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Title: Unprecedented quality factors at accelerating gradients up to 45 MVm −1 in niobium superconducting resonators via low temperature nitrogen infusion

Abstract

Here, we report the finding of new surface treatments that permit to manipulate the niobium resonator nitrogen content in the first few nanometers in a controlled way, and the resonator fundamental Mattis-Bardeen surface resistance and residual resistance accordingly. In particular, we find surface infusion conditions that systematically a) increase the quality factor of these 1.3 GHz superconducting radio frequency (SRF) bulk niobium resonators, up to very high gradients; b) increase the achievable accelerating gradient of the cavity compared to its own baseline with state-of-the-art surface processing. Cavities subject to the new surface process have larger than two times the state of the art Q at 2K for accelerating fields > 35 MV/m. Moreover, very high accelerating gradients ~ 45 MV/m are repeatedly reached, which correspond to peak magnetic surface fields of 190 mT, among the highest measured for bulk niobium cavities. These findings open the opportunity to tailor the surface impurity content distribution to maximize performance in Q and gradients, and have therefore very important implications on future performance and cost of SRF based accelerators. They also help deepen the understanding of the physics of the RF niobium cavity surface.

Authors:
; ; ; ; ; ; ; ; ; ; ;
Publication Date:
Research Org.:
Fermi National Accelerator Laboratory (FNAL), Batavia, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), High Energy Physics (HEP)
OSTI Identifier:
1437715
Alternate Identifier(s):
OSTI ID: 1407126
Report Number(s):
arXiv:1701.06077; FERMILAB-PUB-17-458-TD
Journal ID: ISSN 0953-2048
Grant/Contract Number:  
Early Career Award "Impurity D; GARD Program; AC02-07CH11359
Resource Type:
Published Article
Journal Name:
Superconductor Science and Technology
Additional Journal Information:
Journal Name: Superconductor Science and Technology Journal Volume: 30 Journal Issue: 9; Journal ID: ISSN 0953-2048
Publisher:
IOP Publishing
Country of Publication:
United Kingdom
Language:
English
Subject:
43 PARTICLE ACCELERATORS; SRF; nitrogen doping; nitrogen infusion; high Q; high accelerating gradient; radio frequency surface resistance

Citation Formats

Grassellino, A., Romanenko, A., Trenikhina, Y., Checchin, M., Martinello, M., Melnychuk, O. S., Chandrasekaran, S., Sergatskov, D. A., Posen, S., Crawford, A. C., Aderhold, S., and Bice, D. Unprecedented quality factors at accelerating gradients up to 45 MVm −1 in niobium superconducting resonators via low temperature nitrogen infusion. United Kingdom: N. p., 2017. Web. doi:10.1088/1361-6668/aa7afe.
Grassellino, A., Romanenko, A., Trenikhina, Y., Checchin, M., Martinello, M., Melnychuk, O. S., Chandrasekaran, S., Sergatskov, D. A., Posen, S., Crawford, A. C., Aderhold, S., & Bice, D. Unprecedented quality factors at accelerating gradients up to 45 MVm −1 in niobium superconducting resonators via low temperature nitrogen infusion. United Kingdom. https://doi.org/10.1088/1361-6668/aa7afe
Grassellino, A., Romanenko, A., Trenikhina, Y., Checchin, M., Martinello, M., Melnychuk, O. S., Chandrasekaran, S., Sergatskov, D. A., Posen, S., Crawford, A. C., Aderhold, S., and Bice, D. Mon . "Unprecedented quality factors at accelerating gradients up to 45 MVm −1 in niobium superconducting resonators via low temperature nitrogen infusion". United Kingdom. https://doi.org/10.1088/1361-6668/aa7afe.
@article{osti_1437715,
title = {Unprecedented quality factors at accelerating gradients up to 45 MVm −1 in niobium superconducting resonators via low temperature nitrogen infusion},
author = {Grassellino, A. and Romanenko, A. and Trenikhina, Y. and Checchin, M. and Martinello, M. and Melnychuk, O. S. and Chandrasekaran, S. and Sergatskov, D. A. and Posen, S. and Crawford, A. C. and Aderhold, S. and Bice, D.},
abstractNote = {Here, we report the finding of new surface treatments that permit to manipulate the niobium resonator nitrogen content in the first few nanometers in a controlled way, and the resonator fundamental Mattis-Bardeen surface resistance and residual resistance accordingly. In particular, we find surface infusion conditions that systematically a) increase the quality factor of these 1.3 GHz superconducting radio frequency (SRF) bulk niobium resonators, up to very high gradients; b) increase the achievable accelerating gradient of the cavity compared to its own baseline with state-of-the-art surface processing. Cavities subject to the new surface process have larger than two times the state of the art Q at 2K for accelerating fields > 35 MV/m. Moreover, very high accelerating gradients ~ 45 MV/m are repeatedly reached, which correspond to peak magnetic surface fields of 190 mT, among the highest measured for bulk niobium cavities. These findings open the opportunity to tailor the surface impurity content distribution to maximize performance in Q and gradients, and have therefore very important implications on future performance and cost of SRF based accelerators. They also help deepen the understanding of the physics of the RF niobium cavity surface.},
doi = {10.1088/1361-6668/aa7afe},
journal = {Superconductor Science and Technology},
number = 9,
volume = 30,
place = {United Kingdom},
year = {Mon Aug 14 00:00:00 EDT 2017},
month = {Mon Aug 14 00:00:00 EDT 2017}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1088/1361-6668/aa7afe

Citation Metrics:
Cited by: 82 works
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Works referencing / citing this record:

Vacancy-Hydrogen Interaction in Niobium during Low-Temperature Baking
journal, May 2020


Niobium near-surface composition during nitrogen infusion relevant for superconducting radio-frequency cavities
text, January 2019

  • Semione, G. D. L.; Dangwal Pandey, Arti; Tober, Steffen
  • Deutsches Elektronen-Synchrotron, DESY, Hamburg
  • DOI: 10.3204/pubdb-2019-04335

Surface characterization of nitrogen-doped Nb (100) large-grain superconducting RF cavity material
journal, April 2018

  • Dangwal Pandey, Arti; Dalla Lana Semione, Guilherme; Prudnikava, Alena
  • Journal of Materials Science, Vol. 53, Issue 14
  • DOI: 10.1007/s10853-018-2310-8

OFHC copper substrates for niobium sputtering: comparison of chemical etching recipes
journal, January 2020


The International Linear Collider
journal, February 2019


Evidence for preferential flux flow at the grain boundaries of superconducting RF-quality niobium
journal, February 2018

  • Sung, Z-H; Lee, P. J.; Gurevich, A.
  • Superconductor Science and Technology, Vol. 31, Issue 4
  • DOI: 10.1088/1361-6668/aaa65d

Improvement of accelerating gradients in niobium quarter wave resonators
journal, July 2019

  • Rai, A.; Potukuchi, P. N.; Patra, P.
  • Superconductor Science and Technology, Vol. 32, Issue 9
  • DOI: 10.1088/1361-6668/ab2794

High-brilliance, high-flux compact inverse Compton light source
journal, August 2018


Vacancy-Hydrogen Interaction in Niobium during Low-Temperature Baking
text, January 2020

  • Wenskat, Marc; Cizek, Jakub; Liedke, Maciej Oskar
  • Deutsches Elektronen-Synchrotron, DESY, Hamburg
  • DOI: 10.3204/pubdb-2020-02437