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Title: The effects of inorganic surface treatments on photogenerated carrier mobility and lifetime in PbSe quantum dot thin films

Authors:
; ; ; ;
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1405501
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Chemical Physics
Additional Journal Information:
Journal Name: Chemical Physics Journal Volume: 471 Journal Issue: C; Journal ID: ISSN 0301-0104
Publisher:
Elsevier
Country of Publication:
Netherlands
Language:
English

Citation Formats

Goodwin, E. D., Straus, Daniel B., Gaulding, E. Ashley, Murray, Christopher B., and Kagan, Cherie R. The effects of inorganic surface treatments on photogenerated carrier mobility and lifetime in PbSe quantum dot thin films. Netherlands: N. p., 2016. Web. doi:10.1016/j.chemphys.2015.07.031.
Goodwin, E. D., Straus, Daniel B., Gaulding, E. Ashley, Murray, Christopher B., & Kagan, Cherie R. The effects of inorganic surface treatments on photogenerated carrier mobility and lifetime in PbSe quantum dot thin films. Netherlands. https://doi.org/10.1016/j.chemphys.2015.07.031
Goodwin, E. D., Straus, Daniel B., Gaulding, E. Ashley, Murray, Christopher B., and Kagan, Cherie R. Wed . "The effects of inorganic surface treatments on photogenerated carrier mobility and lifetime in PbSe quantum dot thin films". Netherlands. https://doi.org/10.1016/j.chemphys.2015.07.031.
@article{osti_1405501,
title = {The effects of inorganic surface treatments on photogenerated carrier mobility and lifetime in PbSe quantum dot thin films},
author = {Goodwin, E. D. and Straus, Daniel B. and Gaulding, E. Ashley and Murray, Christopher B. and Kagan, Cherie R.},
abstractNote = {},
doi = {10.1016/j.chemphys.2015.07.031},
journal = {Chemical Physics},
number = C,
volume = 471,
place = {Netherlands},
year = {Wed Jun 01 00:00:00 EDT 2016},
month = {Wed Jun 01 00:00:00 EDT 2016}
}

Journal Article:
Free Publicly Available Full Text
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https://doi.org/10.1016/j.chemphys.2015.07.031

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Cited by: 14 works
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Works referenced in this record:

High Efficiency Carrier Multiplication in PbSe Nanocrystals: Implications for Solar Energy Conversion
journal, May 2004


Hybrid passivated colloidal quantum dot solids
journal, July 2012

  • Ip, Alexander H.; Thon, Susanna M.; Hoogland, Sjoerd
  • Nature Nanotechnology, Vol. 7, Issue 9
  • DOI: 10.1038/nnano.2012.127

Synthesis and characterization of nearly monodisperse CdE (E = sulfur, selenium, tellurium) semiconductor nanocrystallites
journal, September 1993

  • Murray, C. B.; Norris, D. J.; Bawendi, M. G.
  • Journal of the American Chemical Society, Vol. 115, Issue 19, p. 8706-8715
  • DOI: 10.1021/ja00072a025

Surfactant Ligand Removal and Rational Fabrication of Inorganically Connected Quantum Dots
journal, December 2011

  • Zhang, Haitao; Hu, Bo; Sun, Liangfeng
  • Nano Letters, Vol. 11, Issue 12
  • DOI: 10.1021/nl202892p

Ultrasensitive solution-cast quantum dot photodetectors
journal, July 2006

  • Konstantatos, Gerasimos; Howard, Ian; Fischer, Armin
  • Nature, Vol. 442, Issue 7099
  • DOI: 10.1038/nature04855

PbSe Quantum Dot Field-Effect Transistors with Air-Stable Electron Mobilities above 7 cm 2 V –1 s –1
journal, March 2013

  • Liu, Yao; Tolentino, Jason; Gibbs, Markelle
  • Nano Letters, Vol. 13, Issue 4
  • DOI: 10.1021/nl304753n

Formation and Stability of Size-, Shape-, and Structure-Controlled CdTe Nanocrystals:  Ligand Effects on Monomers and Nanocrystals
journal, November 2003

  • Yu, W. William; Wang, Y. Andrew; Peng, Xiaogang
  • Chemistry of Materials, Vol. 15, Issue 22
  • DOI: 10.1021/cm034729t

Effect of Metal Ions on Photoluminescence, Charge Transport, Magnetic and Catalytic Properties of All-Inorganic Colloidal Nanocrystals and Nanocrystal Solids
journal, August 2012

  • Nag, Angshuman; Chung, Dae Sung; Dolzhnikov, Dmitriy S.
  • Journal of the American Chemical Society, Vol. 134, Issue 33
  • DOI: 10.1021/ja301285x

Enhanced Mobility-Lifetime Products in PbS Colloidal Quantum Dot Photovoltaics
journal, December 2011

  • Jeong, Kwang S.; Tang, Jiang; Liu, Huan
  • ACS Nano, Vol. 6, Issue 1
  • DOI: 10.1021/nn2039164

Stoichiometric Control of Lead Chalcogenide Nanocrystal Solids to Enhance Their Electronic and Optoelectronic Device Performance
journal, February 2013

  • Oh, Soong Ju; Berry, Nathaniel E.; Choi, Ji-Hyuk
  • ACS Nano, Vol. 7, Issue 3
  • DOI: 10.1021/nn3057356

Unity quantum yield of photogenerated charges and band-like transport in quantum-dot solids
journal, September 2011

  • Talgorn, Elise; Gao, Yunan; Aerts, Michiel
  • Nature Nanotechnology, Vol. 6, Issue 11
  • DOI: 10.1038/nnano.2011.159

Electroluminescence from single monolayers of nanocrystals in molecular organic devices
journal, December 2002

  • Coe, Seth; Woo, Wing-Keung; Bawendi, Moungi
  • Nature, Vol. 420, Issue 6917
  • DOI: 10.1038/nature01217

Thiocyanate-Capped Nanocrystal Colloids: Vibrational Reporter of Surface Chemistry and Solution-Based Route to Enhanced Coupling in Nanocrystal Solids
journal, October 2011

  • Fafarman, Aaron T.; Koh, Weon-kyu; Diroll, Benjamin T.
  • Journal of the American Chemical Society, Vol. 133, Issue 39
  • DOI: 10.1021/ja206303g

Light-emitting diodes made from cadmium selenide nanocrystals and a semiconducting polymer
journal, August 1994

  • Colvin, V. L.; Schlamp, M. C.; Alivisatos, A. P.
  • Nature, Vol. 370, Issue 6488
  • DOI: 10.1038/370354a0

Highly Photoconductive CdSe Quantum-Dot Films: Influence of Capping Molecules and Film Preparation Procedure
journal, February 2010

  • Talgorn, Elise; Moysidou, Elli; Abellon, Ruben D.
  • The Journal of Physical Chemistry C, Vol. 114, Issue 8
  • DOI: 10.1021/jp9109546

X-ray Photoelectron Spectroscopy of CdSe Nanocrystals with Applications to Studies of the Nanocrystal Surface
journal, April 1994

  • Katari, J. E. Bowen; Colvin, V. L.; Alivisatos, A. P.
  • The Journal of Physical Chemistry, Vol. 98, Issue 15
  • DOI: 10.1021/j100066a034

Colloidal Nanocrystals with Molecular Metal Chalcogenide Surface Ligands
journal, June 2009


On the Mechanism of Lead Chalcogenide Nanocrystal Formation
journal, October 2006

  • Steckel, Jonathan S.; Yen, Brian K. H.; Oertel, David C.
  • Journal of the American Chemical Society, Vol. 128, Issue 40
  • DOI: 10.1021/ja062626g

Enhanced Thermopower in PbSe Nanocrystal Quantum Dot Superlattices
journal, August 2008

  • Wang, Robert Y.; Feser, Joseph P.; Lee, Jong-Soo
  • Nano Letters, Vol. 8, Issue 8, p. 2283-2288
  • DOI: 10.1021/nl8009704

Photoconductivity of PbSe Quantum-Dot Solids: Dependence on Ligand Anchor Group and Length
journal, October 2012

  • Gao, Yunan; Aerts, Michiel; Sandeep, C. S. Suchand
  • ACS Nano, Vol. 6, Issue 11
  • DOI: 10.1021/nn3029716

Quantum Junction Solar Cells
journal, January 2012

  • Tang, Jiang; Liu, Huan; Zhitomirsky, David
  • Nano Letters, Vol. 12, Issue 9
  • DOI: 10.1021/nl302436r

Role of Bond Adaptability in the Passivation of Colloidal Quantum Dot Solids
journal, August 2013

  • Thon, Susanna M.; Ip, Alexander H.; Voznyy, Oleksandr
  • ACS Nano, Vol. 7, Issue 9
  • DOI: 10.1021/nn4021983

Spectroscopic evaluation of surface functionalization efficiency in the preparation of mercaptopropyltrimethoxysilane self-assembled monolayers on glass
journal, April 2009

  • Pallavicini, Piersandro; Dacarro, Giacomo; Galli, Matteo
  • Journal of Colloid and Interface Science, Vol. 332, Issue 2
  • DOI: 10.1016/j.jcis.2008.12.063

Solution-Based Stoichiometric Control over Charge Transport in Nanocrystalline CdSe Devices
journal, September 2013

  • Kim, David K.; Fafarman, Aaron T.; Diroll, Benjamin T.
  • ACS Nano, Vol. 7, Issue 10
  • DOI: 10.1021/nn403132x

Designing High-Performance PbS and PbSe Nanocrystal Electronic Devices through Stepwise, Post-Synthesis, Colloidal Atomic Layer Deposition
journal, February 2014

  • Oh, Soong Ju; Berry, Nathaniel E.; Choi, Ji-Hyuk
  • Nano Letters, Vol. 14, Issue 3
  • DOI: 10.1021/nl404818z

The study of primary and secondary charge carriers in nanosecond pulse irradiated liquid dielectrics using a resonant microwave cavity
journal, June 1977

  • Warman, John M.; Infelta, Pierre P.; De Haas, Matthijs P.
  • Canadian Journal of Chemistry, Vol. 55, Issue 11
  • DOI: 10.1139/v77-309

Flexible and low-voltage integrated circuits constructed from high-performance nanocrystal transistors
journal, January 2012

  • Kim, David K.; Lai, Yuming; Diroll, Benjamin T.
  • Nature Communications, Vol. 3, Issue 1
  • DOI: 10.1038/ncomms2218

Confined-but-Connected Quantum Solids via Controlled Ligand Displacement
journal, June 2013

  • Baumgardner, William J.; Whitham, Kevin; Hanrath, Tobias
  • Nano Letters, Vol. 13, Issue 7
  • DOI: 10.1021/nl401298s

Depleted-Heterojunction Colloidal Quantum Dot Solar Cells
journal, May 2010

  • Pattantyus-Abraham, Andras G.; Kramer, Illan J.; Barkhouse, Aaron R.
  • ACS Nano, Vol. 4, Issue 6
  • DOI: 10.1021/nn100335g

Highly Effective Surface Passivation of PbSe Quantum Dots through Reaction with Molecular Chlorine
journal, November 2012

  • Bae, Wan Ki; Joo, Jin; Padilha, Lazaro A.
  • Journal of the American Chemical Society, Vol. 134, Issue 49
  • DOI: 10.1021/ja309783v

Short-Chain Alcohols Strip X-Type Ligands and Quench the Luminescence of PbSe and CdSe Quantum Dots, Acetonitrile Does Not
journal, December 2012

  • Hassinen, Antti; Moreels, Iwan; De Nolf, Kim
  • Journal of the American Chemical Society, Vol. 134, Issue 51
  • DOI: 10.1021/ja308861d

Free Charges Produced by Carrier Multiplication in Strongly Coupled PbSe Quantum Dot Films
journal, October 2011

  • Aerts, Michiel; Suchand Sandeep, C. S.; Gao, Yunan
  • Nano Letters, Vol. 11, Issue 10
  • DOI: 10.1021/nl202915p

Development of a microwave transmission setup for time-resolved measurements of the transient complex conductivity in bulk samples
journal, August 2005

  • Schins, J. M.; Prins, P.; Grozema, F. C.
  • Review of Scientific Instruments, Vol. 76, Issue 8
  • DOI: 10.1063/1.2008978

The detection of electrons in pulse irradiated liquid hydrocarbons by microwave absorption
journal, October 1973


The study of charge carrier kinetics in semiconductors by microwave conductivity measurements. II.
journal, February 1988

  • Kunst, M.; Beck, G.
  • Journal of Applied Physics, Vol. 63, Issue 4
  • DOI: 10.1063/1.340013

Ligand Exchange and the Stoichiometry of Metal Chalcogenide Nanocrystals: Spectroscopic Observation of Facile Metal-Carboxylate Displacement and Binding
journal, November 2013

  • Anderson, Nicholas C.; Hendricks, Mark P.; Choi, Joshua J.
  • Journal of the American Chemical Society, Vol. 135, Issue 49, p. 18536-18548
  • DOI: 10.1021/ja4086758

Controlling the Trap State Landscape of Colloidal CdSe Nanocrystals with Cadmium Halide Ligands
journal, January 2015

  • Greaney, Matthew J.; Couderc, Elsa; Zhao, Jing
  • Chemistry of Materials, Vol. 27, Issue 3
  • DOI: 10.1021/cm503529j

PbSe Nanocrystal Solids for n- and p-Channel Thin Film Field-Effect Transistors
journal, October 2005


Solution-processed PbS quantum dot infrared photodetectors and photovoltaics
journal, January 2005

  • McDonald, Steven A.; Konstantatos, Gerasimos; Zhang, Shiguo
  • Nature Materials, Vol. 4, Issue 2
  • DOI: 10.1038/nmat1299

Colloidal-quantum-dot photovoltaics using atomic-ligand passivation
journal, September 2011

  • Tang, Jiang; Kemp, Kyle W.; Hoogland, Sjoerd
  • Nature Materials, Vol. 10, Issue 10
  • DOI: 10.1038/nmat3118

Effects of Post-Synthesis Processing on CdSe Nanocrystals and Their Solids: Correlation between Surface Chemistry and Optoelectronic Properties
journal, November 2014

  • Goodwin, E. D.; Diroll, Benjamin T.; Oh, Soong Ju
  • The Journal of Physical Chemistry C, Vol. 118, Issue 46
  • DOI: 10.1021/jp5076912

In Situ Repair of High-Performance, Flexible Nanocrystal Electronics for Large-Area Fabrication and Operation in Air
journal, August 2013

  • Choi, Ji-Hyuk; Oh, Soong Ju; Lai, Yuming
  • ACS Nano, Vol. 7, Issue 9
  • DOI: 10.1021/nn403752d

Controlled growth of tetrapod-branched inorganic nanocrystals
journal, May 2003

  • Manna, Liberato; Milliron, Delia J.; Meisel, Andreas
  • Nature Materials, Vol. 2, Issue 6, p. 382-385
  • DOI: 10.1038/nmat902

Long-range orientation and atomic attachment of nanocrystals in 2D honeycomb superlattices
journal, May 2014


N-Type Colloidal-Quantum-Dot Solids for Photovoltaics
journal, September 2012

  • Zhitomirsky, David; Furukawa, Melissa; Tang, Jiang
  • Advanced Materials, Vol. 24, Issue 46, p. 6181-6185
  • DOI: 10.1002/adma.201202825

The study of charge carrier kinetics in semiconductors by microwave conductivity measurements
journal, November 1986

  • Kunst, M.; Beck, G.
  • Journal of Applied Physics, Vol. 60, Issue 10
  • DOI: 10.1063/1.337612

Photodetectors based on treated CdSe quantum-dot films
journal, November 2005

  • Oertel, David C.; Bawendi, Moungi G.; Arango, Alexi C.
  • Applied Physics Letters, Vol. 87, Issue 21
  • DOI: 10.1063/1.2136227

Activating Carrier Multiplication in PbSe Quantum Dot Solids by Infilling with Atomic Layer Deposition
journal, May 2013

  • ten Cate, Sybren; Liu, Yao; Suchand Sandeep, C. S.
  • The Journal of Physical Chemistry Letters, Vol. 4, Issue 11
  • DOI: 10.1021/jz4007492

Schottky Solar Cells Based on Colloidal Nanocrystal Films
journal, October 2008

  • Luther, Joseph M.; Law, Matt; Beard, Matthew C.
  • Nano Letters, Vol. 8, Issue 10
  • DOI: 10.1021/nl802476m

Highly Efficient Multiple Exciton Generation in Colloidal PbSe and PbS Quantum Dots
journal, May 2005

  • Ellingson, Randy J.; Beard, Matthew C.; Johnson, Justin C.
  • Nano Letters, Vol. 5, Issue 5, p. 865-871
  • DOI: 10.1021/nl0502672

Charge transport in mixed CdSe and CdTe colloidal nanocrystal films
journal, October 2010


Air-Stable All-Inorganic Nanocrystal Solar Cells Processed from Solution
journal, October 2005

  • Gur, Ilan; Fromer, Neil A.; Geier, Michael L.
  • Science, Vol. 310, Issue 5747, p. 462-465
  • DOI: 10.1126/science.1117908

Theory of optical and microwave properties of microscopically inhomogeneous materials
journal, June 1977


Band-like transport, high electron mobility and high photoconductivity in all-inorganic nanocrystal arrays
journal, April 2011

  • Lee, Jong-Soo; Kovalenko, Maksym V.; Huang, Jing
  • Nature Nanotechnology, Vol. 6, Issue 6
  • DOI: 10.1038/nnano.2011.46

Infrared Colloidal Quantum Dots for Photovoltaics: Fundamentals and Recent Progress
journal, September 2010


Bandlike Transport in Strongly Coupled and Doped Quantum Dot Solids: A Route to High-Performance Thin-Film Electronics
journal, April 2012

  • Choi, Ji-Hyuk; Fafarman, Aaron T.; Oh, Soong Ju
  • Nano Letters, Vol. 12, Issue 5
  • DOI: 10.1021/nl301104z

Time-resolved microwave conductivity. Part 2.—Quantum-sized TiO 2 and the effect of adsorbates and light intensity on charge-carrier dynamics
journal, January 1994

  • Martin, Scot T.; Herrmann, Hartmut; Hoffmann, Michael R.
  • J. Chem. Soc., Faraday Trans., Vol. 90, Issue 21
  • DOI: 10.1039/FT9949003323

Wave-Number-Dependent Dielectric Function of Semiconductors
journal, December 1962


High charge-carrier mobility enables exploitation of carrier multiplication in quantum-dot films
journal, August 2013

  • Sandeep, C. S. Suchand; Cate, Sybren ten; Schins, Juleon M.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3360