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Title: Oxidant K edge x-ray emission spectroscopy of UF 4 and UO 2

The K-Edge (1s) x-ray emission spectroscopy of uranium tetrafluoride and uranium dioxide were compared to each other and to the results of a pair of earlier cluster calculations. Here, using a very simplified approach, it is possible to qualitatively reconstruct the main features of the x-ray emission spectra from the cluster calculation state energies and 2p percentages.
Authors:
 [1] ;  [2] ;  [3] ;  [3] ;  [3]
  1. Univ. of Wisconsin, Oshkosh, WI (United States). Dept. of Physics and Astronomy
  2. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  3. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Publication Date:
Report Number(s):
LLNL-JRNL-742730
Journal ID: ISSN 0734-2101; ark:/13030/qt3q7977vp; TRN: US1802701
Grant/Contract Number:
AC02-05CH11231; AC52-07NA27344
Type:
Accepted Manuscript
Journal Name:
Journal of Vacuum Science and Technology. A, Vacuum, Surfaces and Films
Additional Journal Information:
Journal Volume: 36; Journal Issue: 3; Journal ID: ISSN 0734-2101
Publisher:
American Vacuum Society
Research Org:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Chemical Sciences, Geosciences & Biosciences Division
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; 73 NUCLEAR PHYSICS AND RADIATION PHYSICS; emission spectroscopy; x-ray photoelectron spectroscopy; chemical compounds; nuclear fuel; biotechnology; classical electromagnetism; Materials science
OSTI Identifier:
1435130
Alternate Identifier(s):
OSTI ID: 1418862; OSTI ID: 1458631

Tobin, J. G., Yu, S. -W., Qiao, R., Yang, W. L., and Shuh, D. K.. Oxidant K edge x-ray emission spectroscopy of UF4 and UO2. United States: N. p., Web. doi:10.1116/1.5016393.
Tobin, J. G., Yu, S. -W., Qiao, R., Yang, W. L., & Shuh, D. K.. Oxidant K edge x-ray emission spectroscopy of UF4 and UO2. United States. doi:10.1116/1.5016393.
Tobin, J. G., Yu, S. -W., Qiao, R., Yang, W. L., and Shuh, D. K.. 2018. "Oxidant K edge x-ray emission spectroscopy of UF4 and UO2". United States. doi:10.1116/1.5016393.
@article{osti_1435130,
title = {Oxidant K edge x-ray emission spectroscopy of UF4 and UO2},
author = {Tobin, J. G. and Yu, S. -W. and Qiao, R. and Yang, W. L. and Shuh, D. K.},
abstractNote = {The K-Edge (1s) x-ray emission spectroscopy of uranium tetrafluoride and uranium dioxide were compared to each other and to the results of a pair of earlier cluster calculations. Here, using a very simplified approach, it is possible to qualitatively reconstruct the main features of the x-ray emission spectra from the cluster calculation state energies and 2p percentages.},
doi = {10.1116/1.5016393},
journal = {Journal of Vacuum Science and Technology. A, Vacuum, Surfaces and Films},
number = 3,
volume = 36,
place = {United States},
year = {2018},
month = {1}
}