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Title: The Effect of Thermal Annealing on Charge Transport in Organolead Halide Perovskite Microplate Field-Effect Transistors

Abstract

Transformation of unipolar n-type semiconductor behavior to ambipolar and finally to unipolar p-type behavior in CH3NH3PbI3 microplate field-effect transistors by thermal annealing is reported. The photoluminescence spectra essentially maintain the same features before and after the thermal annealing process, demonstrating that the charge transport measurement provides a sensitive way to probe low-concentration defects in perovskite materials.

Authors:
 [1];  [2];  [1];  [2];  [3];  [2];  [1];  [4];  [3]
+ Show Author Affiliations
  1. Univ. of California, Los Angeles, CA (United States). Dept. of Chemistry and Biochemistry
  2. Univ. of California, Los Angeles, CA (United States). Dept. of Materials Science and Engineering
  3. Univ. of California, Los Angeles, CA (United States). Dept. of Chemistry and Biochemistry. California Nanosystems Inst.
  4. Univ. of California, Los Angeles, CA (United States). Dept. of Materials Science and Engineering. California Nanosystems Inst.
Publication Date:
Research Org.:
Univ. of California, Los Angeles, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
OSTI Identifier:
1533025
Alternate Identifier(s):
OSTI ID: 1401029
Grant/Contract Number:  
SC0008055; EFRI-1433541
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Volume: 29; Journal Issue: 4; Journal ID: ISSN 0935-9648
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; graphene contact; perovskite microplate transistors; thermal annealing

Citation Formats

Li, Dehui, Cheng, Hung-Chieh, Wang, Yiliu, Zhao, Zipeng, Wang, Gongming, Wu, Hao, He, Qiyuan, Huang, Yu, and Duan, Xiangfeng. The Effect of Thermal Annealing on Charge Transport in Organolead Halide Perovskite Microplate Field-Effect Transistors. United States: N. p., 2016. Web. doi:10.1002/adma.201601959.
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Li, Dehui, Cheng, Hung-Chieh, Wang, Yiliu, Zhao, Zipeng, Wang, Gongming, Wu, Hao, He, Qiyuan, Huang, Yu, & Duan, Xiangfeng. The Effect of Thermal Annealing on Charge Transport in Organolead Halide Perovskite Microplate Field-Effect Transistors. United States. https://doi.org/10.1002/adma.201601959
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Li, Dehui, Cheng, Hung-Chieh, Wang, Yiliu, Zhao, Zipeng, Wang, Gongming, Wu, Hao, He, Qiyuan, Huang, Yu, and Duan, Xiangfeng. Wed . "The Effect of Thermal Annealing on Charge Transport in Organolead Halide Perovskite Microplate Field-Effect Transistors". United States. https://doi.org/10.1002/adma.201601959. https://www.osti.gov/servlets/purl/1533025.
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@article{osti_1533025,
title = {The Effect of Thermal Annealing on Charge Transport in Organolead Halide Perovskite Microplate Field-Effect Transistors},
author = {Li, Dehui and Cheng, Hung-Chieh and Wang, Yiliu and Zhao, Zipeng and Wang, Gongming and Wu, Hao and He, Qiyuan and Huang, Yu and Duan, Xiangfeng},
abstractNote = {Transformation of unipolar n-type semiconductor behavior to ambipolar and finally to unipolar p-type behavior in CH3NH3PbI3 microplate field-effect transistors by thermal annealing is reported. The photoluminescence spectra essentially maintain the same features before and after the thermal annealing process, demonstrating that the charge transport measurement provides a sensitive way to probe low-concentration defects in perovskite materials.},
doi = {10.1002/adma.201601959},
journal = {Advanced Materials},
number = 4,
volume = 29,
place = {United States},
year = {Wed Nov 16 00:00:00 EST 2016},
month = {Wed Nov 16 00:00:00 EST 2016}
}
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Journal Article:
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Publisher's Version of Record
https://doi.org/10.1002/adma.201601959
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