
- Regulski, Marcin; Przeniosło, Radosław; Sosnowska, Izabela
- Journal of the Physical Society of Japan, Vol. 73, Issue 12
Disordered Ground State and Magnetic Field-Induced Long-Range Order in an Antiferromagnetic Honeycomb Lattice Compound
journal, October 2010
- Matsuda, M.; Azuma, M.; Tokunaga, M.
- Physical Review Letters, Vol. 105, Issue 18
Neutron-scattering study of antiferromagnetism in
journal, November 1993
- Shamoto, S.; Sato, M.; Tranquada, J. M.
- Physical Review B, Vol. 48, Issue 18
Field-induced multiple order-by-disorder state selection in an antiferromagnetic honeycomb bilayer lattice
journal, April 2016
- Gómez Albarracín, F. A.; Rosales, H. D.
- Physical Review B, Vol. 93, Issue 14
Magnetic Structure of β -MnO 2 : X-ray Magnetic Scattering Study
journal, January 2001
- Sato, Hirohiko; Wakiya, Koji; Enoki, Toshiaki
- Journal of the Physical Society of Japan, Vol. 70, Issue 1
Linear spin wave theory for single-Q incommensurate magnetic structures
journal, March 2015
- Toth, S.; Lake, B.
- Journal of Physics: Condensed Matter, Vol. 27, Issue 16
Quantum phase diagram of a frustrated antiferromagnet on the bilayer honeycomb lattice
journal, June 2016
- Zhang, Hao; Lamas, Carlos A.; Arlego, Marcelo
- Physical Review B, Vol. 93, Issue 23
Spin-gap phase of a quantum spin system on a honeycomb lattice
journal, October 2006
- Takano, Ken’ichi
- Physical Review B, Vol. 74, Issue 14
The ground states of the classical heisenberg and planar models on the triangular and plane hexagonal lattices
journal, February 1986
- Katsura, Shigetoshi; Ide, Tsugio; Morita, Tohru
- Journal of Statistical Physics, Vol. 42, Issue 3-4
Plaquette valence bond ordering in a J 1 – J 2 Heisenberg antiferromagnet on a honeycomb lattice
journal, May 2011
- Mosadeq, H.; Shahbazi, F.; Jafari, S. A.
- Journal of Physics: Condensed Matter, Vol. 23, Issue 22
Novel Spin-Liquid States in the Frustrated Heisenberg Antiferromagnet on the Honeycomb Lattice
journal, November 2010
- Okumura, Soichiro; Kawamura, Hikaru; Okubo, Tsuyoshi
- Journal of the Physical Society of Japan, Vol. 79, Issue 11
Exotic disordered phases in the quantum - model on the honeycomb lattice
journal, January 2013
- Zhang, Hao; Lamas, C. A.
- Physical Review B, Vol. 87, Issue 2
Impact of Mn–O–O–Mn superexchange pathways in a honeycomb lattice Mn oxide with small charge-transfer energy
journal, May 2013
- Wadati, H.; Kato, K.; Wakisaka, Y.
- Solid State Communications, Vol. 162
Schwinger boson mean field theories of spin liquid states on a honeycomb lattice: Projective symmetry group analysis and critical field theory
journal, July 2010
- Wang, Fa
- Physical Review B, Vol. 82, Issue 2
Quantum disordered phase on the frustrated honeycomb lattice
text, January 2010
- Cabra, D. C.; Lamas, C. A.; Rosales, H. D.
- arXiv
Spiral order by disorder and lattice nematic order in a frustrated Heisenberg antiferromagnet on the honeycomb lattice
text, January 2010
- Mulder, A.; Ganesh, R.; Capriotti, L.
- arXiv
Novel spin-liquid states in the frustrated Heisenberg antiferromagnet on the honeycomb lattice
text, January 2010
- Okumura, Soichiro; Kawamura, Hikaru; Okubo, Tsuyoshi
- arXiv
Plaquette valence-bond ordering in J_1-J_2 Heisenberg antiferromagnet on the honeycomb lattice
text, January 2010
- Mosadeq, H.; Shahbazi, F.; Jafari, S. A.
- arXiv
Calculation of magnetic exchange couplings in S=3/2 honeycomb system Bi$_3$Mn$_4$O$_{12}$(NO$_3$)} from first principles
text, January 2011
- Kandpal, Hem C.; Brink, Jeroen van den
- arXiv
Phase Diagram of a Frustrated Quantum Antiferromagnet on the Honeycomb Lattice: Magnetic Order versus Valence-Bond Crystal formation
text, January 2011
- Albuquerque, A. F.; Schwandt, D.; Hetényi, B.
- arXiv
Deconfined criticality in the frustrated Heisenberg honeycomb antiferromagnet
text, January 2013
- Ganesh, R.; Brink, Jeroen van den; Nishimoto, Satoshi
- arXiv
Linear spin wave theory for single-Q incommensurate magnetic structures
text, January 2014
- Toth, S.; Lake, B.
- arXiv
Field induced multiple order-by-disorder state selection in antiferromagnetic honeycomb bilayer lattice
text, January 2015
- Albarracín, F. A. Gómez; Rosales, H. D.
- arXiv
Quantum phase diagram of a frustrated antiferromagnet on the bilayer honeycomb lattice
text, January 2015
- Zhang, Hao; Lamas, Carlos A.; Arlego, Marcelo
- arXiv
Origin of magnetic frustration in Bi$_3$Mn$_4$O$_{12}$(NO$_3$)
text, January 2017
- Alaei, Mojtaba; Mosadeq, Hamid; Sarsari, Ismail Abdolhossaini
- arXiv
Figures / Tables found in this record:
Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.