High Photoluminescence Quantum Yield in Band Gap Tunable Bromide Containing Mixed Halide Perovskites

Sutter-Fella, Carolin M.; Li, Yanbo; Amani, Matin; Ager, Joel W.; Toma, Francesca M.; Yablonovitch, Eli; Sharp, Ian D.; Javey, Ali

doi:10.1021/acs.nanolett.5b04884

Title: High Photoluminescence Quantum Yield in Band Gap Tunable Bromide Containing Mixed Halide Perovskites

Journal Article · Sun Dec 20 19:00:00 EST 2015 · Nano Letters

DOI: https://doi.org/10.1021/acs.nanolett.5b04884 · OSTI ID:1393011

Sutter-Fella, Carolin M. ^[1]; Li, Yanbo ^[2]; Amani, Matin ^[1]; Ager, Joel W. ^[1]; Toma, Francesca M. ^[2]; Yablonovitch, Eli ^[1]; Sharp, Ian D. ^[2]; Javey, Ali ^[1]

Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

Hybrid organic-inorganic halide perovskite based semiconductor materials are attractive for use in a wide range of optoelectronic devices because they combine the advantages of suitable optoelectronic attributes and simultaneously low-cost solution processability. Here, we present a two-step low-pressure vapor-assisted solution process to grow high quality homogeneous CH₃NH₃PbI_3-xBr_x perovskite films over the full band gap range of 1.6-2.3 eV. Photoluminescence light-in versus light-out characterization techniques are used to provide new insights into the optoelectronic properties of Br-containing hybrid organic-inorganic perovskites as a function of optical carrier injection by employing pump-powers over a 6 orders of magnitude dynamic range. The internal luminescence quantum yield of wide band gap perovskites reaches impressive values up to 30%. This high quantum yield translates into substantial quasi-Fermi level splitting and high "luminescence or optically implied" open-circuit voltage. Most importantly, both attributes, high internal quantum yield and high optically implied open-circuit voltage, are demonstrated over the entire band gap range (1.6 eV ≤ E_g ≤ 2.3 eV). These results establish the versatility of Br-containing perovskite semiconductors for a variety of applications and especially for the use as high-quality top cell in tandem photovoltaic devices in combination with industry dominant Si bottom cells. (Figure Presented).

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1393011

Journal Information:: Nano Letters, Journal Name: Nano Letters Journal Issue: 1 Vol. 16; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Characterization of trap states in perovskite films by simultaneous fitting of steady-state and transient photoluminescence measurements Fu, Xiao; Weber, Klaus J.; White, Thomas P. Journal of Applied Physics, Vol. 124, Issue 7 https://doi.org/10.1063/1.5029278	journal	August 2018
Temperature-dependent studies of exciton binding energy and phase-transition suppression in (Cs,FA,MA)Pb(I,Br) ₃ perovskites Ruf, Fabian; Aygüler, Meltem F.; Giesbrecht, Nadja APL Materials, Vol. 7, Issue 3 https://doi.org/10.1063/1.5083792	journal	March 2019
Photophysics of lead-free tin halide perovskite films and solar cells Handa, Taketo; Wakamiya, Atsushi; Kanemitsu, Yoshihiko APL Materials, Vol. 7, Issue 8 https://doi.org/10.1063/1.5109704	journal	August 2019
Surface morphological, optical and electrical characterization of methylammonium lead bromide perovskite (CH ₃ NH ₃ PbBr ₃ ) thin film Chaudhary, Jyoti; Choudhary, Shaily; Negi, Chandra Mohan Singh Physica Scripta, Vol. 94, Issue 10 https://doi.org/10.1088/1402-4896/ab2dc4	journal	August 2019
Electron transition and electron-hole recombination processes in epitaxial BaTiO ₃ films with embedded Co nanocrystals Shi, Deli; Xiong, Zhengwei; Li, Jun Materials Research Express, Vol. 6, Issue 10 https://doi.org/10.1088/2053-1591/ab37e8	journal	August 2019
Understanding macroscale functionality of metal halide perovskites in terms of nanoscale heterogeneities Song, Tze-Bin; Sharp, Ian D.; Sutter-Fella, Carolin M. Journal of Physics: Energy, Vol. 1, Issue 1 https://doi.org/10.1088/2515-7655/aaeee5	journal	December 2018
Beyond Bulk Lifetimes: Insights into Lead Halide Perovskite Films from Time-Resolved Photoluminescence Staub, Florian; Hempel, Hannes; Hebig, Jan-Christoph Physical Review Applied, Vol. 6, Issue 4 https://doi.org/10.1103/physrevapplied.6.044017	journal	October 2016
Time-resolved imaging of carrier transport in halide perovskite thin films and evidence for nondiffusive transport Sridharan, Aravindan; Noel, Nakita K.; Hwang, Hyeon Physical Review Materials, Vol. 3, Issue 12 https://doi.org/10.1103/physrevmaterials.3.125403	journal	December 2019
Triple-halide wide–band gap perovskites with suppressed phase segregation for efficient tandems Xu, Jixian; Boyd, Caleb C.; Yu, Zhengshan J. Science, Vol. 367, Issue 6482 https://doi.org/10.1126/science.aaz5074	journal	March 2020
Methodologies for high efficiency perovskite solar cells Park, Nam-Gyu Nano Convergence, Vol. 3, Issue 1 https://doi.org/10.1186/s40580-016-0074-x	journal	June 2016
Quantification of re-Absorption and re-emission processes to determine photon recycling efficiency in perovskite single crystals Q., Dong,; H., Wei,; Y., Fang, The University of North Carolina at Chapel Hill University Libraries https://doi.org/10.17615/57bk-3140	text	January 2017
Maximizing and stabilizing luminescence from halide perovskites with potassium passivation Abdi Jalebi, Mojtaba; Andaji Garmaroudi, Zahra; Cacovich, Stefania Springer Nature https://doi.org/10.17863/cam.18795	journalarticle	January 2018
A Highly Emissive Surface Layer in Mixed-Halide Multication Perovskites. Andaji-Garmaroudi, Zahra; Abdi-Jalebi, Mojtaba; Guo, Dengyang Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.43272	text	January 2019
Photobrightening in Lead Halide Perovskites: Observations, Mechanisms, and Future Potential Andaji-Garmaroudi, Z.; Anaya, M.; Pearson, Aj Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.46381	text	January 2020
Distributed Feedback Lasers Based on MAPbBr3 Pourdavoud, Neda; Mayer, André; Buchmüller, Maximilian University of Wuppertal https://doi.org/10.25926/emvc-jr58	text	January 2020
Temperature-dependent studies of exciton binding energy and phase-transition suppression in (Cs,FA,MA)Pb(I,Br)$_{3}$ perovskites Ruf, Fabian; Aygüler, Meltem F.; Giesbrecht, Nadja American Institute of Physics (AIP) https://doi.org/10.5445/ir/1000093765	text	January 2019

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