Progress in Tandem Solar Cells Based on Hybrid Organic-Inorganic Perovskites

Chen, Bo; Zheng, Xiaopeng; Bai, Yang; Padture, Nitin P.; Huang, Jinsong

doi:10.1002/aenm.201602400

Title: Progress in Tandem Solar Cells Based on Hybrid Organic-Inorganic Perovskites

Journal Article · 06 March 2017 · Advanced Energy Materials

DOI: https://doi.org/10.1002/aenm.201602400 · OSTI ID:1418514

Chen, Bo ^[1]; Zheng, Xiaopeng ^[1]; Bai, Yang ^[1]; Padture, Nitin P. ^[2]; Huang, Jinsong ^[1]

Univ. of Nebraska, Lincoln, NE (United States). Dept. of Mechanical and Materials Engineering
Brown Univ., Providence, RI (United States)

Owing to their high efficiency, low-cost solution-processability, and tunable bandgap, perovskite solar cells (PSCs) made of hybrid organic-inorganic perovskite (HOIP) thin films are promising top-cell candidates for integration with bottom-cells based on Si or other low-bandgap solar-cell materials to boost the power conversion efficiency (PCE) beyond the Shockley-Quiesser (S-Q) limit. In this review, recent progress in such tandem solar cells based on the emerging PSCs is summarized and reviewed critically. Notable achievements for different tandem solar cell configurations including mechanically-stacked, optical coupling, and monolithically-integrated with PSCs as top-cells are described in detail. Highly-efficient semitransparent PSC top-cells with high transmittance in near-infrared (NIR) region are critical for tandem solar cells. Different types of transparent electrodes with high transmittance and low sheet-resistance for PSCs are reviewed, which presents a grand challenge for PSCs. The strategies to obtain wide-bandgap PSCs with good photo-stability are discussed. In conclusion, the PCE reduction due to reflection loss, parasitic absorption, electrical loss, and current mismatch are analyzed to provide better understanding of the performance of PSC-based tandem solar cells.

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Research Organization:: Univ. of Nebraska, Lincoln, NE (United States). Board of Regents

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE); USDOE

Grant/Contract Number:: EE0006709; DMR-1305913; OIA-1538893

OSTI ID:: 1418514

Alternate ID(s):: OSTI ID: 1401527

Journal Information:: Advanced Energy Materials, Vol. 7, Issue 14; ISSN 1614-6832

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Optical analysis of perovskite/silicon tandem solar cells Jiang, Yajie; Almansouri, Ibraheem; Huang, Shujuan Journal of Materials Chemistry C, Vol. 4, Issue 24 https://doi.org/10.1039/C6TC01276K	journal	January 2016
A Fast Deposition-Crystallization Procedure for Highly Efficient Lead Iodide Perovskite Thin-Film Solar Cells Xiao, Manda; Huang, Fuzhi; Huang, Wenchao Angewandte Chemie International Edition, Vol. 53, Issue 37 https://doi.org/10.1002/anie.201405334	journal	July 2014
Non-wetting surface-driven high-aspect-ratio crystalline grain growth for efficient hybrid perovskite solar cells Yongbo, Yuan,; Yuchuan, Shao,; Zhengguo, Xiao, The University of North Carolina at Chapel Hill University Libraries https://doi.org/10.17615/h36r-a084	text	January 2015
Perovskite-perovskite tandem photovoltaics with optimized bandgaps Eperon, Giles E.; Leijtens, Tomas; Bush, Kevin A. arXiv https://doi.org/10.48550/arxiv.1608.03920	text	January 2016

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