High-Performance Screen-Printed Thermoelectric Films on Fabrics
Abstract
Printing techniques could offer a scalable approach to fabricate thermoelectric (TE) devices on flexible substrates for power generation used in wearable devices and personalized thermo-regulation. However, typical printing processes need a large concentration of binder additives, which often render a detrimental effect on electrical transport of the printed TE layers. Here, we report scalable screenprinting of TE layers on flexible fiber glass fabrics, by rationally optimizing the printing inks consisting of TE particles (p-type Bi0.5Sb1.5Te3 or n-type Bi2Te2.7Se0.3), binders, and organic solvents. We identified a suitable binder additive, methyl cellulose, which offers suitable viscosity for printability at a very small concentration (0.45–0.60 wt.%), thus minimizing its negative impact on electrical transport. Following printing, the binders were subsequently burnt off via sintering and hot pressing. We found that the nanoscale defects left behind after the binder burnt off became effective phonon scattering centers, leading to low lattice thermal conductivity in the printed n-type material. With the high electrical conductivity and low thermal conductivity, the screen-printed TE layers showed high room-temperature ZT values of 0.65 and 0.81 for p-type and n-type, respectively.
- Authors:
-
- Univ. of California, San Diego, CA (United States). Materials Science and Engineering Program
- Univ. of California, San Diego, CA (United States). Dept. of NanoEngineering
- Samsung Advanced Inst. of Technology, Suwon-si, Gyeonggi-do (Korea)
- Univ. of Seoul (Korea). Dept. of Materials Science and Engineering
- Univ. of California, San Diego, CA (United States). Dept. of Mechanical and Aerospace Engineering
- Univ. of California, San Diego, CA (United States). Materials Science and Engineering Program; Univ. of California, San Diego, CA (United States). Dept. of NanoEngineering
- Publication Date:
- Research Org.:
- Univ. of California, San Diego, CA (United States)
- Sponsoring Org.:
- USDOE Advanced Research Projects Agency - Energy (ARPA-E); National Science Foundation (NSF)
- OSTI Identifier:
- 1424227
- Grant/Contract Number:
- AR0000535; DGE-1144086
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Volume: 7; Journal Issue: 1; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 42 ENGINEERING; Devices for energy harvesting; Thermoelectric devices and materials
Citation Formats
Shin, Sunmi, Kumar, Rajan, Roh, Jong Wook, Ko, Dong-Su, Kim, Hyun-Sik, Kim, Sang Il, Yin, Lu, Schlossberg, Sarah M., Cui, Shuang, You, Jung-Min, Kwon, Soonshin, Zheng, Jianlin, Wang, Joseph, and Chen, Renkun. High-Performance Screen-Printed Thermoelectric Films on Fabrics. United States: N. p., 2017.
Web. doi:10.1038/s41598-017-07654-2.
Shin, Sunmi, Kumar, Rajan, Roh, Jong Wook, Ko, Dong-Su, Kim, Hyun-Sik, Kim, Sang Il, Yin, Lu, Schlossberg, Sarah M., Cui, Shuang, You, Jung-Min, Kwon, Soonshin, Zheng, Jianlin, Wang, Joseph, & Chen, Renkun. High-Performance Screen-Printed Thermoelectric Films on Fabrics. United States. https://doi.org/10.1038/s41598-017-07654-2
Shin, Sunmi, Kumar, Rajan, Roh, Jong Wook, Ko, Dong-Su, Kim, Hyun-Sik, Kim, Sang Il, Yin, Lu, Schlossberg, Sarah M., Cui, Shuang, You, Jung-Min, Kwon, Soonshin, Zheng, Jianlin, Wang, Joseph, and Chen, Renkun. Fri .
"High-Performance Screen-Printed Thermoelectric Films on Fabrics". United States. https://doi.org/10.1038/s41598-017-07654-2. https://www.osti.gov/servlets/purl/1424227.
@article{osti_1424227,
title = {High-Performance Screen-Printed Thermoelectric Films on Fabrics},
author = {Shin, Sunmi and Kumar, Rajan and Roh, Jong Wook and Ko, Dong-Su and Kim, Hyun-Sik and Kim, Sang Il and Yin, Lu and Schlossberg, Sarah M. and Cui, Shuang and You, Jung-Min and Kwon, Soonshin and Zheng, Jianlin and Wang, Joseph and Chen, Renkun},
abstractNote = {Printing techniques could offer a scalable approach to fabricate thermoelectric (TE) devices on flexible substrates for power generation used in wearable devices and personalized thermo-regulation. However, typical printing processes need a large concentration of binder additives, which often render a detrimental effect on electrical transport of the printed TE layers. Here, we report scalable screenprinting of TE layers on flexible fiber glass fabrics, by rationally optimizing the printing inks consisting of TE particles (p-type Bi0.5Sb1.5Te3 or n-type Bi2Te2.7Se0.3), binders, and organic solvents. We identified a suitable binder additive, methyl cellulose, which offers suitable viscosity for printability at a very small concentration (0.45–0.60 wt.%), thus minimizing its negative impact on electrical transport. Following printing, the binders were subsequently burnt off via sintering and hot pressing. We found that the nanoscale defects left behind after the binder burnt off became effective phonon scattering centers, leading to low lattice thermal conductivity in the printed n-type material. With the high electrical conductivity and low thermal conductivity, the screen-printed TE layers showed high room-temperature ZT values of 0.65 and 0.81 for p-type and n-type, respectively.},
doi = {10.1038/s41598-017-07654-2},
journal = {Scientific Reports},
number = 1,
volume = 7,
place = {United States},
year = {Fri Aug 04 00:00:00 EDT 2017},
month = {Fri Aug 04 00:00:00 EDT 2017}
}
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