Electron transfer dynamics from single near infrared emitting lead sulfide–cadmium sulfide nanocrystals to titanium dioxide

Zang, Huidong; Routh, Prahlad K.; Meng, Qingping; Cotlet, Mircea

doi:10.1039/C7NR03500D

Title: Electron transfer dynamics from single near infrared emitting lead sulfide–cadmium sulfide nanocrystals to titanium dioxide

Abstract

Electron transfer is demonstrated between single near infrared emitting nanocrystals of PbS/CdS and titanium dioxide.

Authors:

Zang, Huidong ^[1]; Routh, Prahlad K. ^[2]; Meng, Qingping ^[3];

^[2]

Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials
Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials; Stony Brook Univ., NY (United States). Materials Science Dept.
Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics Dept.

Publication Date:: Fri Aug 25 00:00:00 EDT 2017

Research Org.:: Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1392254

Report Number(s):: BNL-114287-2017-JA
Journal ID: ISSN 2040-3364; NANOHL; KC0403020

Grant/Contract Number:: SC0012704

Resource Type:: Accepted Manuscript

Journal Name:: Nanoscale

Additional Journal Information:: Journal Volume: 9; Journal Issue: 38; Journal ID: ISSN 2040-3364

Publisher:: Royal Society of Chemistry

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; energy nanomaterials; quantum dots; solar photovoltaics; Center for Functional Nanomaterials

Citation Formats


                    Zang, Huidong, Routh, Prahlad K., Meng, Qingping, and Cotlet, Mircea. Electron transfer dynamics from single near infrared emitting lead sulfide–cadmium sulfide nanocrystals to titanium dioxide.  United States: N. p., 2017. 
Web.  doi:10.1039/C7NR03500D.

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                    Zang, Huidong, Routh, Prahlad K., Meng, Qingping, & Cotlet, Mircea. Electron transfer dynamics from single near infrared emitting lead sulfide–cadmium sulfide nanocrystals to titanium dioxide.  United States.  https://doi.org/10.1039/C7NR03500D

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                    Zang, Huidong, Routh, Prahlad K., Meng, Qingping, and Cotlet, Mircea. Fri .  
"Electron transfer dynamics from single near infrared emitting lead sulfide–cadmium sulfide nanocrystals to titanium dioxide".  United States.  https://doi.org/10.1039/C7NR03500D.  https://www.osti.gov/servlets/purl/1392254.

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@article{osti_1392254,

  title        = {Electron transfer dynamics from single near infrared emitting lead sulfide–cadmium sulfide nanocrystals to titanium dioxide},

  author       = {Zang, Huidong and Routh, Prahlad K. and Meng, Qingping and Cotlet, Mircea},

  abstractNote = {Electron transfer is demonstrated between single near infrared emitting nanocrystals of PbS/CdS and titanium dioxide.},

  doi          = {10.1039/C7NR03500D},

  journal      = {Nanoscale},

  number       = 38,

  volume       = 9,

  place        = {United States},

  year         = {Fri Aug 25 00:00:00 EDT 2017},

  month        = {Fri Aug 25 00:00:00 EDT 2017}

}

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Journal Article:

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https://doi.org/10.1039/C7NR03500D

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Works referencing / citing this record:

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Title: Electron transfer dynamics from single near infrared emitting lead sulfide–cadmium sulfide nanocrystals to titanium dioxide

Abstract

Citation Formats

Hole Transfer from Single Quantum Dots journal, October 2011

Facts and Artifacts in the Blinking Statistics of Semiconductor Nanocrystals journal, May 2010

Solution-processed PbS quantum dot infrared photodetectors and photovoltaics journal, January 2005

Fluorescence Intermittency in InP Self-Assembled Quantum Dots journal, March 2001

Random Telegraph Signal in the Photoluminescence Intensity of a Single Quantum Dot journal, February 1997

Suppressed Blinking and Auger Recombination in Near-Infrared Type-II InP/CdS Nanocrystal Quantum Dots journal, October 2012

Quantum Dot-Bridge-Fullerene Heterodimers with Controlled Photoinduced Electron Transfer journal, May 2011

Measurement of Emission Lifetime Dynamics and Biexciton Emission Quantum Yield of Individual InAs Colloidal Nanocrystals journal, November 2014

Continuous Distribution of Emission States from Single CdSe/ZnS Quantum Dots journal, April 2006

Colloidal PbS Quantum Dot Solar Cells with High Fill Factor journal, June 2010

Discrete Intensity Jumps and Intramolecular Electronic Energy Transfer in the Spectroscopy of Single Conjugated Polymer Molecules journal, August 1997

Photoluminenscence Blinking Dynamics of Colloidal Quantum Dots in the Presence of Controlled External Electron Traps journal, November 2011

Electron Transfer Dynamics from Single CdSe/ZnS Quantum Dots to TiO 2 Nanoparticles journal, June 2009

Photoluminescence Intermittency of InGaAs/GaAs Quantum Dots Confined in a Planar Microcavity journal, October 2005

On/off blinking and switching behaviour of single molecules of green fluorescent protein journal, July 1997

Thiols Passivate Recombination Centers in Colloidal Quantum Dots Leading to Enhanced Photovoltaic Device Efficiency journal, November 2008

Intermittent Electron Transfer Activity From Single CdSe/ZnS Quantum Dots journal, August 2008

Effective mass approximation for two extreme semiconductors: Band gap of PbS and CuBr nanoparticles journal, May 2004

Competition between Auger Recombination and Hot-Carrier Trapping in PL Intensity Fluctuations of Type II Nanocrystals journal, April 2014

Modified Power Law Behavior in Quantum Dot Blinking: A Novel Role for Biexcitons and Auger Ionization journal, January 2009

Identification of different emitting species in the red fluorescent protein DsRed by means of ensemble and single-molecule spectroscopy journal, November 2001

An Experimental Comparison of the Maximum Likelihood Estimation and Nonlinear Least-Squares Fluorescence Lifetime Analysis of Single Molecules journal, May 2001

Bright infrared quantum-dot light-emitting diodes through inter-dot spacing control journal, May 2012

Size-Dependent Electron Injection from Excited CdSe Quantum Dots into TiO 2 Nanoparticles journal, April 2007

Fluorescence Spectroscopy of Single Lead Sulfide Quantum Dots journal, March 2006

Electron Injection from Colloidal PbS Quantum Dots into Titanium Dioxide Nanoparticles journal, October 2008

An inverted polymer photovoltaic cell with increased air stability obtained by employing novel hole/electron collecting layers journal, January 2009

Simple model for the power-law blinking of single semiconductor nanocrystals journal, December 2002

Shell Thickness Dependent Photoinduced Hole Transfer in Hybrid Conjugated Polymer/Quantum Dot Nanocomposites: From Ensemble to Single Hybrid Level journal, May 2012

Two types of luminescence blinking revealed by spectroelectrochemistry of single quantum dots journal, November 2011

Strong Electronic Coupling and Ultrafast Electron Transfer between PbS Quantum Dots and TiO 2 Nanocrystalline Films journal, December 2011

Broadband-absorbing hybrid solar cells with efficiency greater than 3% based on a bulk heterojunction of PbS quantum dots and a low-bandgap polymer journal, January 2014

Nonradiative Energy Transfer from Individual CdSe/ZnS Quantum Dots to Single-Layer and Few-Layer Tin Disulfide journal, April 2016

Fluorescence intermittency in single cadmium selenide nanocrystals journal, October 1996

Interband and Intraband Optical Studies of PbSe Colloidal Quantum Dots journal, October 2002

Single Photon Counting from Individual Nanocrystals in the Infrared journal, May 2012

Intramolecular Directional Förster Resonance Energy Transfer at the Single-Molecule Level in a Dendritic System journal, November 2003

Influence of self-trapped states on the fluorescence intermittency of single molecules journal, August 2005

“On”/“off” fluorescence intermittency of single semiconductor quantum dots journal, July 2001

PbS Nanocrystal Emission Is Governed by Multiple Emissive States journal, September 2016

Trion Decay in Colloidal Quantum Dots journal, March 2009

Lead Salt Quantum Dots: the Limit of Strong Quantum Confinement journal, November 2000

Exciton−Trion Transitions in Single CdSe–CdS Core–Shell Nanocrystals journal, August 2009

Fluorescence Spectroscopy, Exciton Dynamics, and Photochemistry of Single Allophycocyanin Trimers journal, December 1998

Quantum Dot-Bridge-Fullerene Heterodimers with Controlled Photoinduced Electron Transfer journal, May 2011

Photo/Electrochemical Applications of Metal Sulfide/TiO 2 Heterostructures journal, November 2019

A tyrosinase-induced fluorescence immunoassay for detection of tau protein using dopamine-functionalized CuInS2/ZnS quantum dots journal, June 2019

Photostability and long-term preservation of a colloidal semiconductor-based single photon emitter in polymeric photonic structures journal, January 2019

Hole Transfer from Single Quantum Dots
journal, October 2011

Facts and Artifacts in the Blinking Statistics of Semiconductor Nanocrystals
journal, May 2010

Solution-processed PbS quantum dot infrared photodetectors and photovoltaics
journal, January 2005

Fluorescence Intermittency in InP Self-Assembled Quantum Dots
journal, March 2001

Random Telegraph Signal in the Photoluminescence Intensity of a Single Quantum Dot
journal, February 1997

Suppressed Blinking and Auger Recombination in Near-Infrared Type-II InP/CdS Nanocrystal Quantum Dots
journal, October 2012

Quantum Dot-Bridge-Fullerene Heterodimers with Controlled Photoinduced Electron Transfer
journal, May 2011

Measurement of Emission Lifetime Dynamics and Biexciton Emission Quantum Yield of Individual InAs Colloidal Nanocrystals
journal, November 2014

Continuous Distribution of Emission States from Single CdSe/ZnS Quantum Dots
journal, April 2006

Colloidal PbS Quantum Dot Solar Cells with High Fill Factor
journal, June 2010

Discrete Intensity Jumps and Intramolecular Electronic Energy Transfer in the Spectroscopy of Single Conjugated Polymer Molecules
journal, August 1997

Photoluminenscence Blinking Dynamics of Colloidal Quantum Dots in the Presence of Controlled External Electron Traps
journal, November 2011

Electron Transfer Dynamics from Single CdSe/ZnS Quantum Dots to TiO ₂ Nanoparticles
journal, June 2009

Photoluminescence Intermittency of InGaAs/GaAs Quantum Dots Confined in a Planar Microcavity
journal, October 2005

On/off blinking and switching behaviour of single molecules of green fluorescent protein
journal, July 1997

Thiols Passivate Recombination Centers in Colloidal Quantum Dots Leading to Enhanced Photovoltaic Device Efficiency
journal, November 2008

Intermittent Electron Transfer Activity From Single CdSe/ZnS Quantum Dots
journal, August 2008

Effective mass approximation for two extreme semiconductors: Band gap of PbS and CuBr nanoparticles
journal, May 2004

Competition between Auger Recombination and Hot-Carrier Trapping in PL Intensity Fluctuations of Type II Nanocrystals
journal, April 2014

Modified Power Law Behavior in Quantum Dot Blinking: A Novel Role for Biexcitons and Auger Ionization
journal, January 2009

Identification of different emitting species in the red fluorescent protein DsRed by means of ensemble and single-molecule spectroscopy
journal, November 2001

An Experimental Comparison of the Maximum Likelihood Estimation and Nonlinear Least-Squares Fluorescence Lifetime Analysis of Single Molecules
journal, May 2001

Bright infrared quantum-dot light-emitting diodes through inter-dot spacing control
journal, May 2012

Size-Dependent Electron Injection from Excited CdSe Quantum Dots into TiO ₂ Nanoparticles
journal, April 2007

Fluorescence Spectroscopy of Single Lead Sulfide Quantum Dots
journal, March 2006

Electron Injection from Colloidal PbS Quantum Dots into Titanium Dioxide Nanoparticles
journal, October 2008

An inverted polymer photovoltaic cell with increased air stability obtained by employing novel hole/electron collecting layers
journal, January 2009

Simple model for the power-law blinking of single semiconductor nanocrystals
journal, December 2002

Shell Thickness Dependent Photoinduced Hole Transfer in Hybrid Conjugated Polymer/Quantum Dot Nanocomposites: From Ensemble to Single Hybrid Level
journal, May 2012

Two types of luminescence blinking revealed by spectroelectrochemistry of single quantum dots
journal, November 2011

Strong Electronic Coupling and Ultrafast Electron Transfer between PbS Quantum Dots and TiO ₂ Nanocrystalline Films
journal, December 2011

Broadband-absorbing hybrid solar cells with efficiency greater than 3% based on a bulk heterojunction of PbS quantum dots and a low-bandgap polymer
journal, January 2014

Nonradiative Energy Transfer from Individual CdSe/ZnS Quantum Dots to Single-Layer and Few-Layer Tin Disulfide
journal, April 2016

Fluorescence intermittency in single cadmium selenide nanocrystals
journal, October 1996

Interband and Intraband Optical Studies of PbSe Colloidal Quantum Dots
journal, October 2002

Single Photon Counting from Individual Nanocrystals in the Infrared
journal, May 2012

Intramolecular Directional Förster Resonance Energy Transfer at the Single-Molecule Level in a Dendritic System
journal, November 2003

Influence of self-trapped states on the fluorescence intermittency of single molecules
journal, August 2005

“On”/“off” fluorescence intermittency of single semiconductor quantum dots
journal, July 2001

PbS Nanocrystal Emission Is Governed by Multiple Emissive States
journal, September 2016

Trion Decay in Colloidal Quantum Dots
journal, March 2009

Lead Salt Quantum Dots: the Limit of Strong Quantum Confinement
journal, November 2000

Exciton−Trion Transitions in Single CdSe–CdS Core–Shell Nanocrystals
journal, August 2009

Fluorescence Spectroscopy, Exciton Dynamics, and Photochemistry of Single Allophycocyanin Trimers
journal, December 1998

Quantum Dot-Bridge-Fullerene Heterodimers with Controlled Photoinduced Electron Transfer
journal, May 2011

Photo/Electrochemical Applications of Metal Sulfide/TiO ₂ Heterostructures
journal, November 2019

A tyrosinase-induced fluorescence immunoassay for detection of tau protein using dopamine-functionalized CuInS2/ZnS quantum dots
journal, June 2019

Photostability and long-term preservation of a colloidal semiconductor-based single photon emitter in polymeric photonic structures
journal, January 2019