MoS2-on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries
Abstract
Two-dimensional (2D) heterostructured materials, combining the collective advantages of individual building blocks and synergistic properties, have spurred great interest as a new paradigm in materials science. The family of 2D transition-metal carbides and nitrides, MXenes, has emerged as an attractive platform to construct functional materials with enhanced performance for diverse applications. Here, we synthesized 2D MoS2-on-MXene heterostructures through in situ sulfidation of Mo2TiC2Tx MXene. The computational results show that MoS2-on-MXene heterostructures have metallic properties. Moreover, the presence of MXene leads to enhanced Li and Li2S adsorption during the intercalation and conversion reactions. These characteristics render the as-prepared MoS2-on-MXene heterostructures stable Li-ion storage performance. In conclusion, this work paves the way to use MXene to construct 2D heterostructures for energy storage applications.
- Authors:
-
[2];
[2];
[2]
- Drexel Univ., Philadelphia, PA (United States). A. J. Drexel Nanomaterials Inst., Materials Science and Engineering Dept.; Huazhong Univ. of Science and Technology, Wuhan (China). School of Optical and Electronic Information
- Drexel Univ., Philadelphia, PA (United States). A. J. Drexel Nanomaterials Inst., Materials Science and Engineering Dept.
- Huazhong Univ. of Science and Technology, Wuhan (China). School of Optical and Electronic Information
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Energy Frontier Research Centers (EFRC) (United States). Fluid Interface Reactions, Structures and Transport Center (FIRST)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1435245
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Angewandte Chemie (International Edition)
- Additional Journal Information:
- Journal Name: Angewandte Chemie (International Edition); Journal Volume: 57; Journal Issue: 7; Journal ID: ISSN 1433-7851
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; 36 MATERIALS SCIENCE; density functional theory; heterostructures; lithium-ion batteries; molybdenum disulfide; MXenes
Citation Formats
Chen, Chi, Xie, Xiuqiang, Anasori, Babak, Sarycheva, Asya, Makaryan, Taron, Zhao, Mengqiang, Urbankowski, Patrick, Miao, Ling, Jiang, Jianjun, and Gogotsi, Yury. MoS2-on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries. United States: N. p., 2018.
Web. doi:10.1002/anie.201710616.
Chen, Chi, Xie, Xiuqiang, Anasori, Babak, Sarycheva, Asya, Makaryan, Taron, Zhao, Mengqiang, Urbankowski, Patrick, Miao, Ling, Jiang, Jianjun, & Gogotsi, Yury. MoS2-on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries. United States. https://doi.org/10.1002/anie.201710616
Chen, Chi, Xie, Xiuqiang, Anasori, Babak, Sarycheva, Asya, Makaryan, Taron, Zhao, Mengqiang, Urbankowski, Patrick, Miao, Ling, Jiang, Jianjun, and Gogotsi, Yury. Tue .
"MoS2-on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries". United States. https://doi.org/10.1002/anie.201710616. https://www.osti.gov/servlets/purl/1435245.
@article{osti_1435245,
title = {MoS2-on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries},
author = {Chen, Chi and Xie, Xiuqiang and Anasori, Babak and Sarycheva, Asya and Makaryan, Taron and Zhao, Mengqiang and Urbankowski, Patrick and Miao, Ling and Jiang, Jianjun and Gogotsi, Yury},
abstractNote = {Two-dimensional (2D) heterostructured materials, combining the collective advantages of individual building blocks and synergistic properties, have spurred great interest as a new paradigm in materials science. The family of 2D transition-metal carbides and nitrides, MXenes, has emerged as an attractive platform to construct functional materials with enhanced performance for diverse applications. Here, we synthesized 2D MoS2-on-MXene heterostructures through in situ sulfidation of Mo2TiC2Tx MXene. The computational results show that MoS2-on-MXene heterostructures have metallic properties. Moreover, the presence of MXene leads to enhanced Li and Li2S adsorption during the intercalation and conversion reactions. These characteristics render the as-prepared MoS2-on-MXene heterostructures stable Li-ion storage performance. In conclusion, this work paves the way to use MXene to construct 2D heterostructures for energy storage applications.},
doi = {10.1002/anie.201710616},
journal = {Angewandte Chemie (International Edition)},
number = 7,
volume = 57,
place = {United States},
year = {Tue Jan 02 00:00:00 EST 2018},
month = {Tue Jan 02 00:00:00 EST 2018}
}
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Figures / Tables:
Figure 1.: a) Schematic illustration of the preparation of MoS2/MXenehybrids. S/Mo2TiC2Tx hybrids were obtained by a liquid mixing process(left panel). Then the sulfur loaded MXene (middle panel) was head treated to obtain MoS2-on-MXene heterostructures (right panel). b) Raman spectra and c) XRD patterns of pure Mo2TiC2Tx, MoS2/Mo2TiC2Tx-500 and MoS2/Mo2TiC2Tx-700.
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Enhanced reversible capability of a macroporous ZnMn 2 O 4 /C microsphere anode with a water-soluble binder for long-life and high-rate lithium-ion storage
journal, January 2019
- Li, Huan; Yang, Tianbo; Jin, Bo
- Inorganic Chemistry Frontiers, Vol. 6, Issue 6
A general way to fabricate transition metal dichalcogenide/oxide-sandwiched MXene nanosheets as flexible film anodes for high-performance lithium storage
journal, January 2019
- Wang, Chuang; Zhu, Xiao-Dong; Wang, Ke-Xin
- Sustainable Energy & Fuels, Vol. 3, Issue 10
The dual-function sacrificing template directed formation of MoS 2 /C hybrid nanotubes enabling highly stable and ultrafast sodium storage
journal, January 2019
- Gao, Jingyu; Li, Yapeng; Liu, Yi
- Journal of Materials Chemistry A, Vol. 7, Issue 32
Multiple roles of a heterointerface in two-dimensional van der Waals heterostructures: insights into energy-related applications
journal, January 2019
- Zhu, Yuanzhi; Peng, Wenchao; Li, Yang
- Journal of Materials Chemistry A, Vol. 7, Issue 41
H‐/dT‐MoS 2 ‐on‐MXene Heterostructures as Promising 2D Anode Materials for Lithium‐Ion Batteries: Insights from First Principles
journal, May 2019
- Shao, Yangfan; Gong, Penglai; Pan, Hui
- Advanced Theory and Simulations, Vol. 2, Issue 8
V 4 C 3 T x MXene: A promising active substrate for reactive surface modification and the enhanced electrocatalytic oxygen evolution activity
journal, January 2020
- Du, Cheng‐Feng; Sun, Xiaoli; Yu, Hong
- InfoMat, Vol. 2, Issue 5
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